期刊
MACROMOLECULAR MATERIALS AND ENGINEERING
卷 307, 期 7, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/mame.202100973
关键词
biopolymers; composite hydrogels; flexible electronics; freeze; thaw cycles; human motion detection; nanocellulose; strain sensors
资金
- National Research Foundation (NRF), South Africa
This study reports a poly(vinyl alcohol) (PVA)-based biocomposite hydrogel with good flexibility, toughness, and strain sensitivity. By incorporating conductive polypyrrole/bacterial nanocellulose composite material into the PVA-based hydrogel matrix, a hybrid hydrogel with excellent properties is prepared.
Hydrogels are becoming the default platform for flexible electronic applications-specifically, strain sensors. But the simultaneous realization of compliance, robustness, and strain sensitivity required, using environmentally friendly materials, remains challenging. Here a series of poly(vinyl alcohol) (PVA)-based biocomposite hydrogels, comprising variable quantities of nanocellulose and sodium alginate formed by freeze/thaw cycling, is reported. The results indicate that a hybrid hydrogel is prepared via the incorporation of conductive polypyrrole/bacterial nanocellulose composite material into the optimized PVA-based hydrogel matrix (yield strength = 6.0 MPa, elastic modulus = 2.4 MPa, stretchability >384%). The resulting hybrid material exhibits remarkable toughness, nonlinear conformability, and piezoresistivity and demonstrates good strain sensitivity over a considerable range of deformation (
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