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A review on particulate photocatalytic hydrogen production system: Progress made in achieving high energy conversion efficiency and key challenges ahead

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出版社

PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.rser.2021.111694

关键词

Particulate photocatalytic water-splitting system; Hydrogen production; Photo-reforming; Solar to hydrogen conversion efficiency; Sustainable energy

资金

  1. Department of Science and Technology-Solar Energy Research Initiative (DST-SERI) [DST/TM/SERI/S170(G)]

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Photocatalytic water splitting is a sustainable and clean method for producing renewable hydrogen. Various existing particulate photocatalytic systems have been used for hydrogen production through overall water splitting and photo-reforming of biomass-derived organic substances. Progress has been made in improving the efficiency of existing photocatalysts. Factors affecting the particulate photocatalytic water splitting system need to be addressed to overcome limitations and enhance large-scale hydrogen production efficiency.
Photocatalytic water splitting is a sustainable and clean method to produce renewable hydrogen. The particulate photocatalytic water splitting system has been envisioned as an efficient and cost-effective solution for largescale hydrogen production. Herein, we have reviewed the various existing particulate photocatalytic systems for hydrogen production via overall water splitting, as well as via photo-reforming of biomass-derived organic substances. The progress made in improving the apparent quantum efficiency and solar to the hydrogen conversion efficiency of existing photocatalysts is highlighted. The factors affecting the particulate photocatalytic water splitting system are summarized. Finally, some of the key limitations and future perspectives on large-scale hydrogen production are discussed.

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