4.8 Article

Charge-neutral fermions and magnetic field-driven instability in insulating YbIr3Si7

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NATURE COMMUNICATIONS
卷 13, 期 1, 页码 -

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NATURE PORTFOLIO
DOI: 10.1038/s41467-021-27541-9

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资金

  1. U.S. Department of Energy [DE-SC0019503]
  2. National Science Foundation [DMR-1917511]
  3. Robert A. Welch Foundation [C-1818]
  4. Japan Society for the Promotion of Science (JSPS) [JP15H02106, JP18H01177, JP18H01178, JP18H01180, JP18H05227, JP19H00649, JP20H02600, JP18K03511, JP20H05159, JP19H05824]
  5. JST CREST [JP-MJCR19T5]
  6. U.S. Department of Energy (DOE) [DE-SC0019503] Funding Source: U.S. Department of Energy (DOE)

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The coupling between charge-neutral excitations and spin degrees of freedom in the Kondo insulator YbIr3Si7 is demonstrated, putting restrictions on current theories. The thermal conductivity and specific heat measurements reveal emergent neutral excitations in YbIr3Si7, which are sensitively changed by a field-driven transition between antiferromagnetic phases.
Charge-neutral excitations have been proposed to explain metal-like thermal transport in Kondo insulators. Here, the authors demonstrate the coupling between charge-neutral excitations and spin degrees of freedom in a Kondo insulator YbIr3Si7, which puts restrictions on current theories. Kondo lattice materials, where localized magnetic moments couple to itinerant electrons, provide a very rich backdrop for strong electron correlations. They are known to realize many exotic phenomena, with a dramatic example being recent observations of quantum oscillations and metallic thermal conduction in insulators, implying the emergence of enigmatic charge-neutral fermions. Here, we show that thermal conductivity and specific heat measurements in insulating YbIr3Si7 reveal emergent neutral excitations, whose properties are sensitively changed by a field-driven transition between two antiferromagnetic phases. In the low-field phase, a significant violation of the Wiedemann-Franz law demonstrates that YbIr3Si7 is a charge insulator but a thermal metal. In the high-field phase, thermal conductivity exhibits a sharp drop below 300 mK, indicating a transition from a thermal metal into an insulator/semimetal driven by the magnetic transition. These results suggest that spin degrees of freedom directly couple to the neutral fermions, whose emergent Fermi surface undergoes a field-driven instability at low temperatures.

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