4.5 Article

Direct Polariton-To-Electron Tunneling in Quantum Cascade Detectors Operating in the Strong Light-Matter Coupling Regime

期刊

PHYSICAL REVIEW APPLIED
卷 17, 期 4, 页码 -

出版社

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevApplied.17.044021

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资金

  1. French National Research Agency [ANR-19-CE24-0003-02, ANR-17-ASTR-0008-01, ANR-17-CE24-0016]
  2. European Union FET-Open Grant MIR-BOSE [737017]
  3. Agence Nationale de la Recherche (ANR) [ANR-17-ASTR-0008, ANR-17-CE24-0016, ANR-19-CE24-0003] Funding Source: Agence Nationale de la Recherche (ANR)

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The study focuses on the light-matter coupling phenomenon in midinfrared quantum cascade detectors, demonstrating that a refined semiclassical coupled modes theory is required to accurately describe the spectral features in the photocurrent. Through simulations, the resonant tunneling from the polaritonic states is identified as the predominant extraction mechanism in the system.
Modern optoelectronic devices rely on cavity electrodynamics concepts for improved performances, embedding the active medium in an optical cavity to enhance the light-matter coupling. This coupling rate is usually small compared to the electronic and photon energies. Despite several demonstrations, devices operating with much larger light-matter coupling strength, in the so-called strong light-matter coupling regime, are yet to be demonstrated as viable, practical candidates. One of the main technological obstacles that hamper their dissemination is the comprehension of the carrier current extraction and injection from and into strongly coupled light-matter states. Here, we study this fundamental phenomenon in midinfrared quantum cascade detectors (QCDs) operating in the moderate to strong light-matter coupling regime. They operate around lambda = 10 mu m with a minimum Rabi splitting of 9.3 meV. A simple model based on the usual description of transport in QCDs does not reproduce the polaritonic features in the photocurrent spectra. On the contrary, a more refined approach, based on the semiclassical coupled modes theory, is capable of reproducing both optical and electrical spectra with excellent agreement. By correlating absorption and photoresponse with the simulations, we demonstrate that-in this system-resonant tunneling from the polaritonic states appears to be the predominant extraction mechanism. The dark intersubband states do not have a significant role in the process, contrary to what happens in electrically injected polaritonic emitters.

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