☆ 4.6 Review

Emerging materials for circularly polarized light detection

JOURNAL OF MATERIALS CHEMISTRY C (2022)

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Article Chemistry, Multidisciplinary

Spin-Dependent Photovoltaic and Photogalvanic Responses of Optoelectronic Devices Based on Chiral Two-Dimensional Hybrid Organic-Inorganic Perovskites

Jingying Wang et al.

Summary: Research has shown that integrating chiral organic ligands into two-dimensional hybrid organic-inorganic perovskites can introduce spintronics applications, leading to spin-dependent photovoltaic and photogalvanic responses. This discovery may have potential applications in optoelectronic devices sensitive to light helicity.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Fullerene Desymmetrization as a Means to Achieve Single-Enantiomer Electron Acceptors with Maximized Chiroptical Responsiveness

Wenda Shi et al.

Summary: Solubilized fullerene derivatives have revolutionized the development of organic photovoltaic devices by acting as excellent electron acceptors. Isomers with chirality, particularly single-enantiomer fullerenes, have been separated and utilized for designing fullerenes with large chiroptical responses in organic electronic devices. This study demonstrates the potential of chiral fullerenes in discriminating circularly polarized light with fast light response time and high photocurrent dissymmetry factor in organic electronic technologies.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Chiral Lead-Free Hybrid Perovskites for Self-Powered Circularly Polarized Light Detection

Dong Li et al.

Summary: Metal-halide perovskites have emerged as promising alternatives for CPL detection due to their CPL-sensitive property induced by chiral organics and efficient charge transport of inorganic frameworks. This study successfully developed lead-free halide double perovskites, demonstrating significant chirality and self-powered CPL detection capabilities. The research suggests that hybrid double perovskites can be promising photoelectronic candidates for exploring new green circularly polarized light-sensitive materials with high performance.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Physical

Origin of Chiroptic Amplification in Perylene-Diimide Helicenes

Daniel Aranda et al.

Summary: It has been shown that NP3H exhibits an enhancement of the electronic circular dichroism response in the visible range, attributed to the increase in the magnetic transition dipole moments of the involved electronic states, mainly due to the presence of the double [6]helicene substructure within NP3H. This phenomenon is suggested to arise from an exciton-like coupling, not present in the analogue NPDH. Further computations and analysis support this mechanism, indicating the potential for the double [6]helicene unit to be a key core in designing new chiral conjugated materials with enhanced chiroptical properties in the visible range.

JOURNAL OF PHYSICAL CHEMISTRY C (2021)

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Article Chemistry, Physical

Tuning Transition Electric and Magnetic Dipole Moments: [7]Helicenes Showing Intense Circularly Polarized Luminescence

Hiromu Kubo et al.

Summary: Substituting the [7]helicene framework can enhance the transition magnetic dipole moment (TMDM) for the S-1 -> S-0 transition, resulting in a higher fluorescence emission rate and improved optical properties in the derivative helicenes.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2021)

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Article Chemistry, Multidisciplinary

Chirality Amplified: Long, Discrete Helicene Nanoribbons

Xiao Xiao et al.

Summary: In this study, two polyhelicene frameworks were synthesized, with 18 and 24 fused benzene rings, respectively, exhibiting the largest electronic circular dichroism in the visible spectrum. These helical nanoribbons incorporate multiple helicenes, showing interesting chemical, biological, and chiroptical properties. Coupling with perylene-diimide subunits enhances chiroptic response, with the possibility of further enhancement by axial elongation.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Multidisciplinary Sciences

π-Extended perylene diimide double-heterohelicenes as ambipolar organic semiconductors for broadband circularly polarized light detection

Li Zhang et al.

Summary: In this study, a novel approach of skeleton merging was introduced to address the dilemma between strong coupling with circular polarized light and high charge-carrier mobility in high-performance chiral organic semiconducting molecules. The resulting pi-extended double helicene structure exhibits high dissymmetry factor, extended pi-planar system for charge transport properties, near-infrared light absorption, and ambipolar charge transport abilities, enabling high photoresponsivity and external quantum efficiency in both p- and n-type modes under NIR light irradiation. These characteristics allow for high-performance broadband CPL detections up to the NIR spectral region.

NATURE COMMUNICATIONS (2021)

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Review Chemistry, Multidisciplinary

Recent Progress in Organic Photodetectors and their Applications

Hao Ren et al.

Summary: Organic photodetectors have been attracting attention for their advantages like tunability, low cost, and compatibility with flexible devices. Recent research focuses on improving performance and applications, with future challenges and opportunities in the field.

ADVANCED SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Direct Detection of Circularly Polarized Light Using Chiral Copper Chloride-Carbon Nanotube Heterostructures

Ji Hao et al.

Summary: The study demonstrates high-performance circularly polarized light detectors by synthesizing 0D chiral copper chloride hybrids, showing superior optoelectronic properties. Results show that through the design of chiral heterostructures, high responsivity, competitive anisotropy factor, and low working voltage can be achieved for CPL detection.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Amplification of Dissymmetry Factors in π-Extended [7]- and [9]Helicenes

Zijie Qiu et al.

Summary: In this study, pi-Extended [7]helicene and pi-Extended [9]helicene were successfully synthesized with improved photophysical properties and high circularly polarized luminescence brightness. The research also revealed that a small variation in helical length can cause an increase in dissymmetry factors.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Chemistry, Multidisciplinary

Chiral 2D-Perovskite Nanowires for Stokes Photodetectors

Yingjie Zhao et al.

Summary: High-performance Stokes-parameter photodetectors are realized based on solution-processed chiral-perovskite nanowire arrays, which exhibit responsive circularly polarized light and large polarized ratio to linearly polarized light due to chiral ammonium cations and strictly aligned nanowires. The detectors demonstrate promising applications towards polarization imaging with their small footprint and high performance.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2021)

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Article Materials Science, Multidisciplinary

Strongly Circularly Polarized Crystalline and β-Phase Emission from Poly(9,9-dioctylfluorene)-Based Deep-Blue Light-Emitting Diodes

Li Wan et al.

Summary: This article presents highly efficient circularly polarized polymer light-emitting diodes (CP-PLEDs) for deep-blue emission by blending achiral luminescent polymer with helically chiral molecules. State-of-the-art device performance was achieved with different phase structures, showcasing high current efficiency and emission dissymmetry. The study provides insight into mechanisms underlying strong circularly polarized emission from excitonically coupled polymer chains in solid-state devices.

ADVANCED OPTICAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Great Amplification of Circular Polarization Sensitivity via Heterostructure Engineering of a Chiral Two-Dimensional Hybrid Perovskite Crystal with a Three-Dimensional MAPbI3 Crystal

Xinyuan Zhang et al.

Summary: The construction of a heterostructure crystal, integrating a chiral two-dimensional perovskite with its three-dimensional counterpart, significantly enhances circular polarization sensitivity for CPL detectors. This strategy allows for the creation of a CPL detector with a greatly amplified anisotropy factor, providing a novel approach to modulate circular polarization sensitivity in chiral hybrid perovskites for advanced chiroptical devices.

ACS CENTRAL SCIENCE (2021)

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Review Chemistry, Multidisciplinary

Pathways to increase the dissymmetry in the interaction of chiral light and chiral molecules

Jake L. Greenfield et al.

Summary: The dissymmetric interaction between circularly polarised light and chiral molecules is important across various fields, but the selectivity in absorption or emission of left-handed versus right-handed CP light is often low. Strategies to enhance this interaction include molecular design, modification of light, and creating macroscopic chiral structures, offering hope for advancements in research involving interactions of chiral molecules and light.

CHEMICAL SCIENCE (2021)

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Review Physics, Applied

Chiral spintronics

See-Hun Yang et al.

Summary: Spin currents generated by chiral structures can manipulate chiral topological magnetic excitations through chirality acquired in a spin-orbit interaction. When chiral domain walls form composite walls via antiferromagnetic exchange coupling, novel phenomena such as exchange coupling torque and domain wall drag are observed. This review discusses the recent progress in spin currents derived from or acting on chiral structures and their potential applications.

NATURE REVIEWS PHYSICS (2021)

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Article Chemistry, Multidisciplinary

A Chiral Reduced-Dimension Perovskite for an Efficient Flexible Circularly Polarized Light Photodetector

Lin Wang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Physics, Applied

Helical-chiroptical nanowires generated orbital angular momentum for the detection of circularly polarized light

Zhongxuan Wang et al.

APPLIED PHYSICS LETTERS (2020)

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Circular Polarization Discrimination Enhanced by Anisotropic Media

Zeshi Chu et al.

ADVANCED OPTICAL MATERIALS (2020)

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Perylene Diimide-Embedded Double [8]Helicenes

Bo Liu et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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The Structural Origins of Intense Circular Dichroism in a Waggling Helicene Nanoribbon

Nathaniel J. Schuster et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Highly Efficient Inverted Circularly Polarized Organic Light-Emitting Diodes

Li Wan et al.

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CHEMICAL REVIEWS (2020)

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Surface-Doped Quasi-2D Chiral Organic Single Crystals for Chiroptical Sensing

Xiaobo Shang et al.

ACS NANO (2020)

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Chiroptical Properties in Thin Films of π-Conjugated Systems

Gianluigi Albano et al.

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Supramolecular Nanostructures of Chiral Perylene Diimides with Amplified Chirality for High-Performance Chiroptical Sensing

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