期刊
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
卷 9, 期 40, 页码 13663-13671出版社
AMER CHEMICAL SOC
DOI: 10.1021/acssuschemeng.1c05237
关键词
C-H functionalization; amberlyst 15; multibond formation; green solvent; quinoxalinone
资金
- National Natural Science Foundation of China [22178078, 21871071]
A novel and green multicomponent transformation for the alpha-bifunctionalization of methyl ketones has been successfully achieved by combining heterogeneous catalysis and solar photocatalysis, offering a sustainable and practical alternative for the modification of ketone derivatives in water and under an air atmosphere.
Herein, a novel and green multicomponent transformation for the alpha-bifunctionalization of methyl ketones enabled by heterogeneous catalysis and solar photocatalysis has been described. This reaction is performed in water and under an air atmosphere, affording the corresponding products in a moderate-to-good yield. Our transformation shows a successful combination of heterogeneous catalysis and solar photocatalysis, giving a sustainable and practical alternative for the modification of ketone derivatives.
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