期刊
SCIENCE
卷 375, 期 6578, 页码 302-+出版社
AMER ASSOC ADVANCEMENT SCIENCE
DOI: 10.1126/science.abh1885
关键词
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资金
- Development Program of the Korea Institute of Energy Research (KIER) [C1-2401, C1-2402]
- Basic Science Research Program through the National Research Foundation of Korea (NRF) - Ministry of Education [NRF-2020R1A6A1A03038697]
- NRF - Ministry of Science, ICT, and Future Planning [2020M1A2A2080746, 2020M1A2A208075011]
- European Union [881603, 764047]
The study replaced the commonly used mesoporous titanium dioxide electron transport layer with a thin layer of polyacrylic acid-stabilized tin(IV) oxide quantum dots, which improved the efficiency and stability of perovskite solar cells and enabled successful scaling up of PSCs production.
Improvements to perovskite solar cells (PSCs) have focused on increasing their power conversion efficiency (PCE) and operational stability and maintaining high performance upon scale-up to module sizes. We report that replacing the commonly used mesoporous-titanium dioxide electron transport layer (ETL) with a thin layer of polyacrylic acid-stabilized tin(IV) oxide quantum dots (paa-QD-SnO2) on the compact-titanium dioxide enhanced light capture and largely suppressed nonradiative recombination at the ETL-perovskite interface. The use of paa-QD-SnO2 as electron-selective contact enabled PSCs (0.08 square centimeters) with a PCE of 25.7% (certified 25.4%) and high operational stability and facilitated the scale-up of the PSCs to larger areas. PCEs of 23.3, 21.7, and 20.6% were achieved for PSCs with active areas of 1, 20, and 64 square centimeters, respectively.
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