期刊
SENSORS AND ACTUATORS B-CHEMICAL
卷 368, 期 -, 页码 -出版社
ELSEVIER SCIENCE SA
DOI: 10.1016/j.snb.2022.132146
关键词
PtSnx; RGO; SnO2; Hydrogen; Gas sensor
资金
- National Key Rsearch and Development Program of China [2020YFB2008702]
- National Natural Science Foundation of China [51422402, 51674067]
- Fundamental Research Funds for the Central Universities [N2101016, N180102032, N180408018]
- Liaoning Revitalization Talents Program [XLYC1807160]
This study successfully reduced the operating temperature and improved moisture resistance of H2 sensors by using PtSnx modified rGO-SnO2 nanocomposites. The nanocomposites exhibited ppm-level H2 sensing performance at 175°C and showed good moisture resistance, reproducibility, and long-term stability. The research suggests that PtSnx-rGO-SnO2 nanocomposites may be a promising material for high-performance H2 detection.
Currently, semiconductor sensors typically require high operating temperatures (> 200 ?) to detect H-2, which increases energy consumption and safety hazards. This work uses PtSnx to modify rGO-SnO2 nanocomposites to reduce the operating temperature and improve moisture resistance. PtSnx-rGO-SnO2 nanocomposites are synthesized by a simple reflow reaction and have ppm-level H(2 )sensing performance at 175 C with good moisture resistance. The PtSnx-rGO-SnO2 nanocomposite has a thickness of-20 nm. Spherical PtSnx nanoparticles and capsule-shaped SnO2 nanoparticles were grown on the rGO surface. The spherical PtSnx nanoparticles are-15 nm in diameter and the capsule-shaped SnO2 nanoparticles are-5 nm in diameter and-10 nm in length. The phase of PtSnx intermetallic compound varied as the Pt/Sn molar ratio increases. The 0.5 % PtSn2-rGO-SnO2 nanocomposites exhibited the highest response of 20.25 to 500 ppm H-2 at the optimal operating temperature of 175 ? with a short response/recovery times of 1 s/17 s. The 0.5 % PtSn2-rGO-SnO2 nanocomposites also had excellent moisture resistance, reproducibility, and long-term stability. This work reveals that PtSnx-rGO-SnO2 nanocomposites are a promising sensing material for high-performance H-2 detection.
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