期刊
CHEMPLUSCHEM
卷 86, 期 12, 页码 1577-1585出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cplu.202100459
关键词
defects; light-emitting devices; metal halides; photophysics; stability
资金
- National Natural Science Foundation of China [21773200]
- Research Grants Council of Hong Kong [RFS2021-1S03]
All-inorganic zero-dimensional (0D) metal halides are composed of isolated metal halide polyhedrons bridged by monovalent alkali metal ions, exhibiting molecule-like electronic configuration and highly attractive optical properties. Compared to their three-dimensional (3D) counterparts, 0D metal halides show characteristic features such as broadband emission and long-term stability. They can be constructed from a diverse range of metal ions and allow high-level impurity doping, offering great structural designability and spectral tunability.
All-inorganic zero-dimensional (0D) metal halides are composed of isolated metal halide polyhedrons bridged by monovalent alkali metal ions. The unique structure gives rise to molecule-like electronic configuration and consequently highly attractive optical properties. In comparison with their three-dimensional (3D) counterparts, the 0D metal halides exhibit characteristic features such as broadband emission and long-term stability. In addition, 0D metal halides can be constructed from a diverse range of metal ions and permit high-level impurity doping, thereby offering great structural designability and spectral tunability. This Review surveys recent advances in 0D metal halides, including crystal preparation, luminescence modulation, and emerging applications.
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