期刊
MATERIALS RESEARCH LETTERS
卷 10, 期 4, 页码 264-270出版社
TAYLOR & FRANCIS INC
DOI: 10.1080/21663831.2022.2036839
关键词
High pressure; phase transition; alloyed CdS0.7Se0.3; warm-white light emission; color rendering index
资金
- National Key RAMP
- D Program of China [2019YFE0120300]
- National Science Foundation of China [12174144, 21725304, 22131006, 12174146, 11774125]
- China Postdoctoral Science Foundation [2021M690065]
Warm white light with enhanced CRI of 93 is achieved by pressure processing, accompanied by a color change. This high CRI warm WLED is of great significance for indoor lighting. The improvement of CRI in CdS0.7Se0.3 QDs was achieved by pressure engineering, accompanied by a phase transition.
IMPACT STATEMENT Warm white light with enhanced color rendering index of 93 is achieved by pressure processing, accompanied by a color change from 'natural' (4298 K) to 'warm' white light (2170 K). Warm WLED with high color rendering index (CRI) are greatly required for the widespread use of solid-state lighting especially indoors. Here, a remarkable improvement of CRI in alloyed CdS0.7Se0.3 QDs was achieved by pressure engineering. Notably, white light with enhanced CRI of 93, higher than pristine CRI of 47, was retained upon the complete release of pressure, accompanied by a color change from 'natural' (4298 K) to 'warm' white light (2170 K). Synchrotron ADXRD shows that CdS0.7Se0.3 QDs experienced an irreversible phase transition from the zinc blende phase to rocksalt structure.
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