4.6 Article

Advances of single-atom catalysts for applications in persulfate-based advanced oxidation technologies

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ELSEVIER SCI LTD
DOI: 10.1016/j.coche.2021.100757

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资金

  1. National Key Research and Development Program of China [2017YFA0207001]
  2. National Natural Science Foundation of China [42022049, 42130707]
  3. Youth Innovation Promotion Association, CAS [2014270]

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This review discusses the application of single-atom catalysts in persulfate activation, including synthesis and characterization strategies, new advances, development trends, and applications for degrading organic pollutants. The review also summarizes the advantages of single-atom catalysts in advanced oxidation processes and suggests future directions for development in the field.
Single-atom catalysts (SACs) have been attracted great attention because of their distinct physical structure and chemical properties, particularly in the field of catalysis. More recently, SACs have been extensively used in persulfate-based advanced oxidation processes (AOPs) for organic pollutant degradation. This review first briefly introduces the synthesis and characterization strategies of SACs, and analyses new progresses and the develop trend of SACs in persulfate activation. Then, a series of applications of SACs in persulfate activation for the degradation of organic pollutants are highlighted. Meanwhile, the strength of SACs in AOPs are summarized, and the opportunities and challenges encountered by SACs in the AOPs field and its future development direction are also proposed.

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