期刊
ADVANCED MATERIALS
卷 34, 期 52, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.202200662
关键词
electrolytes; molecular design; multivalent metal-ion batteries; organic electrodes; storage mechanism
类别
资金
- National Natural Science Foundation of China [52173163]
- National 1000-Talents Program
- Hubei Provincial Natural Science Foundation of China [2019CFA002]
- China Postdoctoral Science Foundation [2021TQ0115, 2021M701302, 2020M672323]
- Innovation Fund of WNLO
This paper analyzes the challenges faced by organic multivalent metal-ion batteries (MMIBs) and discusses possible strategies to overcome them. The charge-storage mechanism is particularly emphasized to enhance the understanding of structure-property relationships for the design of high-performance organic electrodes for MMIBs. The practical applications of organic MMIBs are also explored in this review.
Rechargeable organic multivalent metal-ion batteries (MMIBs) have attracted a surge of interest as promising alternatives for large-scale energy storage applications because they can combine the advantages of both organic electrodes and multivalent metal-ion batteries. However, the development of organic MMIBs is hampered by many factors, which mean they lag far behind organic alkali-metal- (e.g., Li-, Na-, and K-) ion batteries. Herein, the challenges that are specifically faced by organic MMIBs are analyzed and the strategies that can probably solve such challenges are then discussed. As a special challenge that organic MMIBs are facing, the charge-storage mechanism is particularly underlined to deeply understand the structure-property relationships for guiding the future design of high-performance organic electrodes for MMIBs. The perspectives are thereby elaborated in this review with the outlook of practical applications of organic MMIBs.
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