4.7 Article

Numerical model for static chamber measurement of multi-component landfill gas emissions and its application

期刊

ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
卷 29, 期 49, 页码 74225-74241

出版社

SPRINGER HEIDELBERG
DOI: 10.1007/s11356-022-20951-2

关键词

Landfill gas; Numerical model; Landfill cover; Static chamber; Relative error; Multi-components

资金

  1. Pioneer and Leading Goose R&D Program of Zhejiang [2022C03051]
  2. National Natural Science Foundation of China [41977223, 41931289]
  3. National Key R&D Program of China [2018YFC1802303, 2019YFC1806005]
  4. Natural Science Foundation of Zhejiang province [LR20E080002]

向作者/读者索取更多资源

The quantitative assessment of landfill gas emissions is crucial for evaluating the performance of landfill cover systems and gas collection systems. However, the use of static flux chamber technique may result in relative errors in measuring surface emissions of landfill gas. In this study, an integrated approach of in situ tests and numerical modeling was used to quantify the effects of chamber size, insertion depth, and pressure differential on the relative errors. The results showed that the proposed model based on the dusty-gas model (DGM) had a better capacity to predict gas transport compared to Blanc's method. Increasing the size and insertion depth of static chambers could reduce the relative error for CH4 and CO2 flux, while positive pressure differentials led to higher gas emission fluxes.
The quantitative assessment of landfill gas emissions is essential to assess the performance of the landfill cover and gas collection system. The relative error of the measured surface emission of landfill gas may be induced by the static flux chamber technique. This study aims to quantify effects of the size of the chamber, the insertion depth, pressure differential on the relative errors by using an integrated approach of in situ tests, and numerical modeling. A field experiment study of landfill gas emission is conducted by using a static chamber at one landfill site in Xi'an, Northwest China. Additionally, a two-dimensional axisymmetric numerical model for multi-component gas transport in the soil and the static chamber is developed based on the dusty-gas model (DGM). The proposed model is validated by the field data obtained in this study and a set of experimental data in the literature. The results show that DGM model has a better capacity to predict gas transport under a wider range of permeability compared to Blanc's method. This is due to the fact that DGM model can explain the interaction among gases (e.g., CH4, CO2, O-2, and N-2) and the Knudsen diffusion process while these mechanisms are not included in Blanc's model. Increasing the size and the insertion depth of static chambers can reduce the relative error for the flux of CH4 and CO2. For example, increasing the height of chambers from 0.55 to 1.1 m can decrease relative errors of CH4 and CO2 flux by 17% and 18%, respectively. Moreover, we find that gas emission fluxes for the case with positive pressure differential ( increment Pin-out) are greater than that of the case without considering pressure fluctuations. The Monte Carlo method was adopted to carry out the statistical analysis for quantifying the range of relative errors. The agreement of the measured field data and predicted results demonstrated that the proposed model has the capacity to quantify the emission of landfill gas from the landfill cover systems.

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