期刊
FRONTIERS IN CHEMISTRY
卷 9, 期 -, 页码 -出版社
FRONTIERS MEDIA SA
DOI: 10.3389/fchem.2021.781991
关键词
photocatalysis; heterostructures; visible light adsorption; charge carrier separation; tetracycline hydrochloride
资金
- National Natural Science Foundation of China (NSFC) [41975172, 20907021]
Bi5O7I/g-C3N4 p-n junctioned photocatalysts were synthesized by alcohol-heating and calcination in air, showing superior photocatalytic activity and stability. Compared with pure BiOI, Bi5O7I, and g-C3N4, the composite exhibited higher efficiency in the photodegradation of Rhodamine B and tetracycline hydrochloride.
Bi5O7I/g-C3N4 p-n junctioned photocatalysts were synthesized by alcohol-heating and calcination in air. The structures, morphologies and optical properties of as-prepared samples were characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM), transmission electron microscopy (TEM), UV-Vis diffuse reflectance spectroscopy (DRS). Photocatalytic activity of the heterojunctioned composites were evaluated by degradation of Rhodamine B (RhB) and tetracycline hydrochloride (TCH) under visible light illumination. The results indicated that the composites exhibited superior efficiencies for photodegradation of RhB and TCH in comparison with pure BiOI, Bi5O7I and g-C3N4. An effective built-in electric field was formed by the interface between p-type Bi5O7I and n-type g-C3N4, which promoted the efficient separation of photoinduced electron-hole pairs. In addition, 8% Bi5O7I/g-C3N4 composite showed excellent photostability in a five-cycle photocatalytic experiment. Experiments on scavenging active intermediates revealed the roles of active species.
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