4.8 Article

Orderly disorder in magic-angle twisted trilayer graphene

期刊

SCIENCE
卷 376, 期 6589, 页码 193-+

出版社

AMER ASSOC ADVANCEMENT SCIENCE
DOI: 10.1126/science.abk1895

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资金

  1. Programmable Quantum Materials, an Energy Frontier Research Center - US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES) [DE-SC0019443]
  2. NSF MRSEC program through Columbia in the Center for Precision-Assembled Quantum Materials (PAQM) [DMR-2011738, DMR-2004691]
  3. Air Force Office of Scientific Research [FA9550-21-1-0378]
  4. STC Center for Integrated Quantum Materials
  5. NSF [DMR-1231319, DMR-2002850]
  6. ARO MURI grant [W911NF14-0247]
  7. NSF DMREF [1922165]
  8. FAS Division of Science, Research Computing Group at Harvard University
  9. Elemental Strategy Initiative by the MEXT, Japan [JPMXP0112101001]
  10. JSPS KAKENHI [19H05790, JP20H00354]
  11. Direct For Mathematical & Physical Scien
  12. Division Of Materials Research [1922165] Funding Source: National Science Foundation

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The magic-angle twisted trilayer graphene has shown a potential for engineering strongly correlated flat bands. Using low-temperature scanning tunneling microscopy, researchers have observed a strong reconstruction of the moire lattice in real trilayer samples, leading to the formation of localized twist-angle faults. These localized regions exhibit different electronic structures compared to the background regions, resulting in a doping-dependent, spatially granular electronic landscape.
Magic-angle twisted trilayer graphene (TTG) has recently emerged as a platform to engineer strongly correlated flat bands. We reveal the normal-state structural and electronic properties of TTG using low-temperature scanning tunneling microscopy at twist angles for which superconductivity has been observed. Real trilayer samples undergo a strong reconstruction of the moire lattice, which locks layers into near-magic-angle, mirror symmetric domains comparable in size with the superconducting coherence length. This relaxation introduces an array of localized twist-angle faults, termed twistons and moire solitons, whose electronic structure deviates strongly from the background regions, leading to a doping-dependent, spatially granular electronic landscape. The Fermi-level density of states is maximally uniform at dopings for which superconductivity has been observed in transport measurements.

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