☆ 4.5 Review

Review and Development of Anode Electrocatalyst Carriers for Direct Methanol Fuel Cell

ENERGY TECHNOLOGY (2022)

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Review Chemistry, Physical

A comprehensive and critical review on recent progress in anode catalyst for methanol oxidation reaction

Afdhal Yuda et al.

Summary: This paper reviews the synthesis of anode electrocatalysts for methanol oxidation reaction, with a focus on their activity and durability. It compares noble and non-noble metal catalysts and examines the effects of manipulating catalysts through various factors. It also discusses the challenges and approaches in making direct methanol fuel cells a reliable source of energy.

CATALYSIS REVIEWS-SCIENCE AND ENGINEERING (2022)

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Article Chemistry, Inorganic & Nuclear

Enhanced Electrocatalytic Performance of Pt Nanoparticles Incorporated CeO2 Nanorods on Polyaniline-Chitosan Support for Methanol Electrooxidation (Experimental and Statistical Analysis)

Mehri-Saddat Ekrami-Kakhki et al.

Summary: The study successfully synthesized Pt-CeO(2)NRs/PA-CH nanocomposite with enhanced electrocatalytic activity for methanol oxidation, making it a promising catalyst for fuel cells. Statistical analysis revealed the significant effects of temperature, methanol concentration, and scan rate on the anodic peak potential and current density of the reaction.

JOURNAL OF CLUSTER SCIENCE (2021)

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Article Chemistry, Applied

Mesoporous CeO2-C hybrid spheres as efficient support for platinum nanoparticles towards methanol electrocatalytic oxidation

Weili Li et al.

Summary: The research successfully prepared a hybrid material CeO2-C for improving the electrocatalytic performance of Pt catalyst, with CeO2-C showing superior support and conductivity, leading to enhanced catalytic performance for methanol oxidation reaction.

JOURNAL OF RARE EARTHS (2021)

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Article Chemistry, Physical

Probing the enhanced methanol electrooxidation mechanism on platinum-metal oxide catalyst

Ya-Wei Zhou et al.

Summary: The study employs Pt-SnO2 nanoflakes as a catalyst, where the electronic structure manipulation favors the selective enhancement of the non-CO pathway for electrochemical methanol oxidation reaction.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Chemistry, Multidisciplinary

Au nanowires with high aspect ratio and atomic shell of Pt-Ru alloy for enhanced methanol oxidation reaction

Xiran Zhu et al.

Summary: The study investigates a catalyst design strategy for the electrocatalysis of methanol oxidation reaction in direct methanol fuel cells. Different catalyst configurations were tested, with Au@Pt-ML@Ru-ML showing the best electrocatalytic activity and CO tolerance. This method offers a viable approach for achieving high noble-metal utilization efficiency and high catalytic performance.

CHINESE CHEMICAL LETTERS (2021)

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Review Environmental Sciences

Environmental aspects of fuel cells: A review

Mohammad Ali Abdelkareem et al.

Summary: Fossil fuels are the main energy supply globally but have environmental impacts, while fuel cells are efficient energy conversion devices. Fuel cells are considered more environmentally friendly and efficient than conventional energy sources, but still face operational and environmental challenges that need to be compared in context.

SCIENCE OF THE TOTAL ENVIRONMENT (2021)

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Review Engineering, Multidisciplinary

Recent Advances in Electrode Design Based on One-Dimensional Nanostructure Arrays for Proton Exchange Membrane Fuel Cell Applications

Shangfeng Du

Summary: 1D Pt-based electrocatalysts demonstrate excellent catalytic activities and stability in the oxygen reduction reaction. Research on 3D ordered electrodes has shown potential for high-performance PEMFCs, while addressing mass transfer and durability challenges of Pt/C nanoparticle electrodes.

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Article Materials Science, Ceramics

Hierarchical nanostructures of MgCo2O4 on reduced graphene oxide as a high-performance catalyst for methanol electro-oxidation

Mohammad Bagher Askari et al.

Summary: The hybrid of MgCo2O4 with reduced graphene oxide (rGO) serves as an efficient and low-cost catalyst for the anode of direct methanol fuel cells (DMFC). The pivotal role of rGO in the structure of MgCo2O4-rGO catalyst was demonstrated through various tests, showing significantly improved power density. Practical single-cell tests confirmed the suitability of the proposed catalyst for DMFC applications, with power density enhancements observed with MgCo2O4-rGO-based anode compared to MgCo2O4-based anode.

CERAMICS INTERNATIONAL (2021)

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Review Chemistry, Physical

Supported bimetallic nanoparticles as anode catalysts for direct methanol fuel cells: A review

Akaljot Kaur et al.

Summary: This article reviews the advancements in the field of supported bimetallic nanoparticles in direct methanol fuel cells, discussing the performance of BMNPs with varied structures, compositions, and morphologies on different support materials, and evaluating the pros and cons of various support materials.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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Review Chemistry, Multidisciplinary

Polyaniline-based nanocomposites for direct methanol fuel cells (DMFCs)-A Recent Review

Suba Lakshmi Madaswamy et al.

Summary: Polyaniline plays a significant role in direct methanol fuel cells due to its high conductivity, unique redox properties, high flexibility, better solubility, reasonable stability, ease of synthesis, and low cost. This review discusses in detail the nanocomposites of polyaniline with other electrochemically active materials and nitrogen-doped carbon materials derived from PANI-based nanocomposites.

JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY (2021)

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Article Electrochemistry

Poly (5-aminoindole)-modified TiO2NTs nanocomposites supported palladium as an anode catalyst for enhanced electrocatalytic oxidation of methanol

Mai Xu et al.

Summary: A facile method for developing anode catalyst for direct methanol fuel cells with high electrocatalytic activity and durability is reported here. The incorporation of PAIn within TiO2NTs matrix significantly enhances the electrocatalytic activity and stability of the fuel cell catalyst support. The electrocatalytic mass activity of the Ti/TiO2NTs/PAIn/Pd is much higher than commercial Pd black and Pt black, showing potential for fuel cell applications.

ELECTROCHIMICA ACTA (2021)

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Article Energy & Fuels

Atomic Layer Deposition of NiO on Self-Supported Co3O4 Nanoneedle Array for Electrocatalytic Methanol Oxidation Reaction

Jia Cheng et al.

Summary: In this study, a NiO-Co3O4 nanoneedle array was prepared using atomic layer deposition for methanol oxidation reaction in direct methanol fuel cells, showing promising catalytic activity and stability.

ENERGY TECHNOLOGY (2021)

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Article Chemistry, Multidisciplinary

Characterization and Electrocatalytic Features of PtPd and PdPt Bimetallic Nanoparticles for Methanol Electro-oxidation

America Higareda et al.

Summary: This study focuses on the comprehensive investigation of PtPd and PdPt bimetallic nanoparticles supported on Vulcan XC-72 carbon for methanol oxidation reaction in alkaline media. The optimal electrocatalyst identified was PtPd (1 : 0.5)/C, which outperformed commercial Pt/C with a significantly higher current density and improved CO anti-poisoning ability, offering valuable insights for the development of new and efficient electrocatalysts.

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Metal-semiconductor oxide (WO3@W) induces an efficient electro-photo synergistic catalysis for MOR and ORR

Zhongshui Li et al.

Summary: The study focuses on utilizing the metal-semiconductor contact mode to construct efficient electro-photo catalysts under irradiation. The findings demonstrate that oxide-derived metal nanostructures can significantly enhance the bifunctional electrocatalytic activity, providing a new approach for the application of direct methanol fuel cells.

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Review Thermodynamics

Polygeneration systems based on high temperature fuel cell (MCFC and SOFC) technology: System design, fuel types, modeling and analysis approaches

A. S. Mehr et al.

Summary: There is a growing interest in high temperature fuel cells for their potential in multi-service applications. Integration of SOFC and MCFC systems is receiving much attention for proposing polygeneration plants. The most common polygeneration designs involve utilizing the exhaust gases from fuel cell systems for heat recovery.

ENERGY (2021)

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Article Energy & Fuels

Vertically Aligned Few-Layer Crumpled MoS2 Hybrid Nanostructure on Porous Ni Foam toward Promising Binder-Free Methanol Electro-Oxidation Application

Arthi Gopalakrishnan et al.

Summary: The study presents a novel MoS2 nanosheet hybrid structure with excellent electrocatalytic performance on porous Ni foam. This unique nanomaterial architecture enables rapid charge transfer and shows promising potential for various electrochemical applications. The binder-free electrode exhibits outstanding methanol electro-oxidation performance with high current tolerance, durability, and low overpotential, making it a suitable candidate for catalytic and electrochemical applications.

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Zr-MOF@Polyaniline as an efficient platform for nickel deposition: Application to methanol electro-oxidation

Sara Sheikhi et al.

Summary: The Zr-MOF@PANI-Ni-NPs composite showed excellent electrocatalytic performance towards methanol oxidation reaction, with significantly improved electrochemistry of nickel observed on the electrode surface. Compared to stepwise-modified electrodes, the oxidation current of methanol was highly increased on Zr-MOF@PANI-Ni-NPs/GCE in alkaline solution.

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Recent advances in designing and tailoring nanofiber composite electrolyte membranes for high-performance proton exchange membrane fuel cells

Hang Wang et al.

Summary: The article discusses the importance of proton exchange membrane (PEM) in proton exchange membrane fuel cells (PEMFC) and the current research status of preparing nanofiber composite proton exchange membranes (NCPEMs) using nanocomposite technology. By introducing nanofibers, long-range proton transport channels can be formed and the skeleton can be reinforced to improve the performance of PEMFCs.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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FeNi-functionalized 3D N, P doped graphene foam as a noble metal-free bifunctional electrocatalyst for direct methanol fuel cells

Caijin Shi et al.

Summary: A novel 3D FeNi-functionalized N, P doped graphene foam electrocatalyst (FeNi@NP-GF) was prepared, showing enhanced catalytic performance in ORR reaction due to the synergistic effect of Fe/Ni and N species and multiple active sites in the 3D porous graphene material. Furthermore, FeNi@NP-GF also acted as a good support for Pt nanoparticles, exhibiting remarkable catalytic activity and high stability for methanol electrooxidation in acid medium.

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Pt-Ru/polyaniline/carbon nanotube composites with three-layer tubular structure for efficient methanol oxidation

Xiaoling Zhang et al.

Summary: The study successfully prepared Pt-Ru/polyaniline/carbon nanotubes composites with excellent performance, showing higher activity and stability compared to Pt/C and other catalysts.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Article Chemistry, Physical

In-situ loading synthesis of graphene supported PtCu nanocube and its high activity and stability for methanol oxidation reaction

Yi Yang et al.

Summary: A perfect PtCu nanocube with partial hollow structure was synthesized through a hydrothermal reaction, showing enhanced electrocatalytic activity and stability in methanol oxidation reaction. Control of shape-control additives and polymers played crucial roles in determining the final product morphology. In situ immobilization onto graphene further improved the catalytic performance and durability of PtCu nanocubes, possibly due to their unique cubic morphology and the synergistic effect of PtCu and CuI decorated on the surface and graphene.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Review Chemistry, Physical

Solid oxide fuel cell (SOFC) performance evaluation, fault diagnosis and health control: A review

Jingxuan Peng et al.

Summary: Solid oxide fuel cells are a promising alternative energy source for new energy vehicles, distributed power generation, and military equipment, offering advantages such as high efficiency, low noise, low emission, and flexible fuel. To commercialize them effectively, performance evaluation, fault diagnosis, and health control strategies are essential for improving cell performance and ensuring efficient and stable operation.

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Article Chemistry, Applied

Robust copper nanocrystal/nitrogen-doped carbon monoliths as carbon monoxide-resistant electrodes for methanol oxidation reaction

Fei Chen et al.

Summary: This research presents a simple strategy to synthesize copper nanocrystal/nitrogen-doped carbon monoliths as active and stable electrodes for methanol oxidation reaction. These Cu/N-C monoliths exhibit high electrical conductivity and mechanical robustness, allowing them to be used directly as electrodes for MOR without the need for substrates or additives.

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Article Chemistry, Physical

Testing PtCu Nanoparticles Supported on Highly Ordered Mesoporous Carbons CMK3 and CMK8 as Catalysts for Low-Temperature Fuel Cells

Julia Garcia-Cardona et al.

Summary: Pt(Cu) nanoparticles supported on CMK3 and CMK8 ordered mesoporous carbons have been synthesized by electroless deposition of Cu followed by galvanic exchange with Pt. The nanoparticles exhibit higher activity due to a PtCu alloy core covered by a Pt-rich shell, which is attributed to the favorable geometric and ligand effects of Cu on Pt reducing the adsorption energy of intermediates on Pt.

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Article Chemistry, Physical

The Effect of Tin Addition to Platinum Catalysts with Different Morphologies towards Methanol Electrooxidation in Alkaline Media

Rebecca P. R. Anjos et al.

Summary: Direct methanol fuel cells using anion exchange membranes have attracted great interest, and developing electrocatalysts for methanol electrooxidation reaction in alkaline media is crucial. The study investigated the effects of platinum nanoparticle morphology and the presence of tin oxide in the electrocatalysts. Results showed that cubic-shaped platinum nanoparticles with (100) preferential orientation exhibited higher catalytic activity in alkaline media, with Pt/C(100) showing the highest current density for MEOR. SnO2 was found to enhance the catalytic activity of polycrystalline platinum, while decreasing it for Pt(100).

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Article Chemistry, Multidisciplinary

Unveiling the enhanced electrocatalytic activity at electrochemically synthesized Pt-WOx hybrid nanostructure interfaces

Lee Seul Oh et al.

Summary: In this study, a simple synthesis strategy was utilized to prepare Pt-WOx hybrid nanostructures, which exhibited excellent catalytic hydrogen evolution reaction performance. The Pt mass activity was approximately 17 times higher than that of commercial Pt catalysts, and the turnover frequency was 7.4 times higher. The enhanced electrocatalytic performance is attributed to the creation of Pt-WOx interfacial sites.

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One-step fabrication of CuO-doped TiO2 nanotubes enhanced the catalytic activity of Pt nanoparticles towards the methanol oxidation reaction in acid media

Qinglan Fu et al.

Summary: This study presents a novel Pt-CuO-TiO2/C catalyst with excellent electrocatalytic properties for the methanol oxidation reaction, showing a high mass activity of 1537.3 mA mg(Pt)(-1) and great CO resistance. The catalyst also demonstrates outstanding electrochemical stability, making it an advanced electrocatalyst for fuel cell applications.

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Summary: The study focused on the preparation of M-doped WO3 (M = Sn or In) films via evaporation-driven deposition during low-speed dip coating, with Sn- and In-doping easily achieved by controlling the chemical composition. The crystallinity of the films varied with heating temperature, affecting the electrochromic response and stability, with In-WO3 films showing faster color change and good cycle stability in the visible wavelength region compared to WO3 or Sn-WO3 films.

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Mesoporous cobalt phosphate electrocatalyst prepared using liquid crystal template for methanol oxidation reaction in alkaline solution

Merfat S. Al-Sharif et al.

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Sungyool Bong et al.

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In situ growth of metal organic frameworks derived hierarchical hollow porous Co3O4/NiCo2O4 nanocomposites on nickel foam as self-supported flexible electrode for methanol electrocatalytic oxidation

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Wushuang Chen et al.

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Pt-Ru nanoparticles anchored on poly(brilliant cresyl blue) as a new polymeric support: Application as an efficient electrocatalyst in methanol oxidation reaction

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Enhanced electrocatalytic activity of PtCu bimetallic nanoparticles on CeO2/carbon nanotubes for methanol electro-oxidation

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Amorphous nickel coating on carbon nanotubes supported Pt nanoparticles as a highly durable and active electrocatalyst for methanol oxidation reaction

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Ultrafine Pt nanoparticles supported on double -shelled C/TiO 2 hollow spheres material as highly efficient methanol oxidation catalysts

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FePt nanoalloys on N-doped graphene paper as integrated electrode towards efficient formic acid electrooxidation

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Electrosynthesis of Co3O4 and Co(OH)(2) ultrathin nanosheet arrays for efficient electrocatalytic water splitting in alkaline and neutral media

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Nitrogen-doped porous carbon sphere supported Pt nanoparticles for methanol and ethanol electro-oxidation in alkaline media

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Histidine-assisted synthesis of CeO2 nanoparticles for improving the catalytic performance of Pt-based catalysts in methanol electrooxidation

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A comprehensive review on recent material development of passive direct methanol fuel cell

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Methanol Electrooxidation Reaction in Alkaline Medium on Glassy Carbon Electrode Modified with Ordered Mesoporous Ni/Al2O3

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Structurally defined SnO2 substrates, nanostructured Au/SnO2 interfaces, and their distinctive behavior in benzene and methanol oxidation

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High electrocatalytic performance of nitrogen-doped carbon nanofiber-supported nickel oxide nanocomposite for methanol oxidation in alkaline medium

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Synergetic effect of bimetallic Au-Ru/TiO2 catalysts for complete oxidation of methanol

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Strong and Robust Polyaniline-Based Supramolecular Hydrogels for Flexible Supercapacitors

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Palladium-Based Catalysts as Electrodes for Direct Methanol Fuel Cells: A Last Ten Years Review

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Review and advances of direct methanol fuel cells: Part II: Modeling and numerical simulation

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Porous Co3O4/NiO core/shell nanowire array with enhanced catalytic activity for methanol electro-oxidation

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One-step electrochemical synthesis of Pt-CeO2 composite thin films on a glassy carbon electrode

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Electrochemical-reduced graphene oxide-modified carbon fiber as Pt-Au nanoparticle support and its high efficient electrocatalytic activity for formic acid oxidation

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Rational design of galvanically replaced Pt-anchored electrospun WO3 nanofibers as efficient electrode materials for methanol oxidation

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Titanium nitride-carbon nanotube core-shell composites as effective electrocatalyst supports for low temperature fuel cells

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A facile soft-template synthesis of ordered mesoporous carbon/tungsten carbide composites with high surface area for methanol electrooxidation

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Support materials for PEMFC and DMFC electrocatalysts-A review

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CeO2/rGO/Pt sandwich nanostructure: rGO-enhanced electron transmission between metal oxide and metal nanoparticles for anodic methanol oxidation of direct methanol fuel cells

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Formation of Pt-TiO2-rGO 3-phase junctions with significantly enhanced electro-activity for methanol oxidation

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PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2012)

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Microwave-assisted one-pot synthesis of metal/metal oxide nanoparticles on graphene and their electrochemical applications

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Preparation of the Flexible Polypyrrole/Polypropylene Composite Fibrous Film for Electrochemical Capacitor

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Flexible and macroporous network-structured catalysts composed of conducting polymers and Pt/Ag with high electrocatalytic activity for methanol oxidation

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JOURNAL OF MATERIALS CHEMISTRY (2011)

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Pt nanoparticles supported on WO3/C hybrid materials and their electrocatalytic activity for methanol electro-oxidation

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Influence of ultrathin poly-(3,4-ethylenedioxythiophene) (PEDOT) film supports on the electrodeposition and electrocatalytic activity of discrete platinum nanoparticles

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JOURNAL OF SOLID STATE ELECTROCHEMISTRY (2011)

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Review Chemistry, Physical

Nanocatalyst for direct methanol fuel cell (DMFC)

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INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2010)

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Platinum particles supported on titanium nitride: an efficient electrode material for the oxidation of methanol in alkaline media

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Development of a self-supported single-wall carbon nanotube-based gas diffusion electrode with spatially well-defined reaction and diffusion layers

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JOURNAL OF POWER SOURCES (2010)

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Electrocatalytic activity of Pt nanoparticles deposited on porous TiO2 supports toward methanol oxidation

Chung-Shou Chen et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2009)

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Methanol Electro-Oxidation on Pt-Ru Alloy Nanoparticles Supported on Carbon Nanotubes

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ENERGIES (2009)

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Pt/Carbon Nanofiber Nanocomposites as Electrocatalysts for Direct Methanol Fuel Cells: Prominent Effects of Carbon Nanofiber Nanostructures

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Effect of the support properties on the preparation and performance of platinum catalysts supported on carbon nanofibers

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JOURNAL OF POWER SOURCES (2009)

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Tungsten trioxide nanorods as supports for platinum in methanol oxidation

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Platinum supported on functionalized ordered mesoporous carbon as electrocatalyst for direct methanol fuel cells

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JOURNAL OF POWER SOURCES (2007)

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Electrocatalytic enhancement of methanol oxidation by graphite nanofibers with a high loading of PtRu alloy nanoparticles

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CARBON (2007)

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Electro-oxidation of methanol on TiO2 nanotube supported platinum electrodes

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JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY (2006)

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An electrocatalyst for methanol oxidation based on tungsten trioxide microspheres and platinum

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Sol-gel derived WOx and WOx/Pt films for direct methanol fuel cell catalyst applications

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ELECTROCHIMICA ACTA (2005)

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Methanol oxidative fuel cell:: electrochemical synthesis and characterization of low-priced WO3-Pt anode material

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