期刊
ADVANCED MATERIALS
卷 34, 期 29, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.202201547
关键词
carbon capture and utilization; CO; (2) management; dual-functional materials; energy sustainability; smart materials
类别
资金
- Natural Sciences and Engineering Research Council of Canada (NSERC)
- Mathematics of Information Technology and Complex Systems (Mitacs)
- University of Waterloo
- Waterloo Institute for Nanotechnology
This article reviews the latest progress in sustainable CO2 management materials, including capture, catalytic conversion, and direct utilization. The article offers insights that span multiple scopes of material research and summarizes the major difficulties and future potential for implementing advanced materials and technologies.
With the rising level of atmospheric CO2 worsening climate change, a promising global movement toward carbon neutrality is forming. Sustainable CO2 management based on carbon capture and utilization (CCU) has garnered considerable interest due to its critical role in resolving emission-control and energy-supply challenges. Here, a comprehensive review is presented that summarizes the state-of-the-art progress in developing promising materials for sustainable CO2 management in terms of not only capture, catalytic conversion (thermochemistry, electrochemistry, photochemistry, and possible combinations), and direct utilization, but also emerging integrated capture and in situ conversion as well as artificial-intelligence-driven smart material study. In particular, insights that span multiple scopes of material research are offered, ranging from mechanistic comprehension of reactions, rational design and precise manipulation of key materials (e.g., carbon nanomaterials, metal-organic frameworks, covalent organic frameworks, zeolites, ionic liquids), to industrial implementation. This review concludes with a summary and new perspectives, especially from multiple aspects of society, which summarizes major difficulties and future potential for implementing advanced materials and technologies in sustainable CO2 management. This work may serve as a guideline and road map for developing CCU material systems, benefiting both scientists and engineers working in this growing and potentially game-changing area.
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