A highly reversible glass-fiber-based flexible lithium anode via embedding lithophilic cobalt quantum dots

Article Chemistry, Multidisciplinary

Regulating Interfacial Chemistry in Lithium-Ion Batteries by a Weakly Solvating Electrolyte**

Yu-Xing Yao et al.

Summary: The research reveals a weakly solvating electrolyte that improves the performance of Li-ion batteries by forming unique anion-derived interfaces, demonstrating fast-charging and long-term cycling characteristics.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Efforts towards Practical and Sustainable Li/Na-Air Batteries

Kai Chen et al.

Summary: The relationship between structure and performance of Li-O-2 batteries has been deeply elucidated in the past 20 years. Our research group focuses on optimizing cathode design and developing anode protection strategies to achieve large capacity, long life, and low charge overpotential.

CHINESE JOURNAL OF CHEMISTRY (2021)

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Review Chemistry, Multidisciplinary

Lithium-Air Batteries: Air-Electrochemistry and Anode Stabilization

Kai Chen et al.

Summary: The development of high energy-density, low-cost, and safe batteries is crucial for technological innovation and changing human lifestyle. Lithium-air batteries are promising candidates for next-generation batteries due to their high energy density. However, research on lithium-air batteries is still in its early stages, with challenges including electrolyte decomposition and anode corrosion.

ACCOUNTS OF CHEMICAL RESEARCH (2021)

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Article Chemistry, Multidisciplinary

Identifying the Critical Anion-Cation Coordination to Regulate the Electric Double Layer for an Efficient Lithium-Metal Anode Interface

Rui Xu et al.

Summary: The electric double layer (EDL) chemistry at the electrode/electrolyte interface is found to predominantly control the competitive reduction reactions during SEI construction on Li metal anode. Introducing multi-valent cation additives has been validated as a promising strategy to enhance the performance of SEI, shedding new light on the targeted regulation of reactive alkali metal interfaces.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

High lithiophilic nitrogen-doped carbon nanotube arrays prepared by in-situ catalyze for lithium metal anode

Chenyang Zhao et al.

Summary: The article introduces a method to construct nitrogen-doped carbon nanotube arrays on stainless steel mesh as a lithium composite anode to inhibit lithium dendrite growth, effectively improving its cycling stability and safety. The composite anode maintained 98.9% stability over 300 cycles and constructed a full battery with LiFePO4 as the cathode, retaining 95.4% capacity after 100 cycles.

CHINESE CHEMICAL LETTERS (2021)

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Article Chemistry, Multidisciplinary

A Highly Reversible Lithium Metal Anode by Constructing Lithiophilic Bi-Nanosheets

Xiaoyu Liu et al.

Summary: In this study, a 3D lithiophilic skeleton modified with nanoscale Bi sheets (Ni@Bi Foam, NBF) was constructed to address the issues of lithium plating/stripping and volume expansion during cycling. The NBF showed outstanding cycling stability and high Coulombic efficiency, as well as high reversibility in symmetrical cells. Furthermore, the NBF@Li anode exhibited superior long-term cycling and rate performance, even in high areal loading conditions, showcasing its potential for use in high-performance metal batteries.

SMALL (2021)

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Article Chemistry, Applied

Ag-modified hydrogen titanate nanowire arrays for stable lithium metal anode in a carbonate-based electrolyte

Zhipeng Wen et al.

Summary: A novel Ag@HTO nanowire array was successfully synthesized for stable Li deposition/stripping in a commercial carbonate-based electrolyte, showing excellent performance when assembled with a commercial high voltage cathode material.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Editorial Material Chemistry, Physical

Three-dimensional fiber network reinforced polymer electrolyte for dendrite-free all-solid-state lithium metal batteries

Zheng Zhang et al.

ENERGY STORAGE MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Super-Assembled Hierarchical CoO Nanosheets-Cu Foam Composites as Multi-Level Hosts for High-Performance Lithium Metal Anodes

Runhao Zhang et al.

Summary: By growing lithiophilic CoO nanosheets on Cu foam, a multi-level structure in 3D framework is formed, achieving uniform lithium deposition and improving charge transfer rate and capacity retention of the electrode.

SMALL (2021)

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Article Chemistry, Physical

Atomic layer deposition assisted superassembly of ultrathin ZnO layer decorated hierarchical Cu foam for stable lithium metal anode

Runhao Zhang et al.

Summary: A three-dimensional framework composed of a surface-modified thin ZnO layer and multi-level Cu nanofibers was developed as an advanced Li metal anode host, enabling uniform deposition of Li, high Coulombic efficiency, and remarkable cycling stability. This structure provides a larger specific surface area to distribute the surface charge uniformly, adjust the current density, and ensure more uniform Li deposition, leading to dendrite-free Li deposition and improved plating/stripping behavior.

ENERGY STORAGE MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Functional Separators Regulating Ion Transport Enabled by Metal-Organic Frameworks for Dendrite-Free Lithium Metal Anodes

Zhendong Hao et al.

Summary: Regulating anion migration near lithium metal and promoting homogeneous lithium deposition are effective strategies to address the dendrites issue in lithium metal batteries. Developing a functional separator to manage ion transport can achieve a highly stable Li plating/stripping cycling and improve the discharge capacity and rate performance of LMBs.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Multidisciplinary Sciences

Atomic-scale regulation of anionic and cationic migration in alkali metal batteries

Pan Xiong et al.

Summary: Regulating the transport of anions and cations at the atomic scale is crucial in membrane-based separation technologies and the development of high-performance alkali metal batteries. The use of negatively charged Ti0.87O2 nanosheets coated polypropylene separators can reduce the non-uniform transport of alkali metal ions and detrimental shuttling effect of anions, ensuring homogeneous ion flux and promoting fast alkali-ion diffusion.

NATURE COMMUNICATIONS (2021)

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Article Chemistry, Applied

MOF-derived multifunctional filler reinforced polymer electrolyte for solid-state lithium batteries

Zheng Zhang et al.

Summary: A new multifunctional filler was proposed to reinforce polymer electrolytes, resulting in composite solid electrolytes (CSEs) with high ionic conductivity and stability. The electrolyte exhibited excellent interfacial stability in Li symmetrical batteries, and the solid-state lithium batteries showed superior cycle stability and capacity retention after multiple cycles. This work presents a novel strategy for building high-performance SSLBs.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Wax-Transferred Hydrophobic CVD Graphene Enables Water-Resistant and Dendrite-Free Lithium Anode toward Long Cycle Li-Air Battery

Yong Ma et al.

Summary: A tactic for water-resistant Li anode by implementing a wax-assisted transfer protocol is reported, using a high-quality CVD graphene layer to passivate the Li surface. The graphene coating serves as an artificial SEI, guiding homogeneous Li plating/stripping and protecting the Li surface from moisture erosion. The passivated Li anodes demonstrate superb cycling performance in lithium-air batteries, showing excellent air and electrochemical stability.

ADVANCED SCIENCE (2021)

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Article Chemistry, Physical

A Lithium-Metal Anode with Ultra-High Areal Capacity (50 mAh cm-2) by Gridding Lithium Plating/Stripping

Pan Xu et al.

Summary: By using a functionalized framework and a phosphorized copper mesh as a support skeleton, a lithium anode with excellent performance and practical application significance has been achieved, addressing the issues encountered during Li plating/stripping process in lithium metal batteries.

ENERGY STORAGE MATERIALS (2021)

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Article Chemistry, Physical

A highly reversible sodium metal anode by mitigating electrodeposition overpotential

Pan Xu et al.

Summary: Phosphorizing treatment was used to create a sodiophilic phosphorized copper mesh as a current collector for metallic sodium hosting, resulting in improved electrodeposition efficiency and behavior for sodium plating/stripping.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Multidisciplinary

Regulated lithium plating and stripping by a nano-scale gradient inorganic-organic coating for stable lithium metal anodes

Yipeng Sun et al.

Summary: The innovative nano-scale protective film design for lithium metal anodes (LMAs) utilizing mechanically enhanced hybrid inorganic-organic polyurea through gradient coating achieved by molecular layer deposition (MLD) is able to stabilize the lithium metal anodes. This design can confine the electro-deposition of lithium and tolerate volume changes, while also effectively facilitating and regulating uniform lithium nucleation and deposition.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

An artificial hybrid interphase for an ultrahigh-rate and practical lithium metal anode

Anjun Hu et al.

Summary: An artificial hybrid SEI layer composed of lithium-antimony alloy and lithium fluoride was constructed to reduce electron tunneling between the Li anode and SEI, resulting in uniform Li deposition and stable Li plating/stripping behaviors at an ultrahigh rate. This work uncovers the internal mechanism of Li+ transport within the SEI component, providing a pathway to stabilize the Li anode under practical high-rate conditions.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Ag coated 3D-Cu foam as a lithiophilic current collector for enabling Li2S-based anode-free batteries

Hao Cheng et al.

Summary: The key to practical lithium-metal batteries lies in stabilizing lithium deposition and reducing excess lithium. By constructing an anode-free full battery with Ag@3D-Cu as the current collector and Li2S-based electrode, the goal of regulating lithium deposition and avoiding excess lithium has been achieved.

CHEMICAL COMMUNICATIONS (2021)

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Article Chemistry, Multidisciplinary

An oxygen-blocking oriented multifunctional solid-electrolyte interphase as a protective layer for a lithium metal anode in lithium-oxygen batteries

Xiao-Dong Lin et al.

Summary: This study combines electrochemical polishing technology with LiNO3 reduction chemistry to construct a stable and molecularly smooth SEI on the Li metal surface, with a unique multi-layered structure encapsulating soluble NO2- species. This SEI film not only prevents negative effects from NO2- dissolution, but also effectively suppresses dendrite growth and O-2 permeation on the Li surface, substantially improving the cycle lives of O-2-saturated symmetric Li cells and Li-O-2 batteries. The work provides an effective strategy to protect Li metal anodes and offers novel insights into rational electrolyte additive utilization.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Multidisciplinary Sciences

A highly stable lithium metal anode enabled by Ag nanoparticle-embedded nitrogen-doped carbon macroporous fibers

Yongjin Fang et al.

Summary: In this study, a three-dimensional hybrid host was developed to inhibit dendritic lithium formation in lithium batteries, resulting in a more stable lithium plating/stripping behavior. When coupled with a commercial cathode, the assembled full cell showed high rate capability and stable cycling life.

SCIENCE ADVANCES (2021)

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Review Chemistry, Multidisciplinary

A Route Toward Smart System Integration: From Fiber Design to Device Construction

Wei Weng et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Physical

In Situ Conversion of Cu3P Nanowires to Mixed Ion/Electron-Conducting Skeleton for Homogeneous Lithium Deposition

Changzhi Sun et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Regulating Uniform Li Plating/Stripping via Dual-Conductive Metal-Organic Frameworks for High-Rate Lithium Metal Batteries

Tian-Shi Wang et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Regulating Lithium Nucleation and Deposition via MOF-Derived Co@C-Modified Carbon Cloth for Stable Li Metal Anode

Ting Zhou et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Copper Nitride Nanowires Printed Li with Stable Cycling for Li Metal Batteries in Carbonate Electrolytes

Dongsoo Lee et al.

ADVANCED MATERIALS (2020)

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Article Engineering, Environmental

Enhancing Li-S redox kinetics by fabrication of a three dimensional Co/CoP@nitrogen-doped carbon electrocatalyst

Yijuan Li et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Article Nanoscience & Nanotechnology

Stable Lithium Metal Anode Enabled by 3D Soft Host

Hua Wang et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Multidisciplinary

A Mixed Lithium-Ion Conductive Li2S/Li2Se Protection Layer for Stable Lithium Metal Anode

Fanfan Liu et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

A Two-Dimensional Mesoporous Polypyrrole-Graphene Oxide Heterostructure as a Dual-Functional Ion Redistributor for Dendrite-Free Lithium Metal Anodes

Haodong Shi et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Lithiophilic Zn Sites in Porous CuZn Alloy Induced Uniform Li Nucleation and Dendrite-free Li Metal Deposition

Shang-Sen Chi et al.

NANO LETTERS (2020)

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Article Chemistry, Multidisciplinary

3D Flexible, Conductive, and Recyclable Ti3C2Tx MXene-Melamine Foam for High-Areal-Capacity and Long-Lifetime Alkali-Metal Anode

Haodong Shi et al.

ACS NANO (2020)

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Article Chemistry, Multidisciplinary

A Soft Lithiophilic Graphene Aerogel for Stable Lithium Metal Anode

Tianyu Yang et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

In Situ Designing a Gradient Li+ Capture and Quasi-Spontaneous Diffusion Anode Protection Layer toward Long-Life Li-O2 Batteries

Yue Yu et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

The Stabilization Effect of CO2in Lithium-Oxygen/CO2Batteries

Kai Chen et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Electrochemistry

An efficient Co-NC composite additive for enhancing interface performance of carbon-based perovskite solar cells

Cong Geng et al.

ELECTROCHIMICA ACTA (2020)

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Article Chemistry, Physical

Dendrite-free lithium metal anode with lithiophilic interphase from hierarchical frameworks by tuned nucleation

Zheng Luo et al.

ENERGY STORAGE MATERIALS (2020)

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Article Chemistry, Physical

High reversible Li plating and stripping by in-situ construction a multifunctional lithium-pinned array

Pan Xu et al.

ENERGY STORAGE MATERIALS (2020)

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Article Engineering, Chemical

In situ constructing lithiophilic NiFx nanosheets on Ni foam current collector for stable lithium metal anode via a succinct fluorination strategy

Gaoxu Huang et al.

CHEMICAL ENGINEERING JOURNAL (2020)

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Article Chemistry, Multidisciplinary

Electrode Protection in High-Efficiency Li-O2 Batteries

Gang Huang et al.

ACS CENTRAL SCIENCE (2020)

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Article Chemistry, Physical

CuO-C modified glass fiber films with a mixed ion and electron-conducting scaffold for highly stable lithium metal anodes

Xiaojie Shen et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Article Chemistry, Multidisciplinary

Beyond the concentrated electrolyte: further depleting solvent molecules within a Li+ solvation sheath to stabilize high-energy-density lithium metal batteries

Zhi Chang et al.

ENERGY & ENVIRONMENTAL SCIENCE (2020)

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Article Chemistry, Physical

3D lithiophilic-lithiophobic-lithiophilic dual-gradient porous skeleton for highly stable lithium metal anode

Hongfei Zheng et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Article Chemistry, Physical

Inducing ordered Li deposition on a PANI-decorated Cu mesh for an advanced Li anode

Xin-Yu Hu et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Article Chemistry, Multidisciplinary

MOF-derived lithiophilic CuO nanorod arrays for stable lithium metal anodes

Lei Wei et al.

NANOSCALE (2020)

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Article Chemistry, Physical

Cu coated soft fabric as anode for lithium metal batteries

Luhan Ye et al.

ENERGY STORAGE MATERIALS (2020)

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Review Materials Science, Multidisciplinary

Recent Advances in Electrode Fabrication for Flexible Energy-Storage Devices

Yukun Wang et al.

ADVANCED MATERIALS TECHNOLOGIES (2019)

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Article Chemistry, Multidisciplinary

A Lightweight 3D Cu Nanowire Network with Phosphidation Gradient as Current Collector for High-Density Nucleation and Stable Deposition of Lithium

Chen Zhang et al.

ADVANCED MATERIALS (2019)

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Article Electrochemistry

A highly stable glass fiber host for lithium metal anode behaving enhanced coulombic efficiency

Xiaojie Shen et al.

ELECTROCHIMICA ACTA (2019)

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Article Chemistry, Multidisciplinary

Prevention of dendrite growth and volume expansion to give high-performance aprotic bimetallic Li-Na alloy-O-2 batteries

Jin-ling Ma et al.

NATURE CHEMISTRY (2019)

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Article Chemistry, Physical

MOF-derived porous Co3O4-NC nanoflake arrays on carbon fiber cloth as stable hosts for dendrite-free Li metal anodes

Guangyu Jiang et al.

ENERGY STORAGE MATERIALS (2019)

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Article Energy & Fuels

Stress-driven lithium dendrite growth mechanism and dendrite mitigation by electroplating on soft substrates

Xu Wang et al.

NATURE ENERGY (2018)

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Article Chemistry, Multidisciplinary

A Versatile Strategy to Fabricate 3D Conductive Frameworks for Lithium Metal Anodes

Li-Ya Qi et al.

ADVANCED MATERIALS INTERFACES (2018)

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Review Nanoscience & Nanotechnology

Reviving the lithium metal anode for high-energy batteries

Dingchang Lin et al.

NATURE NANOTECHNOLOGY (2017)

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Article Chemistry, Physical

Stabilizing Li/electrolyte interface with a transplantable protective layer based on nanoscale LiF domains

Zhe Peng et al.

NANO ENERGY (2017)

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Review Chemistry, Multidisciplinary

Toward Safe Lithium Metal Anode in Rechargeable Batteries: A Review

Xin-Bing Cheng et al.

CHEMICAL REVIEWS (2017)

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Article Chemistry, Multidisciplinary

A novel synergistic composite with multi-functional effects for high-performance Li-S batteries

Yi-Juan Li et al.

ENERGY & ENVIRONMENTAL SCIENCE (2016)

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Article Multidisciplinary Sciences

Lithium-coated polymeric matrix as a minimum volume-change and dendrite-free lithium metal anode

Yayuan Liu et al.

NATURE COMMUNICATIONS (2016)

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Review Chemistry, Physical

Li-O2 and Li-S batteries with high energy storage

Peter G. Bruce et al.

NATURE MATERIALS (2012)

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A highly reversible glass-fiber-based flexible lithium anode via embedding lithophilic cobalt quantum dots

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