4.7 Article

How do aerosols above the residual layer affect the planetary boundary layer height?

期刊

SCIENCE OF THE TOTAL ENVIRONMENT
卷 814, 期 -, 页码 -

出版社

ELSEVIER
DOI: 10.1016/j.scitotenv.2021.151953

关键词

Large-eddy simulation; Planetary boundary layer; Virtual dome effect; Aloft umbrella effect; Dome effective height

资金

  1. CAS Strategic Priority Research Program [XDA23020301]
  2. major science and technology project of Inner Mongolia Autonomous Region [2020ZD0013]
  3. National Natural Science Foundation of China [42061130215]
  4. Royal Society [NAF \R1\201354]

向作者/读者索取更多资源

The study reveals that absorption aerosols and scattering aerosols have different effects on the development of the planetary boundary layer (PBL). Absorption aerosols can promote the development of PBL and heat the morning residual layer (MRL), while scattering aerosols exhibit a similar suppression effect on PBL regardless of their vertical location. However, the role of different types of aerosols in the upper atmosphere needs further exploration.
We revealed that the absorption aerosol lying below or above the morning residual layer (MRL) promotes (stove effect, heating the MRL layer) or strongly inhibits (dome effect, heating the temperature inversion layer) the development of planetary boundary layer (PBL) after sunrise, while scattering aerosol exhibits similar suppression (surface or aloft umbrella effect) on the PBL regardless of its vertical location. However, the role of different type of aerosols (i.e., strong absorption aerosol and purely scattering aerosol) present from MRL to upper atmosphere remains lacking and therefore, needs to be further explored. Utilizing a large-eddy simulation model constrained by the in-situ observations in urban Beijing, we observed that the dome inhibition of absorption aerosols on PBL development becomes weaker as elevating the aerosol layer, and the effect (virtual dome effect) remains no change beyond a certain height, which is defined as the dome effective height z. This height z is highly related to the surface sensible heat flux. By comparison, the altitude of light-scattering aerosols relative to the MRL was less important. The scattering aerosols exhibit similar inhibition from MRL to upper atmosphere (aloft umbrella effect), but to a weaker extent than the virtual dome effect. The virtual dome effect and aloft umbrella effect play a leading role during some extremely polluted scenarios with deep aerosol layer, such as sandstorms and volcanic eruptions. Aerosol dome, virtual dome, and aloft umbrella effects, together with aerosol stove and surface umbrella effects, further advance the understanding on aerosol-PBL interactions, which is, more broadly, applied to interpret the impact of aerosol on PBL over other ecosystems as well as exoplanet atmospheres.

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