4.7 Article

Comparative evaluation of artificial neural networks for the performance prediction of Pt-based catalysts in water gas shift reaction

期刊

INTERNATIONAL JOURNAL OF ENERGY RESEARCH
卷 46, 期 7, 页码 9602-9620

出版社

WILEY
DOI: 10.1002/er.7829

关键词

artificial neural networks; catalysis; machine learning; WGSR

资金

  1. Korea Institute of Energy Technology Evaluation and Planning (KETEP) - Korea government (MOTIE) [20214000000500]
  2. Basic Science Research Program through the National Research Foundation of Korea (NRF) - Ministry of Education [2019R1F1A106365312]
  3. Korea Institute of Energy Technology Evaluation & Planning (KETEP) [20214000000500] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

向作者/读者索取更多资源

In this study, four different ANNs were used for predicting the performance of Pt-based catalysts in water gas shift reaction, with the multilayer perceptron model showing the best performance. It was demonstrated how selecting the optimal ANN structure can improve prediction accuracy and reduce computational load.
Artificial neural networks (ANNs) methods have recently been used for modeling and predicting catalysis, which has been conventionally described using reaction kinetics. ANNs-based techniques for analyzing complex catalytic systems have shown a high level of accuracy and dependability. In contrast, there is still a lack of strategies to select an appropriate ANNs algorithm according to size and quality of data, the complexity of the reaction, and catalyst characteristics. In this study, four different ANNs were proposed for the performance prediction of Pt-based catalysts in water gas shift reaction: multilayer perceptron, long short-term memory, recurrent neural network, and gated recurrent unit. By identifying the optimal ANN structure such as training/testing dataset ratio, topology, and epochs, the capability of the ANNs is comparatively evaluated in terms of prediction accuracy, computational load, and the quantity of required data for model training. As a case study, the effect of types and contents of promoters and supports in Pt-based catalysts on CO conversion was analyzed. As a result, it was revealed that the multilayer perceptron model shows better performance than the others with the highest accuracy (mean square error = 0.0068) and lowest computation time. In addition, it was identified using the multiplayer perceptron model that Pt/Ca/TiO2 of 10 wt% Ca is the most favorable catalyst by achieving CO conversion over 90% at an operating temperature of 300 degrees C.

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