Recent Advances on Tuning the Interlayer Coupling and Properties in van der Waals Heterostructures

2D van der Waals (vdW) heterostructures are receiving increasing research attention due to the theoretically amazing properties and unprecedented application potential. However, the as-synthesized heterostructures are generally underperforming due to the weak interlayer coupling, which inspires the researchers to find ways to modulate the interlayer coupling and properties, realizing the tailored performance for actual applications. There have been a lot of publications regarding the controllable regulation of the structures and properties of 2D vdW heterostructures in the past few years, while a review work summarizing the current advances is not yet available, though it is significant. This paper conducts a state-of-the-art review regarding the current research progress of performance modulation of vdW heterostructures by different techniques. First, the general synthesis methods of vdW heterostructures are summarized. Then, different performance modulation techniques, that is, mechanical-based, external fields-assisted, and particle beam irradiation-based methods, are discussed and compared in detail. Some of the newly proposed concepts are described. Thereafter, applications of vdW heterostructures with tailored properties are reviewed for the application prospects of the topic around this area. Moreover, the future research challenges and prospects are discussed, aiming at triggering more research interest and device applications around this topic.

Automated summary

2D vdW heterostructures have attracted research attention for their theoretical properties and application potentials. However, the synthesized heterostructures generally underperform due to weak interlayer coupling. This paper provides a state-of-the-art review of different techniques for performance modulation of vdW heterostructures, summarizing general synthesis methods and discussing mechanical-based, external fields-assisted, and particle beam irradiation-based methods. The applications and future prospects of tailored properties in vdW heterostructures are also reviewed.