Catalytic hydrogenation of aromatic ring over ruthenium nanoparticles supported on α-Al2O3 at room temperature

Article Multidisciplinary Sciences

Selective hydrogenolysis of catechyl lignin into propenylcatechol over an atomically dispersed ruthenium catalyst

Shuizhong Wang et al.

Summary: An atomically dispersed Ru catalyst has been developed for efficient cleavage of C-O bonds in C-lignin without hydrogenation of C=C bonds, resulting in high yields of propenylcatechol with high TONs.

NATURE COMMUNICATIONS (2021)

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Article Chemistry, Physical

One-step efficient non-hydrogen conversion of cellulose into γ-valerolactone over AgPW/CoNi@NG composite

Shanhui Zhu et al.

Summary: The efficient conversion of cellulose into value-added GVL is achieved by CoNi nanoparticles encapsulated in N-doped thin graphene shell combined with Ag+-exchanged heteropolyacid, achieving a high yield of 55.9%. The composite catalyst demonstrates high resistance to the corrosion of LA and FA, showing excellent catalytic stability. LA-adsorption FTIR spectra and DFT calculations suggest that FA can rapidly reduce LA due to its low dissociation energy barrier and high dissociation rate.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Chemistry, Physical

Catalytic waste Kraft lignin hydrodeoxygenation to liquid fuels over a hollow Ni-Fe catalyst

Xiaomeng Dou et al.

Summary: The depolymerization and demethoxylation of Kraft lignin (KL) was achieved using a novel H-NiFe2O4 catalyst under mild conditions, with high liquid product yield and minimal coke yield. The catalytic performance of H-NiFe2O4 benefits from the synergy of Ni and Fe, promoting lignin depolymerization while suppressing condensation reactions. Plausible reaction pathways of KL depolymerization over H-NiFe2O4 are discussed, demonstrating the potential of this catalytic system for efficient conversion of KL into liquid fuels.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Review Chemistry, Physical

Recent Advances of Catalysis in the Hydrogenation and Dehydrogenation of N-Heterocycles for Hydrogen Storage

Khai Chen Tan et al.

Summary: The lack of efficient hydrogen storage methods is a technical barrier in implementing hydrogen energy. Liquid organic hydrogen carriers, particularly N-heterocycles, show promise for both on-board and off-board hydrogen storage, but face kinetic barriers that require efficient catalysts for improvement.

JOURNAL OF PHYSICAL CHEMISTRY C (2021)

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Article Multidisciplinary Sciences

Sustainable production of benzene from lignin

Qinglei Meng et al.

Summary: Efficient production of benzene from lignin is of great importance but has not been realized. In this study, a strategy is developed to transform lignin into benzene over RuW/zeolite catalyst in water, with a high yield of 18.8% on lignin weight basis. This high-performance protocol paves the way for efficiently producing benzene using lignin as the feedstock.

NATURE COMMUNICATIONS (2021)

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Article Chemistry, Multidisciplinary

Techno-economic analysis and life cycle assessment of a biorefinery utilizing reductive catalytic fractionation

Andrew W. Bartling et al.

Summary: Reductive catalytic fractionation (RCF) is a promising method to fractionate lignocellulose and convert lignin to a narrow product slate. Analyses of techno-economic, life cycle assessment, and air emissions are crucial for guiding research towards commercialization, with a focus on cost and sustainability considerations.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Review Chemistry, Multidisciplinary

Guidelines for performing lignin-first biorefining

Mahdi M. Abu-Omar et al.

Summary: The valorisation of lignin is crucial for the economic viability of the lignocellulosic biorefining industry. The lignin-first biorefining approach, which considers lignin valorisation in the design phase, has been shown to make the fullest use of lignocellulose. Despite the diverse approaches to reporting and analyzing results from lignin-first methods, we propose guidelines for analyzing critical data in order to facilitate direct comparisons between studies.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Chemistry, Physical

Mechanistic Understanding of the Heterogeneous, Rhodium-Cyclic (Alkyl)(Amino)Carbene-Catalyzed (Fluoro-)Arene Hydrogenation

Daniel Moock et al.

ACS CATALYSIS (2020)

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Article Chemistry, Physical

From Lignin to Chemicals: Hydrogenation of Lignin Models and Mechanistic Insights into Hydrodeoxygenation via Low-Temperature C-O Bond Cleavage

Charles E. J. J. Vriamont et al.

ACS CATALYSIS (2019)

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Article Chemistry, Multidisciplinary

Microenvironment Engineering of Ruthenium Nanoparticles Incorporated into Silica Nanoreactors for Enhanced Hydrogenations

Xiaomin Ren et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Applied

Selective cleavage of C-O bond in benzyl phenyl ether over Pd/AC at room temperature

Tao Xie et al.

FUEL PROCESSING TECHNOLOGY (2019)

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Article Chemistry, Physical

Thermostable Rh Metal Nanoparticles Formed on Al2O3 by High-Temperature H2 Reduction and Its Impact on Three-Way Catalysis

Masato Machida et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2019)

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Article Chemistry, Applied

Bimetallic effects in the catalytic hydrogenolysis of lignin and its model compounds on Nickel-Ruthenium catalysts

Chen Zhu et al.

FUEL PROCESSING TECHNOLOGY (2019)

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Article Chemistry, Multidisciplinary

Engineering Energy Level of Metal Center: Ru Single-Atom Site for Efficient and Durable Oxygen Reduction Catalysis

Meiling Xiao et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Physical

C-O cleavage of diphenyl ether followed by C-C coupling reactions over hydrophobized Pd/HY catalysts

Cristiane A. Scaldaferri et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2019)

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Article Chemistry, Physical

Metal-Organic Framework Nodes Support Single-Site Nickel(II) Hydride Catalysts for the Hydrogenolysis of Aryl Ethers

Yang Song et al.

ACS CATALYSIS (2019)

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Article Energy & Fuels

Mechanism of Ni-catalyzed selective C-O cleavage of lignin model compound benzyl phenyl ether under mild conditions

Chen Zhu et al.

JOURNAL OF THE ENERGY INSTITUTE (2019)

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Article Chemistry, Multidisciplinary

Selective hydrodeoxygenation of lignin oil to valuable phenolics over Au/Nb2O5 in water

Lin Dong et al.

GREEN CHEMISTRY (2019)

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Article Chemistry, Multidisciplinary

Ru/hydroxyapatite as a dual-functional catalyst for efficient transfer hydrogenolytic cleavage of aromatic ether bonds without additional bases

Manti Hua et al.

GREEN CHEMISTRY (2019)

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Article Chemistry, Multidisciplinary

Selective cleavage of lignin and lignin model compounds without external hydrogen, catalyzed by heterogeneous nickel catalysts

Liang Jiang et al.

CHEMICAL SCIENCE (2019)

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Review Chemistry, Multidisciplinary

Metal Catalysts for Heterogeneous Catalysis: From Single Atoms to Nanoclusters and Nanoparticles

Lichen Liu et al.

CHEMICAL REVIEWS (2018)

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Article Chemistry, Physical

Rhodium(0) nanoparticles supported on ceria as catalysts in hydrogenation of neat benzene at room temperature

Serdar Akbayrak

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2018)

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Article Chemistry, Multidisciplinary

Multicomponent Pt-Based Zigzag Nanowires as Selectivity Controllers for Selective Hydrogenation Reactions

Shuxing Bai et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2018)

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Article Chemistry, Multidisciplinary

Efficient and Mild Transfer Hydrogenolytic Cleavage of Aromatic Ether Bonds in Lignin-Derived Compounds over Ru/C

Haoran Wu et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2018)

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Article Chemistry, Multidisciplinary

Catalytic Transfer Hydrogenolysis of Lignin-Derived Aromatic Ethers Promoted by Bimetallic Pd/Ni Systems

Francesco Mauriello et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2018)

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Article Chemistry, Multidisciplinary

Polysilane-Immobilized Rh-Pt Bimetallic Nanoparticles as Powerful Arene Hydrogenation Catalysts: Synthesis, Reactions under Batch and Flow Conditions and Reaction Mechanism

Hiroyuki Miyamura et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2018)

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Article Chemistry, Physical

Rh(CAAC)-Catalyzed Arene Hydrogenation: Evidence for Nanocatalysis and Sterically Controlled Site-Selective Hydrogenation

Ba L. Tran et al.

ACS CATALYSIS (2018)

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Article Chemistry, Physical

Remarkable Enhancement in Hydrogenation Ability by Phosphidation of Ruthenium: Specific Surface Structure Having Unique Ru Ensembles

Shinya Furukawa et al.

ACS CATALYSIS (2018)

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Article Multidisciplinary Sciences

Accelerating water dissociation kinetics by isolating cobalt atoms into ruthenium lattice

Junjie Mao et al.

NATURE COMMUNICATIONS (2018)

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Article Chemistry, Physical

Highly Active and Selective RuPd Bimetallic NPs for the Cleavage of the Diphenyl Ether C-O Bond

Miao Guo et al.

ACS CATALYSIS (2018)

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Review Chemistry, Physical

State-of-the-art catalytic hydrogenolysis of lignin for the production of aromatic chemicals

Chongbo Cheng et al.

CATALYSIS SCIENCE & TECHNOLOGY (2018)

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Article Chemistry, Multidisciplinary

Production of Jet Fuel-Range Hydrocarbons from Hydrodeoxygenation of Lignin over Super Lewis Acid Combined with Metal Catalysts

Hongliang Wang et al.

CHEMSUSCHEM (2018)

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Article Engineering, Chemical

Core/Shell Ruthenium Halloysite Nanocatalysts for Hydrogenation of Phenol

Vladimir Vinokurov et al.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2017)

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Article Chemistry, Physical

Enhancement of C-O bond cleavage to afford aromatics in the hydrodeoxygenation of anisole over ruthenium-supporting mesoporous metal oxides

Tuan Ngoc Phan et al.

APPLIED CATALYSIS A-GENERAL (2017)

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Article Chemistry, Multidisciplinary

Palladium-Catalyzed Hydrolytic Cleavage of Aromatic C-O Bonds

Meng Wang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2017)

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Article Chemistry, Multidisciplinary

Chemo- and Regioselective Hydrogenolysis of Diaryl Ether C-O Bonds by a Robust Heterogeneous Ni/C Catalyst: Applications to the Cleavage of Complex Lignin-Related Fragments

Fang Gao et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2016)

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Article Chemistry, Physical

MOF-Based Catalysts for Selective Hydrogenolysis of Carbon Oxygen Ether Bonds

Vitalie Stavila et al.

ACS CATALYSIS (2016)

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Article Chemistry, Multidisciplinary

Conversion of lignin model compounds under mild conditions in pseudo-homogeneous systems

Lu Chen et al.

GREEN CHEMISTRY (2016)

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Article Chemistry, Physical

Liquid phase selective hydrogenation of phenol to cyclohexanone over Ru/Al2O3 nanocatalyst under mild conditions

A. N. Raut et al.

KINETICS AND CATALYSIS (2016)

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Article Multidisciplinary Sciences

Highly selective hydrogenation of arenes using nanostructured ruthenium catalysts modified with a carbon-nitrogen matrix

Xinjiang Cui et al.

NATURE COMMUNICATIONS (2016)

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Article Chemistry, Physical

Selective Hydrodeoxygenation of Lignin-Derived Phenols to Cyclohexanols or Cyclohexanes over Magnetic CoNx@NC Catalysts under Mild Conditions

Xiaohao Liu et al.

ACS CATALYSIS (2016)

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Article Chemistry, Physical

Selective arene production from transfer hydrogenolysis of benzyl phenyl ether promoted by a co-precipitated Pd/Fe3O4 catalyst

E. Paone et al.

CATALYSIS SCIENCE & TECHNOLOGY (2016)

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Article Chemistry, Physical

Highly active electron-deficient Pd clusters on N-doped active carbon for aromatic ring hydrogenation

Renfeng Nie et al.

CATALYSIS SCIENCE & TECHNOLOGY (2016)

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Article Chemistry, Physical

High Efficient Hydrogenation of Lignin-Derived Monophenols to Cyclohexanols over Pd/γ-Al2O3 under Mild Conditions

Jian Yi et al.

CATALYSTS (2016)

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Review Chemistry, Multidisciplinary

Knocking on Wood: Base Metal Complexes as Catalysts for Selective Oxidation of Lignin Models and Extracts

Susan K. Hanson et al.

ACCOUNTS OF CHEMICAL RESEARCH (2015)

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Article Chemistry, Physical

Ruthenium Nanoparticles Stabilized in Cross-Linked Dendrimer Matrices: Hydrogenation of Phenols in Aqueous Media

Anton Maximov et al.

CHEMCATCHEM (2015)

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Review Chemistry, Multidisciplinary

Catalytic Transformation of Lignin for the Production of Chemicals and Fuels

Changzhi Li et al.

CHEMICAL REVIEWS (2015)

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Article Engineering, Chemical

Cleavage of Lignin-Derived 4-O-5 Aryl Ethers over Nickel Nanoparticles Supported on Niobic Acid-Activated Carbon Composites

Shaohua Jin et al.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2015)

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Article Chemistry, Physical

Mesoporous ZSM-5 Zeolite-Supported Ru Nanoparticles as Highly Efficient Catalysts for Upgrading Phenolic Biomolecules

Liang Wang et al.

ACS CATALYSIS (2015)

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Article Chemistry, Physical

Catalytic Hydrogenolysis of Aryl Ethers: A Key Step in Lignin Valorization to Valuable Chemicals

Muhammad Zaheer et al.

ACS CATALYSIS (2015)

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Article Chemistry, Physical

RuPd Alloy Nanoparticles Supported on N-Doped Carbon as an Efficient and Stable Catalyst for Benzoic Acid Hydrogenation

Minghui Tang et al.

ACS CATALYSIS (2015)

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Article Chemistry, Physical

Rhodium-mediated hydrogenolysis/hydrolysis of the aryl ether bond in supercritical carbon dioxide/water: an experimental and theoretical approach

Maya Chatterjee et al.

CATALYSIS SCIENCE & TECHNOLOGY (2015)

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Article Chemistry, Multidisciplinary

Regioselective and Stereospecific Deuteration of Bioactive Aza Compounds by the Use of Ruthenium Nanoparticles

Gregory Pieters et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2014)

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Article Chemistry, Multidisciplinary

Highly efficient, NiAu-catalyzed hydrogenolysis of lignin into phenolic chemicals

Jiaguang Zhang et al.

GREEN CHEMISTRY (2014)

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Article Chemistry, Physical

Understanding the surface chemistry of carbon nanotubes: Toward a rational design of Ru nanocatalysts

Bruno F. Machado et al.

JOURNAL OF CATALYSIS (2014)

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Article Chemistry, Multidisciplinary

One-Step Synthesis of Highly Efficient Nanocatalysts on the Supports with Hierarchical Pores Using Porous Ionic Liquid-Water Gel

Xinchen Kang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2014)

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Article Chemistry, Multidisciplinary

Titanium Nitride-Nickel Nanocomposite as Heterogeneous Catalyst for the Hydrogenolysis of Aryl Ethers

Valerio Molinari et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2014)

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Article Chemistry, Applied

Production of Lower Olefins with Highly Dispersed Ru Catalysts Supported on Al-SBA-15 in Fischer-Tropsch Synthesis

Sufang Chen et al.

TOPICS IN CATALYSIS (2014)

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Article Chemistry, Physical

Hydrogenation of Benzoic Acid and Derivatives over Pd Nanoparticles Supported on N-Doped Carbon Derived from Glucosamine Hydrochloride

Xuan Xu et al.

ACS CATALYSIS (2014)

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Article Electrochemistry

Application of the condensed Fukui function to predict reactivity in core-shell transition metal nanoparticles

Thomas C. Allison et al.

ELECTROCHIMICA ACTA (2013)

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Article Chemistry, Physical

Controlled synthesis of highly dispersed semi-embedded ruthenium nanoparticles in porous carbon framework with more exposed active sites

Ying Li et al.

CATALYSIS COMMUNICATIONS (2012)

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Article Chemistry, Multidisciplinary

Solvent Effects on the Hydrogenolysis of Diphenyl Ether with Raney Nickel and their Implications for the Conversion of Lignin

Xingyu Wang et al.

CHEMSUSCHEM (2012)

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Article Chemistry, Multidisciplinary

A Heterogeneous Nickel Catalyst for the Hydrogenolysis of Aryl Ethers without Arene Hydrogenation

Alexey G. Sergeev et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2012)

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Review Multidisciplinary Sciences

Valorization of Biomass: Deriving More Value from Waste

Christopher O. Tuck et al.

SCIENCE (2012)

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Article Chemistry, Multidisciplinary

Is It Homogeneous or Heterogeneous Catalysis Derived from [RhCp*Cl2]2? In Operando XAFS, Kinetic, and Crucial Kinetic Poisoning Evidence for Subnanometer Rh4 Cluster-Based Benzene Hydrogenation Catalysis

Ercan Bayram et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2011)

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Article Chemistry, Multidisciplinary

Highly Selective Hydrogenation of Phenol and Derivatives over a Pd@Carbon Nitride Catalyst in Aqueous Media

Yong Wang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2011)

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Article Chemistry, Multidisciplinary

TiO2-supported Rh nanoparticles: From green catalyst preparation to application in arene hydrogenation in neat water

Claudie Hubert et al.

GREEN CHEMISTRY (2010)

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Article Chemistry, Physical

Study of Catalytic Sites on Ruthenium For Hydrogenation of N-ethylcarbazole: Implications of Hydrogen Storage via Reversible Catalytic Hydrogenation

Katarzyna Morawa Eblagon et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2010)

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Article Chemistry, Applied

Selective oxidation of CO in excess H2 over Ru/Al2O3 catalysts modified with metal oxide

Xirong Chen et al.

JOURNAL OF NATURAL GAS CHEMISTRY (2007)

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Article Chemistry, Physical

Use of water as a solvent in directing hydrogenation reactions of aromatic acids over Pd/carbon nanofibre catalysts

James A. Anderson et al.

CATALYSIS LETTERS (2007)

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Article Chemistry, Multidisciplinary

Near-monodisperse tetrahedral rhodium nanoparticles on charcoal: The shape-dependent catalytic hydrogenation of arenes

Kang Hyun Park et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2007)

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Article Chemistry, Physical

Kinetics of steam reforming of methane on Ru/Al2O3 catalyst promoted with Mn oxides

A Berman et al.

APPLIED CATALYSIS A-GENERAL (2005)

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Article Chemistry, Physical

Preparation of Ru nanoparticles supported on γ-Al2O3 and its novel catalytic activity for ammonia synthesis

A Miyazaki et al.

JOURNAL OF CATALYSIS (2001)

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Review Chemistry, Physical

Kinetics of liquid-phase hydrogenation reactions over supported metal catalysts - a review

UK Singh et al.

APPLIED CATALYSIS A-GENERAL (2001)

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Catalytic hydrogenation of aromatic ring over ruthenium nanoparticles supported on α-Al2O3 at room temperature

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