4.8 Review

Ionogel-Based Membranes for Safe Lithium/Sodium Batteries

期刊

ADVANCED MATERIALS
卷 34, 期 52, 页码 -

出版社

WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.202200945

关键词

electrochemical stability; ionogels; lithium; sodium batteries; safety; solid-state electrolytes

资金

  1. National Natural Science Foundation of China [51972132, 52002141]
  2. Program for HUST Academic Frontier Youth Team [2016QYTD04]

向作者/读者索取更多资源

This review discusses the recent advances in ionogel electrolytes for safe lithium/sodium batteries, including their structure, properties, and applications. Ionogel electrolytes, composed of ionic liquids and solid matrices, offer advantages such as nonvolatility and nonflammability.
Alkali (lithium, sodium)-based second batteries are considered one of the brightest candidates for energy-storage applications in order to utilize the random and intermittent renewable energy to achieve carbon neutrality. Conventional lithium/sodium batteries containing liquid organic electrolytes are vulnerable to electrolytes leakage and even combustion, which hinders their large-scale and reliable application. All-solid-state electrolytes which are considered to have better safety have been developed in recent years. However, most of them suffer from low ionic conductivity and large interfacial resistance with the electrode. Ionogel-electrolyte membranes composed of ionic liquids and solid matrices, have attracted much attention because of their nonvolatility, nonflammability, and superior chemical and electrochemical properties. This review focuses on the most recent advances of ionogel electrolytes that sprang up with the emerging demand and progress of safe lithium/sodium batteries. The ionogel-electrolyte membranes are discussed based on the framework components and preparation methods. Their structure and properties, including ionic conductivity, mechanical strength, electrochemical stabilities, and so on, are demonstrated in combination with their applications. The current challenges and insights on the future development of ionogel electrolytes for advanced safe lithium/sodium batteries are also proposed.

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