期刊
ATMOSPHERE
卷 12, 期 10, 页码 -出版社
MDPI
DOI: 10.3390/atmos12101283
关键词
nitrogen dioxide; sulphur dioxide; carbon monoxide; OMI; TROPOMI
资金
- International Development Research Centre (IDRC)
- Swedish International Development Cooperation Agency (SIDA) through the Artificial Intelligence for Development (AI4D) program
- African Centre for Technology Studies (ACTS).
This study used satellite observations to investigate the trends of nitrogen dioxide, sulfur dioxide, and carbon monoxide in the East African region, identifying seasonal fires in savanna woodlands and urban areas as major sources of pollution. The study found no trend in nitrogen dioxide, a decreasing trend in sulfur dioxide, and varying trends in carbon monoxide at different altitudes in the atmosphere.
The atmospheric chemistry constituents of nitrogen dioxide (NO2), sulphur dioxide (SO2) and carbon monoxide (CO) are associated with air pollution and climate change. In sub-Saharan Africa, a lack of sufficient ground-based and aircraft observations has, for a long time, limited the study of these species. This study thus utilized satellite observations as an alternative source of data to study the abundance of these species over the East African region. The instruments used included the Ozone Monitoring Instrument (OMI), the Atmospheric InfraRed Sounder (AIRS), and the TROPOspheric Monitoring Instrument (TROPOMI). An investigation of trends in the data series from 2005 to 2020 was carried out using the sequential Mann-Kendall test while the Pearson correlation coefficient was used to compare the data records of the instruments. The analysis revealed no trend in NO2 (p > 0.05), a decreasing trend in SO2 (p < 0.05), a decreasing trend (p < 0.05) in CO closer to the surface (850 hPa to 500 hPa) and an increasing trend (p < 0.05) in CO higher up in the atmosphere (400 hPa to 1 hPa). There is likely a vertical ascent of CO. The correlation between the instrument records was 0.54 and 0.77 for NO2 and CO, respectively. Furthermore, seasonal fires in the savanna woodlands were identified as the major source of NO2 and CO over the region, while cities such as Kampala, Nairobi, and Bujumbura and towns such as Dar es Salaam and Mombasa were identified as important NO2 hotspots. Similarly, the active volcano at Mt. Nyiragongo near Goma was identified as the most important SO2 hotspot.
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