4.7 Article

Enhanced NO2 gas-sensing performance at room temperature using exfoliated MoS2 nanosheets

期刊

SENSORS AND ACTUATORS A-PHYSICAL
卷 332, 期 -, 页码 -

出版社

ELSEVIER SCIENCE SA
DOI: 10.1016/j.sna.2021.113137

关键词

Liquid-phase exfoliation; Exfoliated MoS2 nanosheets; Room temperature; NO2 gas sensor

资金

  1. Ministry of Education and Training [B2021-BKA-07]
  2. Vingroup Joint Stock Company
  3. Domestic Master/PhD Scholarship Programme of Vingroup Innovation Foundation (VINIF), Vingroup Big Data Institute (VINBIGDATA) [VINIF.2020. ThS.98]

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MoS2 nanosheets exfoliated from bulk MoS2 through sonication probe exhibit enhanced NO2 gas sensing properties, with high response rates, low detection limits, and excellent long-term stability, showing potential for future practical applications.
Features such as surface-to-volume ratio, sensitive surface, and bandgap vary with the number of material layers of semiconductor two-dimensional transition metal dichalcogenides with superior responsivity at room temperature (RT) and their possible application as flexible electronic devices. Herein, a significant enhancement of NO2 gas sensing properties of few-layered MoS2 nanosheets exfoliated from bulk MoS2 through a simple sonication probe was reported. The gas responses of the sensor based on the exfoliated MoS2 nanosheets to 0.5-5 ppm NO2 at RT were as high as 5.3-8 times. At RT, the humidity effect to the performance of the exfoliated MoS2 sensor was insignificant. The exfoliated MoS2 sensor also exhibited an ultra-low detection limit of 27 ppb, excellent selectivity, and reliable long-term stability within 8 weeks, which are crucial for future application of the sensor in practical devices. The NO2 sensing mechanism of the exfoliated MoS2 nanosheets was discussed in detail. (C) 2021 Elsevier B.V. All rights reserved.

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