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Article
Chemistry, Multidisciplinary
Subhajit Bhattacharjee et al.
Summary: A perovskite-based photoelectrochemical device is reported to produce H-2 fuel and reform waste substrates with high product selectivity and formation rates, utilizing an oxidation catalyst to generate value-added products. The device shows significantly higher activity compared to conventional photoreforming systems and offers versatility in treating various waste streams. This PEC platform demonstrates potential as a commercially viable alternative for waste utilization.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
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Yinwen Li et al.
Summary: Polyethylene terephthalate (PET) and CO2, two chemical wastes that urgently need to be transformed in the environment, are simultaneously converted in a one-pot catalytic process through the synergistic coupling of three reactions. The chemical equilibria of both reactions are shifted forward, leading to significantly enhanced PET depolymerization. This synergistic catalytic process provides an effective way to simultaneously recycle two wastes and produce high-value chemicals.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2022)
Article
Chemistry, Physical
Jianying Wang et al.
Summary: Upcycling plastic waste pollution for sustainable resources and energy is an ideal solution to environmental issues. This study reports an electrochemical upcycling approach using Cu-based nanowire catalysts to oxidize PET waste and produce valued chemicals and green hydrogen.
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
(2022)
Article
Chemistry, Physical
Yuhou Pei et al.
Summary: This study proposes a method of substituting the sluggish oxygen evolution reaction with glycerol oxidation reaction for efficient CO2 electroreduction, which achieves the coproduction of formate at both the cathode and anode. A highly efficient CO2ER system is successfully established with a specific catalyst, demonstrating the potential of non-noble metal catalysts for organic oxidation reactions.
JOURNAL OF MATERIALS CHEMISTRY A
(2022)
Article
Chemistry, Physical
Genxiang Wang et al.
Summary: Electrolytic systhesis technique is considered a promising avenue for producing fuels or chemicals, with the potential to convert CO2 into value-added products for carbonneutral goals. Challenges remain in practice due to the lack of high-performance and cost-effective electrocatalysts, as well as high energy consumption.
Article
Materials Science, Multidisciplinary
Lvlv Ji et al.
Summary: Through a temperature-controlled strategy, researchers have successfully prepared bimetallic Co-Fe phosphide nanoframes with a skeletal hollow structure, providing more accessible active sites and channels, exhibiting excellent catalytic activity for oxygen evolution reaction.
SCIENCE CHINA-MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Xinfa Wei et al.
Summary: This study presents a strategy for efficient formic acid synthesis by conducting concurrent cathodic CO2 reduction and anodic partial methanol oxidation reactions, resulting in significantly lowered potential and high Faraday efficiency in CO2 reduction.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Multidisciplinary Sciences
Xiao Zhang et al.
Summary: The study demonstrates that Pt1 and Ptn stabilized on α-MoC surface can catalyze the WGS reaction at low temperatures, preventing catalyst deactivation due to oxidation and showing high stability with a high metal-normalized turnover number.
Review
Chemistry, Multidisciplinary
Cheng Tang et al.
Summary: The emerging electrocatalytic refinery (e-refinery) is a more sustainable and environmentally friendly strategy for converting renewable feedstocks and energy sources into transportable fuels and chemicals. Challenges remain in understanding mechanistic aspects and materials design for complex reactions in e-refinery processes.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
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Article
Chemistry, Multidisciplinary
Shuheng Tian et al.
Summary: A one-pot catalytic method has been demonstrated to convert polylactic acid into alanine using a Ru/TiO2 catalyst and ammonia solution treatment. The process achieves a 77% yield of alanine at 140 degrees C with an overall selectivity of 94% through recycling experiments.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2021)
Review
Chemistry, Physical
Rui Li et al.
Summary: This review highlights the importance of integrating anode and cathode reactions for efficient use of electrical energy in electrocatalysis conversion processes, as well as the production of high-value substances. It provides a comprehensive overview of recent advances in co-electrolysis processes for valuable chemical production, discussing popular reactions such as hydrogen evolution and carbon dioxide reduction integrated with anodic oxidation reactions. Additionally, challenges and future prospects for these integrated reactions are proposed to benefit researchers and facilitate progress in the field.
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(2021)
Article
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Xingchen Jiao et al.
Summary: This article summarizes recent achievements in the conversion of plastics into valuable fuels under mild conditions, such as solar-driven conversion, enzyme-driven conversion, and low-temperature catalytic conversion. Other potentially used strategies and in situ characterization technologies in plastics degradation under moderate conditions are also presented.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Changsheng Cao et al.
Summary: The study introduces a novel approach to simultaneously produce formate on both electrodes through a selective electrocatalytic method, achieving high efficiency and reduced energy input. The coupled reaction system based on MOF-derived catalysts demonstrates excellent performance in formate electrosynthesis, providing high current densities and nearly 100% selectivity on both the anode and cathode.
ADVANCED MATERIALS
(2021)
Review
Chemistry, Multidisciplinary
Xi Chen et al.
Summary: This Minireview summarizes recent progress in the chemical upcycling of plastic wastes using various methods, mainly within the past three to five years. It introduces the concept of a plastic-based refinery, transforming plastic wastes into valuable compounds and discusses different chemical methods and emerging technologies.
Review
Chemistry, Multidisciplinary
Huan Chen et al.
Summary: Chemical recycling and upcycling processes are considered the most promising strategy for recovering value from waste plastics, but they often come with high costs and stringent conditions compared to current recycling methods.
Article
Chemistry, Physical
Peng Zhu et al.
Summary: Liquid fuels generated from the electrochemical CO2 reduction reaction have high energy densities and storage advantages, but are often produced in low concentrations and mixed with impurities due to limitations in current traditional CO2 electrolyzers and CO2RR catalysts. Strategies in reactor engineering and catalyst improvement are proposed to overcome these challenges and make electrochemical production of liquid fuels more competitive in the future.
Article
Chemistry, Physical
Hongfei Cheng et al.
Summary: This study presents a novel electrolyzer design that can simultaneously achieve efficient hydrogen generation, CO2 absorption, and methanol upgrading, using transition metal phosphides as low-cost catalysts. The electrolyzer exhibits a low working voltage and high Faraday efficiencies for hydrogen evolution and formic acid conversion reactions, under various current densities. The innovative strategy based on low-cost catalyst materials shows potential for simultaneous hydrogen production and CO2 capture.
Review
Chemistry, Multidisciplinary
M. R. Karimi Estahbanati et al.
Summary: This review discusses the latest advances and future trends in the chemical upcycling of waste plastics using processes such as photocatalytic, electrolytic, and microwave-assisted pyrolysis as more environmentally friendly alternatives. It highlights how transforming different types of plastics waste using alternative energy sources can result in value-added products, contributing to a more sustainable and circular economy.
Review
Multidisciplinary Sciences
Matthew MacLeo et al.
Summary: Plastic pollution that accumulates and is poorly reversible in the environment can have significant negative impacts such as changes to ecosystems, biological effects, and societal impacts. Therefore, a global response is needed to rapidly reduce plastic emissions through reductions in consumption of virgin plastic materials and internationally coordinated waste management strategies.
Review
Multidisciplinary Sciences
LaShanda T. J. Korley et al.
Summary: Chemical recycling and polymer upcycling offer solutions to the challenges of plastic waste heterogeneity and property reductions, enabling circularity and reducing energy consumption and environmental impacts. The industrial adoption of these approaches is encouraging and plays a critical role in addressing the fate of plastics and advancing next-generation materials design.
Article
Multidisciplinary Sciences
Hua Zhou et al.
Summary: This study investigates a nickel-cobalt phosphide electrocatalyst for electroreforming PET plastic into valuable chemicals and fuel. The process shows profitability at high current densities and the developed catalyst demonstrates excellent performance in achieving desired products.
NATURE COMMUNICATIONS
(2021)
Review
Chemistry, Physical
Feng-Yang Chen et al.
Summary: This review summarizes critical mechanisms that could influence the stability of the oxygen evolution reaction (OER) and discusses the importance of stability in large-scale electrolysis industrialization. Additionally, it provides catalyst and reactor design principles for overcoming OER stability challenges.
Review
Chemistry, Multidisciplinary
Genxiang Wang et al.
Summary: This article provides a comprehensive review of recent research progress on the selective electrocatalytic conversion of CO2 into value-added products. It covers the history and fundamental science of electrocatalytic CO2RR, the design, preparation, and performance evaluation of electrocatalysts, factors influencing the CO2RR, and associated theoretical calculations. Emphasis is placed on emerging trends in selective electrocatalytic conversion of CO2 and discussions on structure-performance relationships and mechanisms.
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(2021)
Review
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Yingjie Li et al.
ADVANCED ENERGY MATERIALS
(2020)
Review
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Lei Fan et al.
Review
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Ina Vollmer et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2020)
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Seungwoo Choi et al.
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
(2020)
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Song Song et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2019)
Review
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Md Golam Kibria et al.
ADVANCED MATERIALS
(2019)
Article
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Cameron Hepburn et al.
Article
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Saisai Zhou et al.
CHEMICAL ENGINEERING JOURNAL
(2018)
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Hui Yang et al.
ADVANCED ENERGY MATERIALS
(2018)
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Fengwang Li et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2017)
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Cao Guan et al.
ADVANCED ENERGY MATERIALS
(2017)
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Jianying Wang et al.
ADVANCED ENERGY MATERIALS
(2017)
Article
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Changzhou Yuan et al.
ADVANCED FUNCTIONAL MATERIALS
(2012)
Review
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Juan Carlos Serrano-Ruiz et al.
CHEMICAL SOCIETY REVIEWS
(2011)
Article
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Youngkook Kwon et al.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2011)
Article
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Nicola Armaroli et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2007)