期刊
JOURNAL OF ENERGY CHEMISTRY
卷 62, 期 -, 页码 204-219出版社
ELSEVIER
DOI: 10.1016/j.jechem.2021.03.020
关键词
Organic thermoelectric materials; Electronic structure; Organic semiconductors
资金
- National Key Research and Development Program of China [2017YFA0204700, 2018YFE0200700]
- National Natural Science Foundation of China [21805285]
- Key Research Program of Frontier Sciences of CAS [QYZDY-SSW-SLH024]
This review focuses on the regulation of electronic structures of organic materials for efficient thermoelectric conversion. Rational design and precise modulation of electronic structures have shown great potential in exploring state-of-the-art organic thermoelectric materials.
Electronic structures, which play a key role in determining electrical and optical properties of pi-conjugated organic materials, have attracted tremendous interest. Efficient thermoelectric (TE) conversion of organic materials has rigorous requirements on electronic structures. Recently, the rational design and precise modulation of electronic structures have exhibited great potential in exploring state-of-the-art organic TE materials. This review focuses on the regulation of electronic structures of organic materials toward efficient TE conversion. First, we present the basic knowledge regarding electronic structures and the requirements for efficient TE conversion of organic materials, followed by a brief introduction of commonly used methods for electronic structure characterization. Next, we highlight the key strategies of electronic structure engineering for high-performance organic TE materials. Finally, an overview of the electronic structure engineering of organic TE materials, along with current challenges and future research directions, are provided. (C) 2021 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved.
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