4.8 Article

Cyclotron resonance overtones and near-field magnetoabsorption via terahertz Bernstein modes in graphene

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NATURE PHYSICS
卷 18, 期 4, 页码 462-+

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NATURE PORTFOLIO
DOI: 10.1038/s41567-021-01494-8

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资金

  1. Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) [314695032, SFB 1277]
  2. DFG [DM 1/5-1]
  3. AFOSR [FA955021-1-0319]
  4. NSF QII-TAQS program [1936263]
  5. Gordon and Betty Moore Foundation EPiQS Initiative [GBMF9643]
  6. MIT Pappalardo Fellowship
  7. MIT undergraduate research opportunities program
  8. Johnson & Johnson research scholars program
  9. National Science Foundation [CMMI 1538127]
  10. Foundation for Advancement of Theoretical Physics 'Basis' [20-1-3-43-1]
  11. Ministry of Science and Higher Education of the Russian Federation [075-15-2021-606]

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Deviation from cyclotron resonance behavior in graphene is reported, showing overtone resonances due to ultraslow magnetoplasmonic excitations. Absorption of radiation via non-local collective modes can facilitate a strong photoresponse, potentially useful for infrared and terahertz technology.
Electrons in an external magnetic field absorb electromagnetic radiation via cyclotron resonance. Deviations from this behaviour in the form of overtone resonances due to ultraslow magnetoplasmonic excitations are now reported for graphene. Two-dimensional electron systems subjected to a perpendicular magnetic field absorb electromagnetic radiation via cyclotron resonance (CR). Here we report a qualitative deviation from this well-known behaviour in graphene. Our measurements of the terahertz photoresponse reveal a resonant burst at the main overtone of the CR that exceeds the signal detected at the position of the ordinary CR. The dependencies of photoresponse on the magnetic field, doping level and sample geometry suggest that the origin of this anomaly lies in the near-field magnetoabsorption facilitated by the Bernstein modes-ultraslow magnetoplasmonic excitations reshaped by non-local electron dynamics. Close to CR harmonics, these modes are characterized by a flat dispersion and diverging plasmonic density of states that amplify radiation absorption. Besides carrying fundamental interest, our results show that radiation absorption via non-local collective modes can facilitate a strong photoresponse-a behaviour potentially useful for infrared and terahertz technology.

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