期刊
ADVANCED ENERGY MATERIALS
卷 12, 期 22, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/aenm.202200435
关键词
photocatalysis; photosynthesis; plastic upcycling; selectivity; solar energy conversion
类别
资金
- National Natural Science Foundation of China [22005048]
- Natural Science Foundation of Jiangsu Province [BK20200399]
- Zhishan Young Scholar Program of Southeast University
- A*STAR under the AME IRG grant [A2083c0050]
- Singapore Ministry of Education Academic Research Fund Tier 1 grant [RT 05/19]
- Nanyang Technological University 5th ACE grant call
- 2021 American Chemical Society Green Chemistry Institute Pharmaceutical Roundtable Ignition Grant
This review comprehensively summarizes the recent advances in plastic conversion through photocatalysis, with a focus on the photocatalytic mechanism and the selective C-C and C-H bond transformations of plastics. The challenges and perspectives on establishing a sustainable and circular plastic economy are also discussed.
Plastic waste remains a global challenge due to the massive amounts being produced without satisfactory treatment technologies for recycling and upcycling. Photocatalytic processes are emerging as green and promising approaches to upcycle plastics into value-added products under mild conditions using sunlight as the energy source. In this review, the recent advances in plastic conversion through photocatalysis have been comprehensively summarized. Special emphasis is placed on the photocatalytic mechanism and the selective C-C and C-H bond transformations of plastics to access fuels, chemicals, and materials. Finally, the challenges and the perspectives on establishing a new paradigm toward a sustainable and circular plastic economy are also put forward.
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