A renewable biomass-based lignin film as an effective protective layer to stabilize zinc metal anodes for high-performance zinc-iodine batteries

Article Multidisciplinary Sciences

Integrated 'all-in-one' strategy to stabilize zinc anodes for high-performance zinc-ion batteries

Canpeng Li et al.

Summary: An 'all-in-one' (AIO) electrode was developed by combining structural design, interface modification, and electrolyte optimization, which can effectively improve the stability and performance of zinc-ion batteries.

NATIONAL SCIENCE REVIEW (2022)

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Article Chemistry, Multidisciplinary

Enhanced Redox Kinetics and Duration of Aqueous I2/I- Conversion Chemistry by MXene Confinement

Xinliang Li et al.

Summary: The study introduced a Nb2CTX host and achieved electro-oxidation of I- ions in MXene through electrodeposition strategy, thereby improving redox kinetics and duration. The aqueous Zn battery based on a Zn metal anode and ZnSO4 electrolyte showed outstanding performance, surpassing other aqueous MXenes and I-2-metal batteries.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Boosting Zinc Electrode Reversibility in Aqueous Electrolytes by Using Low-Cost Antisolvents

Junnan Hao et al.

Summary: A similar antisolvent strategy has been used to enhance Zn reversibility and suppress dendrite growth in Zn plating/stripping, with promising results shown in 50% methanol electrolyte. This low-cost strategy can be easily applied to other solvents, demonstrating practical universality and potential for enhancing performance in electrochemistry and energy storage research.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Review Chemistry, Physical

Strategies for the Stabilization of Zn Metal Anodes for Zn-Ion Batteries

Zhehan Yi et al.

Summary: Zinc-ion batteries are considered promising candidates for next-generation energy storage systems due to their high safety, resource availability, and environmental friendliness. However, the instability of the Zn metal anode has hindered their reliable deployment, and efforts have been made to overcome this through electrode structure design, interface modification, and electrolyte/separator optimization. Understanding and categorizing these strategies based on their intrinsic mechanisms are important for the development of novel Zn metal anodes for ZIBs.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

A hafnium oxide-coated dendrite-free zinc anode for rechargeable aqueous zinc-ion batteries

Bin Li et al.

Summary: In this study, a simple strategy involving application of a HfO2 coating was used to guide uniform deposition of Zn2+ to suppress formation of zinc dendrites, resulting in improved electrochemical performance of zinc anode. The HfO2-coated zinc anode demonstrated lower voltage hysteresis and better cycling performance in zinc-zinc symmetric cells and Zn-MnO2 full cells, showing potential for future development of rechargeable aqueous zinc-ion batteries.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Article Chemistry, Physical

Redistributing Zn-ion flux by interlayer ion channels in Mg-Al layered double hydroxide-based artificial solid electrolyte interface for ultra-stable and dendrite-free Zn metal anodes

Yang Yang et al.

Summary: Proposing an Mg-Al layered double hydroxide-based artificial solid electrolyte interface (SEI) with Zn-ion diffusion channels successfully addresses the long-standing issues of zinc-ion batteries, achieving stable Zn deposition and improved Coulombic efficiency. Additionally, zinc-ion capacitors paired with Zn@LDH anode and high-loading active carbon cathode demonstrate outstanding cycling stability at high current densities and can achieve an ultralong lifespan.

ENERGY STORAGE MATERIALS (2021)

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Article Chemistry, Physical

Eliminating Zn dendrites by commercial cyanoacrylate adhesive for zinc ion battery

Ziyi Cao et al.

Summary: By using a spin-coating method to uniformly coat Zn with a commercial cyanoacrylate adhesive, a stable artificial solid/electrolyte interphase is formed to protect the Zn surface and regulate Zn ion nucleation barriers, leading to improved cycling stability and high Coulombic efficiency.

ENERGY STORAGE MATERIALS (2021)

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Article Chemistry, Physical

An In Situ Artificial Cathode Electrolyte Interphase Strategy for Suppressing Cathode Dissolution in Aqueous Zinc Ion Batteries

Lishang Zhang et al.

Summary: The study proposes an in situ artificial cathode electrolyte interphase (CEI) strategy to kinetically suppress vanadium dissolution in aqueous zinc ion batteries. By introducing strontium ions as a sacrifice guest, a protective CEI coating layer is formed on the cathode surface, preventing vanadium from dissolving and improving the recharge capacity retention of the cathode. This work provides a general strategy for constructing the electrode-electrolyte interface to suppress vanadium-based cathodes dissolution in aqueous electrolytes.

SMALL METHODS (2021)

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Review Chemistry, Physical

Progress and prospect of the zinc-iodine battery

Yongqiang Yang et al.

Summary: The zinc-iodine battery has advantages in high energy density and low cost, but still faces challenges in practical applications. Key factors include selecting suitable materials as the cathode and electrolyte, controlling the energy storage reaction process, and inhibiting the self-transformation of by-products.

CURRENT OPINION IN ELECTROCHEMISTRY (2021)

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Review Chemistry, Multidisciplinary

Advances and Perspectives of Cathode Storage Chemistry in Aqueous Zinc-Ion Batteries

Xiao Wang et al.

Summary: This review discusses the key challenges of rechargeable aqueous zinc-ion batteries, analyzing the structural features and electrochemical properties of different cathode materials, and proposing various electrode design strategies to guide future research activities. The focus is mainly on achieving high energy density and durable cathode materials.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Engineering Polymer Glue towards 90% Zinc Utilization for 1000 Hours to Make High-Performance Zn-Ion Batteries

Yiding Jiao et al.

Summary: A new ion-selective polymer glue coated on the zinc anode allows for rapid zinc ion migration and uniform electrodeposition, resulting in a record-high zinc utilization of 90% for 1000 hours. When paired with a vanadium-based cathode, the zinc-ion battery exhibits an ultrahigh device-scale energy density of 228 Wh kg(-1), comparable to commercial lithium-ion batteries.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Physical

Dendrites-Free Zn Metal Anodes Enabled by an Artificial Protective Layer Filled with 2D Anionic Nanosheets

Ying Zhang et al.

Summary: The unique 2D Zn-Sb3P2O14 protective layer effectively addresses the issues of dendrite growth and side reactions of metallic zinc in aqueous batteries, enabling stable electron deposition and high Coulombic efficiency.

SMALL METHODS (2021)

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Article Chemistry, Multidisciplinary

Rational Design of Sulfur-Doped Three-Dimensional Ti3C2Tx MXene/ZnS Heterostructure as Multifunctional Protective Layer for Dendrite-Free Zinc-Ion Batteries

Yongling An et al.

Summary: By designing and constructing a protective heterogeneous layer composed of sulfur-doped three-dimensional (3D) MXene and ionic conductive ZnS on the zinc anode, the issues of dendrite growth and side reactions hindering the practical applications of zinc anode in aqueous batteries have been successfully addressed. This results in a stable and dendrite-free zinc anode with notable cycling stability and high-rate performance.

ACS NANO (2021)

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Article Chemistry, Physical

A liquid metal assisted dendrite-free anode for high-performance Zn-ion batteries

Hao Jia et al.

Summary: This study proposes a method using a liquid metal coating as a protective layer to prevent dendrite growth on the zinc metal anode surface. The liquid metal layer effectively inhibits dendrite formation, accelerates zinc nucleation speed and electron transfer, improves charge transfer efficiency, significantly reduces interfacial resistance, and extends the cycling life of zinc batteries.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Multidisciplinary

Activating the I0/I+ redox couple in an aqueous I2-Zn battery to achieve a high voltage plateau

Xinliang Li et al.

Summary: This study demonstrates the activation of reversible redox behavior in iodine conversion batteries through electrolyte adjustment, achieving significant performance enhancements.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

An Ultra-Long-Life Lithium-Rich Li1.2Mn0.6Ni0.2O2 Cathode by Three-in-One Surface Modification for Lithium-Ion Batteries

Xiaokai Ding et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Multidisciplinary Sciences

Lamella-nanostructured eutectic zinc-aluminum alloys as reversible and dendrite-free anodes for aqueous rechargeable batteries

Sheng-Bo Wang et al.

NATURE COMMUNICATIONS (2020)

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Article Chemistry, Multidisciplinary

Designing Dendrite-Free Zinc Anodes for Advanced Aqueous Zinc Batteries

Junnan Hao et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

An In-Depth Study of Zn Metal Surface Chemistry for Advanced Aqueous Zn-Ion Batteries

Junnan Hao et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Lignin Source and Structural Characterization

Run-Cang Sun

CHEMSUSCHEM (2020)

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Article Chemistry, Multidisciplinary

High-Voltage and Ultrastable Aqueous Zinc-Iodine Battery Enabled by N-Doped Carbon Materials: Revealing the Contributions of Nitrogen Configurations

Donglin Yu et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2020)

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Article Chemistry, Multidisciplinary

A Metal-Organic Framework as a Multifunctional Ionic Sieve Membrane for Long-Life Aqueous Zinc-Iodide Batteries

Huijun Yang et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Physical

Dendrite-free Zn anode with dual channel 3D porous frameworks for rechargeable Zn batteries

Wenbin Guo et al.

ENERGY STORAGE MATERIALS (2020)

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Article Chemistry, Physical

Highly stable Zn metal anodes enabled by atomic layer deposited Al2O3 coating for aqueous zinc-ion batteries

Huibing He et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Article Nanoscience & Nanotechnology

Novel Insights into Energy Storage Mechanism of Aqueous Rechargeable Zn/MnO2 Batteries with Participation of Mn2+

Yongfeng Huang et al.

NANO-MICRO LETTERS (2019)

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Article Nanoscience & Nanotechnology

Artificial Solid-Electrolyte Interface Facilitating Dendrite-Free Zinc Metal Anodes via Nanowetting Effect

Mingqiang Liu et al.

ACS APPLIED MATERIALS & INTERFACES (2019)

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Article Engineering, Environmental

Ultrafast adsorption of heavy metal ions onto functionalized lignin-based hybrid magnetic nanoparticles

Yongchao Zhang et al.

CHEMICAL ENGINEERING JOURNAL (2019)

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Article Chemistry, Multidisciplinary

Inside Cover: Synergistic N-Heterocyclic Carbene/Palladium-Catalyzed Umpolung 1,4-Addition of Aryl Iodides to Enals (Angew. Chem. Int. Ed. 1/2020)

Wenjun Yang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Multidisciplinary

Lignin@Nafion Membranes Forming Zn Solid-Electrolyte Interfaces Enhance the Cycle Life for Rechargeable Zinc-Ion Batteries

Du Yuan et al.

CHEMSUSCHEM (2019)

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Article Chemistry, Physical

Interweaving 3D Network Binder for High-Areal-Capacity Si Anode through Combined Hard and Soft Polymers

Tiefeng Liu et al.

ADVANCED ENERGY MATERIALS (2019)

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Review Chemistry, Multidisciplinary

Issues and opportunities facing aqueous zinc-ion batteries

Boya Tang et al.

ENERGY & ENVIRONMENTAL SCIENCE (2019)

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Article Chemistry, Multidisciplinary

Long-life and deeply rechargeable aqueous Zn anodes enabled by a multifunctional brightener-inspired interphase

Zhiming Zhao et al.

ENERGY & ENVIRONMENTAL SCIENCE (2019)

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Article Chemistry, Physical

A Metal-Organic Framework Host for Highly Reversible Dendrite-free Zinc Metal Anodes

Zhuo Wang et al.

JOULE (2019)

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Article Chemistry, Physical

Highly reversible zinc metal anode for aqueous batteries

Fei Wang et al.

NATURE MATERIALS (2018)

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Review Chemistry, Applied

Lignin in storage and renewable energy applications: A review

Jose Luis Espinoza-Acosta et al.

JOURNAL OF ENERGY CHEMISTRY (2018)

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Editorial Material Multidisciplinary Sciences

Aligning academia and industry for unified battery performance metrics

Zhan Lin et al.

NATURE COMMUNICATIONS (2018)

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Article Chemistry, Physical

Controlling the sustainability and shape change of the zinc anode in rechargeable aqueous Zn/LiMn2O4 battery

Wenlong Xiong et al.

ENERGY STORAGE MATERIALS (2018)

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Article Chemistry, Multidisciplinary

Effect of Heavy Metal (Zn) on Redox Property of Hydrochar Produced from Lignin, Cellulose, and D-Xylose

Dandan Mai et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2017)

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Review Multidisciplinary Sciences

Lignin Valorization: Improving Lignin Processing in the Biorefinery

Arthur J. Ragauskas et al.

SCIENCE (2014)

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Article Chemistry, Physical

A consistent and accurate ab initio parametrization of density functional dispersion correction (DFT-D) for the 94 elements H-Pu

Stefan Grimme et al.

JOURNAL OF CHEMICAL PHYSICS (2010)

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Article Computer Science, Interdisciplinary Applications

QUICKSTEP: Fast and accurate density functional calculations using a mixed Gaussian and plane waves approach

J VandeVondele et al.

COMPUTER PHYSICS COMMUNICATIONS (2005)

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A renewable biomass-based lignin film as an effective protective layer to stabilize zinc metal anodes for high-performance zinc-iodine batteries

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