期刊
SMALL
卷 17, 期 52, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/smll.202104551
关键词
aggregation; carbon dots; color temperature; electroluminescence; white-light-emitting diodes
类别
资金
- National Natural Science Foundation of China [52102159, 51972060, 12074068, 22103013]
- Natural Science Foundation of Fujian Province [2020J02017]
- Education Department of Fujian Province [JAT200083, JAT200086]
This study demonstrates white CDs-LEDs with adjustable CCTs through the utilization of aggregation-induced emission, achieving white LEDs with different color temperatures. These LEDs exhibit excellent brightness and external quantum efficiency performance.
Carbon dots (CDs) as one of the most promising carbon-based nanomaterials are inspiring extensive research in optoelectronic applications. White-light-emitting diodes (WLEDs) with tunable correlated color temperatures (CCTs) are crucial for applications in white lighting. However, the development of high-performance CDs-based electroluminescent WLEDs, especially those with adjustable CCTs, remains a challenge. Herein, white CDs-LEDs with CCTs from 2863 to 11 240 K are successfully demonstrated by utilizing aggregation-induced emission red-shifting and broadening of CDs. As a result, a series of warm white, pure white, and cold white CDs-LEDs are realized with adjustable emissions in sequence along the blackbody radiation curve. These CDs-LEDs reach maximum brightness and external quantum efficiency up to 1414-4917 cd m(-2) and 0.08-0.87%, respectively, which is among the best performances of white CDs-LEDs. To the best of the authors ' knowledge, this is the first time that CCT-tunable white electroluminescent CDs-LEDs are demonstrated through controlling the aggregation degrees of CDs.
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