☆ 4.8 Review

Research Progress of a Composite Metal Oxide Catalyst for VOC Degradation

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2022)

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Review Environmental Sciences

Comprehensive review on catalytic degradation of Cl-VOCs under the practical application conditions

Fawei Lin et al.

Summary: This review provides a holistic perspective on the progress and achievements in catalytic degradation of chlorinated volatile organic compounds (Cl-VOCs), focusing on six representative Cl-VOCs and summarizing their degradation efficiency, long-term stability, and the effects of water and other components. Strategies for alleviating Cl poisoning are also highlighted to guide the development of catalysts for efficient elimination of Cl-VOCs under practical application conditions.

CRITICAL REVIEWS IN ENVIRONMENTAL SCIENCE AND TECHNOLOGY (2022)

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Article Engineering, Chemical

Structural characterizations of copper incorporated manganese oxide OMS-2 material and its efficiencies on toluene oxidation

C. Kaewbuddee et al.

Summary: The incorporation of high-valent copper into the K-OMS-2 catalyst framework significantly improves specific surface area, oxygen adsorption ratio, and Cu3+/Cu2+ ratio, enhancing catalytic activity and toluene removal at low reaction temperatures.

CHEMICAL ENGINEERING COMMUNICATIONS (2022)

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Article Engineering, Environmental

Synergistic mechanism of Cu-Mn-Ce oxides in mesoporous ceramic base catalyst for VOCs microwave catalytic combustion

Shuoyi Feng et al.

Summary: Cu-Mn-Ce mesoporous catalysts showed high efficiency in degrading volatile organic compounds (VOCs) under microwave catalytic combustion, achieving almost 100% removal efficiency. The excellent performance and stability of the catalyst can be attributed to the synergistic effects of the dispersed catalyst on the mesoporous carrier, which increases defects and enhances catalytic activity.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Engineering, Environmental

Nitrogen-rich layered carbon for adsorption of typical volatile organic compounds and low-temperature thermal regeneration

Li Tan et al.

Summary: Disc-like nitrogen-rich porous carbon materials (HAT-Xs) were synthesized with different C/N ratios by controlling the synthesis temperature. Among them, HAT-650 synthesized at 650 degrees Celsius exhibited the highest adsorption capacity and excellent reusability for ethyl acetate, making it a promising adsorbent for industrial applications.

JOURNAL OF HAZARDOUS MATERIALS (2022)

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Review Engineering, Environmental

Catalytic ozonation of VOCs at low temperature: A comprehensive review

Biyuan Liu et al.

Summary: VOCs abatement has attracted increasing interest due to their detrimental effects on the environment and human health. Catalytic ozonation with the assistance of ozone is considered as a feasible and effective method for VOCs elimination. This review systematically reviews the emerging advances of catalytic ozonation of different VOCs and discusses the reaction mechanisms and influencing factors.

JOURNAL OF HAZARDOUS MATERIALS (2022)

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Article Engineering, Environmental

Catalytic stability enhancement for pollutant removal via balancing lattice oxygen mobility and VOCs adsorption

Yuan Feng et al.

Summary: The Pt-1/MnOx catalyst shows different catalytic stabilities for the oxidation of toluene and iso-hexane, with improved stability for toluene oxidation after hydrogen reduction treatment. Balancing lattice oxygen mobility and organic compounds adsorption is crucial for the catalytic stability of Pt-1/MnOx.

JOURNAL OF HAZARDOUS MATERIALS (2022)

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Article Chemistry, Applied

Co-Mn oxides supported on hierarchical macro-mesoporous silica for CO and VOCs oxidation

S. Todorova et al.

Summary: The hierarchical macro-mesoporous silica (MMS) was used for catalyst support for oxidation reactions. The MMS was synthesized by the emulsions templating mechanism and modified separately or simultaneously with cobalt and manganese oxides. The modified materials showed partially blocked pores due to the oxides, with Co3O4 agglomerates and amorphous manganese oxide filling up the mesopores.

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Evaluation of the performance of catalytic oxidation of VOCs by a mixed oxide at a semi-pilot scale†

Rita Ribeiro et al.

Summary: This study evaluated the catalytic performance of a new mixed oxide Co-Al-Ce towards the oxidation of n-butanol and toluene, showing its excellent oxidation ability for n-butanol and promoting effect on the oxidation of toluene in mixtures. The mixed oxide outperformed the commercial catalyst in semi-pilot scale testing.

CANADIAN JOURNAL OF CHEMICAL ENGINEERING (2021)

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Electric field assisted benzene oxidation over Pt-Ce-Zr nano-catalysts at low temperature

Xuteng Zhao et al.

Summary: This study demonstrates that the combination of electric field with 1% Pt/Ce0.75Zr0.25O2 catalyst can improve the catalytic performance of benzene oxidation at low temperature, increase the adsorbed oxygen content on the catalyst surface, accelerate the generation and consumption of intermediate products, and produce new intermediate products.

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Formation of Catalytic Active Sites in Hydrothermally Obtained Binary Ceria-Iron Oxides: Composition and Preparation Effects

Tanya Tsoncheva et al.

Summary: A series of mesoporous cerium-iron binary oxides were prepared using CTAB as a template via a hydrothermal technique. The influence of Fe/Ce ratio and variations in preparation techniques on the properties of the materials were studied extensively. The shared Ce-O-Fe structures played a key role in the catalytic behavior, which could be controlled by the Fe/Ce ratio and the hydrothermal synthesis procedure.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Review Engineering, Environmental

How to achieve complete elimination of Cl-VOCs: A critical review on byproducts formation and inhibition strategies during catalytic oxidation

Fawei Lin et al.

Summary: This review examines the formation of byproducts in the catalytic oxidation of Cl-VOCs, with a focus on the potential risks posed by polychlorinated byproducts. Strategies to inhibit byproducts formation are explored, with an emphasis on the need to develop catalysts for the efficient and complete elimination of Cl-VOCs. Further research is needed to understand the migration and evolution routes of Cl species and design catalysts to achieve truly complete elimination of Cl-VOCs without secondary pollution.

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Article Chemistry, Physical

Boosting catalytic oxidation of propane over mixed-phase CoO-Co3O4 nanoparticles: Effect of CoO

Zhao Liu et al.

Summary: A series of pure Co3O4 and mixed-phase CoO-Co3O4 nanoparticles were successfully synthesized through a facile citric acid complex strategy, showing good catalytic activity and stability in propane conversion.

CHEMICAL PHYSICS (2021)

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Toluene catalytic oxidation over the layered MOx - δ-MnO2 (M = Pt, Ir, Ag) composites originated from the facile self-driving combustion method

Xuxu Zhai et al.

Summary: A series of layered manganese oxides catalysts were successfully prepared by self-driving combustion (SDC) technology using potassium permanganate and citric acid as precursors. Noble metals were employed to modulate the obtained manganese oxide matrix, resulting in new nanocatalysts with improved catalytic performance, with 0.5Pt-SDC-13 exhibiting the highest activity.

FUEL (2021)

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Article Materials Science, Multidisciplinary

Insights into key parameters of MnO2 catalyst toward high catalytic combustion performance

Luming Li et al.

Summary: The study found that the crystal phases and properties of MnO2 materials affect their catalytic activity and stability in toluene combustion, with alpha-MnO2 showing the best activity but inferior cycle stability, while delta-MnO2 has the easiest reduction property among all investigated manganese oxides.

JOURNAL OF MATERIALS SCIENCE (2021)

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Ternary mixed-oxide synergy effects of nano TiO2-FexOy-MOk (M = Mn, Ce, Co) on α-pinene catalytic oxidation process assisted by nonthermal plasma

Yan Gao et al.

Summary: The ternary nanocatalyst TiO2-FexOy-CoOk showed better catalytic oxidation properties, achieving high conversion efficiency of alpha-pinene and CO2 selectivity. The synergy effect between TiO2, FexOy and CoOk was stronger than other combinations, indicating a potential method to enhance odorous VOCs catalytic oxidation efficiency and reduce energy consumption.

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Article Chemistry, Multidisciplinary

Surface Modification of Cobalt-Manganese Mixed Oxide and Its Application for Low-Temperature Propane Catalytic Combustion

Yihao Liu et al.

Summary: The Co-Mn mixed metal oxide catalysts were synthesized using selective dissolve method, with 0.05 M-Co3Mn1 exhibiting the best catalytic activity, excellent stability, and regeneration ability.

CHEMISTRYSELECT (2021)

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Effects of Ni substitution on active oxygen species and electronic interactions over La0.8Ce0.2MnO3/mesoporous ZSM-5 for oxidizing C6H14

Jian Li et al.

Summary: The study investigated the effect of MZ molecular sieves and La0.8Ce0.2MnO3/MZ catalyst prepared from fly ash on hexane oxidation. Results showed that Ni substitution improved catalytic activity, with outer lattice oxygen species identified as the active oxygen species, while factors like specific surface area were relatively secondary.

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Reversible Absorption of Volatile Organic Compounds by Switchable-Hydrophilicity Solvents: A Case Study of Toluene with N,N-Dimethylcyclohexylamine

Yingjie Li et al.

Summary: In this study, the use of N,N-dimethylcyclohexylamine as a switchable-hydrophilicity solvent for the absorption of toluene showed excellent performance in separation processes. By bubbling CO2 and N-2, efficient desorption and separation were achieved, and the absorption capacity of the solvent remained comparable even after multiple cycles. This innovative and reversible remediation strategy utilizing switchable-hydrophilicity solvents has the potential to be a more environmentally friendly and energy-efficient alternative to traditional absorbents for reducing VOC pollution.

ACS OMEGA (2021)

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Review Chemistry, Physical

Recent advances in VOC elimination by catalytic oxidation technology onto various nanoparticles catalysts: a critical review

Yunlong Guo et al.

Summary: This review summarizes recent advances in catalytic elimination of VOCs using nanoparticles catalysts, including evaluation of catalyst performance, discussion of catalytic mechanisms, and summary of catalytic reactors. The integration of photothermocatalysis is also highlighted. Future research should focus on addressing scientific issues and challenges posed by VOC pollution.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Chemistry, Physical

Improved reactivity for toluene oxidation on MnOx/CeO2-ZrO2 catalyst by the synthesis of cubic-tetragonal interfaces

Caixia Zhou et al.

Summary: The CeO2-ZrO2 solid solutions with cubic-tetragonal interfaces were prepared and found to enhance catalytic activity for toluene oxidation. The interfaces promoted the adsorption of toluene and the formation of key intermediates at low temperatures, leading to higher catalytic activity. This promotion role might be related to the morphology, surface area and interface components of Ce-Zr supports.

APPLIED SURFACE SCIENCE (2021)

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Article Energy & Fuels

Excellent adsorptive performance of novel magnetic nano-adsorbent functionalized with 8-hydroxyquinoline-5-sulfonic acid for the removal of volatile organic compounds (BTX) vapors

Sinan Kutluay

Summary: In this study, Fe3O4/AC@SiO2@8HQ5SA nanoparticles were successfully synthesized and applied as an efficient adsorbent for the removal of BTX vapors. The adsorption capacity of Fe3O4/AC@SiO2@8HQ5SA towards BTX vapors was found to be excellent, and the material also demonstrated impressive reusability through multiple adsorption-desorption cycles.

FUEL (2021)

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Article Energy & Fuels

Effect of the A-site cation over spinel AMn2O4 (A = Cu2+, Ni2+, Zn2+) for toluene combustion: Enhancement of the synergy and the oxygen activation ability

Yongzhao Zhang et al.

Summary: Through substituting A(2+) and Mn3+, the study investigated the impact of the structure of AMn(2)O(4) spinel catalysts on toluene oxidation. The results showed that the catalytic activity is influenced by the substitution of A-site metal, enhancing low-temperature reducibility and chemisorption oxygen activity. The incorporation of A-site metal can improve the ability of the catalyst to activate molecular state oxygen, thus enhancing catalytic activity.

FUEL (2021)

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Article Energy & Fuels

Catalytic oxidation and reaction kinetics of low concentration benzene over CuxMnyOz/SiO2

Ruiming Fang et al.

Summary: By optimizing copper-manganese catalysts supported on silicon dioxide through adjusting the load of active material, the ratio of bimetal, and calcination conditions, the oxidation efficiency of VOCs was improved, leading to a decrease in activation energy, delay in deactivation, and enhancement in catalytic performance.

FUEL (2021)

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Article Chemistry, Physical

Enhanced catalytic oxidation of VOCs over porous Mn-based mullite synthesized by in-situ dismutation

Ruoyu Liu et al.

Summary: Porous SmMn2O5 mullite with higher Mn4+/Mn3+ ratios, better active oxygen desorption capacity, reducibility, and larger specific surface area was synthesized, which promoted the low-temperature catalytic oxidation of VOCs. Increasing the content of Mn4+ on the surface reduced surface defects and increased the proportion of surface lattice oxygen, facilitating the attack of VOC molecules by lattice oxygen.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Article Engineering, Environmental

Double redox process to synthesize CuO-CeO2 catalysts with strong Cu-Ce interaction for efficient toluene oxidation

Yiqing Zeng et al.

Summary: A novel double redox method was developed to synthesize highly active CuO-CeO2 (CuCe-DR) catalyst, which exhibits higher Ce3+ and Cu2+ ion concentrations and stronger Cu-Ce interaction compared to CuCe-C catalyst. CuCe-DR catalyst shows higher toluene oxidation performance and stability at low temperatures, attributed to the increased surface chemisorbed oxygen and improved redox properties.

JOURNAL OF HAZARDOUS MATERIALS (2021)

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Fabrication of MWCNTs/PDMS mixed matrix membranes for recovery of volatile aromatic compounds from brewed black tea

Jiawei Li et al.

Summary: The novel MWCNTs/PDMS mixed matrix membrane shows excellent separation performance for aromatic compounds in PV process, improving permeation fluxes for MetSa, linalool, and beta-Ionone. Additionally, the membrane demonstrates promising results in recovering VOCs from brewed tea.

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Effect of support nature on catalytic activity of the bimetallic RuCo nanoparticles for the oxidative removal of 1,2-dichloroethane

Xing Zhang et al.

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APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Energy & Fuels

Performance of transition metal (Cu, Fe and Co) modified SCR catalysts for simultaneous removal of NO and volatile organic compounds (VOCs) from coal-fired power plant flue gas

Yin Chen et al.

Summary: A new V-W/Ti SCR catalyst modified by Cu, Fe and Co was prepared for the simultaneous removal of NO and VOCs from coal-fired power plant flue gas. The experimental results showed that the catalyst had good denitration performance at low temperatures and high removal rates for benzene and toluene.

FUEL (2021)

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Article Chemistry, Physical

Selectively recombining the photoinduced charges in bandgap-broken Ag3PO4/GdCrO3 with a plasmonic Ag bridge for efficient photothermocatalytic VOCs degradation and CO2 reduction

Jingwei Li et al.

Summary: This study proposes a strategy to activate a bandgap-broken heterojunction, using plasmonic metal Ag nanoparticles as a bridge, successfully constructing a robust photothermocatalyst. This catalyst exhibits full visible light response, efficient carrier separation, and high redox potentials, leading to a significantly higher photothermocatalytic degradation rate than other heterojunctions.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Chemistry, Physical

Synergistic effect of Pt/Ce and USY zeolite in Pt-based catalysts with high activity for VOCs degradation

Yijun Shi et al.

Summary: Pt/Ce-USY catalysts show superior activity for DCE degradation compared to Pt/USY catalysts, owing to the synergistic effect between abundant acid sites and strong oxidizing sites. For non-chlorinated VOCs degradation, both Pt/USY-r and Pt/Ce-USY-r catalysts exhibit good low-temperature activity, with low T-90 values for benzene, ethyl acetate, and n-hexane degradation, attributed to the active Pt species dispersed on the surface of USY zeolite. The loading of Pt promotes the deep oxidation of CH3Cl and C2H3Cl intermediates to CO2 and inhibits carbon deposition, increasing the durability of the catalyst for VOCs degradation, mainly due to the strong Pt-CeO2 interaction.

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Enhanced hydrophobic UiO-66 (University of Oslo 66) metal-organic framework with high capacity and selectivity for toluene capture from high humid air

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