4.7 Article

Improved visible light photocatalytic degradation of yttrium doped NiMgAl layered triple hydroxides for the effective removal of methylene blue dye

期刊

CHEMOSPHERE
卷 290, 期 -, 页码 -

出版社

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.chemosphere.2021.133299

关键词

Handling Editor; Derek Muir; Layered triple hydroxide; Methylene blue; Photocatalytic degradation; Visible light absorption; Yttrium doped NiMgAl

资金

  1. National Research Foundation of Korea (NRF) [2020K2A9A1A06103609, 2019H1D3A1A01071209, 2020R1A6A3A01099737, 2021R1C1C2010726, 2021R1I1A1A01060380]
  2. Korea Basic Science Institute (National research Facilities and Equipment Center) - Ministry of Education [2019R1A6C1010042, 2021R1A6C103A427]
  3. National Research Foundation of Korea [2020K2A9A1A06103609, 2020R1A6A3A01099737, 2021R1I1A1A01060380, 2021R1C1C2010726] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)

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The fabrication of layered triple hydroxides (LTH) doped with different weight percentages of yttrium (Y) was investigated using hydrothermal method, with the 1 wt.% Y-doped LTH showing the highest photocatalytic degradation efficiency for methylene blue dye under visible light irradiation. The optimized LTH exhibited improved photocatalytic performance due to enhanced visible light absorption, reduced transmission, and improved electron-hole separation.
Fabrication of layered triple hydroxides (LTH) is a typical and remarkable approach to produce new functionalities passionately investigated for photocatalytic removal of organic pollutants from industrial wastewater. The hydrothermal method was used to prepare different weight percentages of yttrium (Y) doped NiMgAl LTH. The structural, functional, optical, and morphological properties of the prepared samples were investigated using Xray diffraction, Fourier transformed-infrared spectroscopy, ultraviolet-visible diffuse reflectance spectroscopy, and scanning electron microscopy. The photocatalytic degradation of the different percentages of Y-doped LTH samples were assessed through the photocatalytic degradation of methylene blue dye under the visible light irradiation. When compared to other lower concentrations of Y doping, the photocatalytic degradation efficiency of 1 wt.% Y-doped LTH was higher. Thus, the optimized LTH's improved photocatalytic performance was attributed to increased visible light absorption with low transmission and improved electron-hole separation.

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