4.7 Article

Elastic loading enhanced NH3 sensing for surface acoustic wave sensor with highly porous nitrogen doped diamond like carbon film

期刊

SENSORS AND ACTUATORS B-CHEMICAL
卷 344, 期 -, 页码 -

出版社

ELSEVIER SCIENCE SA
DOI: 10.1016/j.snb.2021.130175

关键词

N doped DLC; Surface acoustic wave (SAW); Elastic modulus; NH3 gas sensor

资金

  1. Fundamental Research Funds for the Central Universities [2682019CX68]
  2. Scientific Research Foundation of SWJTU [A19205020519072032]
  3. National Natural Science Foundation of China [51902272]
  4. UK Engineering and Physical Sciences Research Council (EPSRC) [EP/P018998/1]
  5. Newton Mobility Grant through Royal Society [IE161019]
  6. National Natural Science Foundation of China

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The study introduced a SAW NH3 gas sensor based on NDLC film, characterized by high sensitivity, low noise, and excellent stability, capable of monitoring NH3 gas in a range from 100 ppb to 100 ppm.
We proposed a surface acoustic wave (SAW) NH3 gas sensor based on nitrogen doped diamond like carbon (NDLC) film. The N-DLC film, prepared using a microwave electron cyclotron resonance plasma chemical vapor deposition (ECR-PECVD) method, is highly porous and physically and chemically stable, and have active polar groups on its surface, which can selectively absorb polar NH3 gas molecules. These features of the film lead to the high sensitivity, low noise and excellent stability of the sensor. The sensor can achieve capabilities of in-situ monitoring NH3 in a concentration range from 100 ppb to 100 ppm with fast response (-5 s) and recovery (-29 s) at room temperature. The NH3 sensing mechanism is attributed to the decreased porosity of the N-DLC film caused by adsorbed NH3 molecules on its polar groups, which leads an increase of the elastic modulus of the film.

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