4.5 Article

Carbon nanotubes-reinforced preparation of flat MoS2 nanomaterials: Co-enhancement of acoustic exfoliation efficiency and dye removal capacity

期刊

FLATCHEM
卷 30, 期 -, 页码 -

出版社

ELSEVIER
DOI: 10.1016/j.flatc.2021.100312

关键词

2D materials; flat MoS2; Carbon nanotubes; Acoustic exfoliation; Dye removal

资金

  1. Natural Science Basic Research Project of Shaanxi Province [2021JZ-43]
  2. National Key Research and Development Program of China [2019YFC1520904]
  3. Key Program for International Science and Technology Cooperation Project of Shaanxi Province [2018KWZ-08]
  4. National Natural Science Foundation of China [61701402, 61804125, 61904148]
  5. Key Research and Development Program of Shaanxi Province [2018GY-025]

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A novel preparation technology was developed to efficiently produce ultrathin MoS2 crystals, with a 15-fold increase in dispersion concentration and significantly improved yield. The addition of MWCNT not only enhanced exfoliation efficiency but also indirectly strengthened the adsorption capacity for MG in wastewater. The adsorbent showed excellent removal capacity, stability, and reproducibility.
A novel and effective preparation technology was developed to prepare ultrathin molybdenum disulfide (MoS2) crystals with a high yield of the top-down exfoliation. Multidimensional carbon nanotubes (MWCNTs) were selected to be an assistant to enhance the effect of the traditional ultrasonic exfoliation efficiency. The rough and messy tubes strengthened the shear force in some parts during the acoustic treatment, which helped to weaken the van der Waals force between the MoS2 layers. Excitingly, this high-efficiency strategy can increase the dispersion concentration of nanosheets by 15 times compared to the traditional acoustic production, which represented the preparation yield was improved greatly. It is found that the addition of MWCNTs not only facilitated the exfoliation efficiency of bulk material but also indirectly improved the adsorption of malachite green (MG) in wastewater. With a maximum removal capacity of 87.80 mg g-1, the adsorption ability of the nanotubes-reinforced layered adsorbent was effectively strengthened. In addition, the performance of reproducibility, stability, functioning free radical types, and the adsorption models were systematically studied.

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