Soybean Protein Fiber Enabled Controllable Li Deposition and a LiF-Nanocrystal-Enriched Interface for Stable Li Metal Batteries

Review Chemistry, Physical

Probing Lithium Metals in Batteries by Advanced Characterization and Analysis Tools

Hyeokjun Park et al.

Summary: Despite decades of research, uncontrolled lithium growth and accompanying side reactions continue to hinder the development of lithium metal batteries.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Dynamic Regulation of Lithium Dendrite Growth with Electromechanical Coupling Effect of Soft BaTiO3 Ceramic Nanofiber Films

Shuhui Xia et al.

Summary: A soft BaTiO3 ceramic nanofiber film with excellent ferroelectricity and piezoelectricity is reported for regulating the deposition of Li metal, addressing the issue of dendrite growth in lithium metal batteries. Experimental results demonstrate that Li-Cu cells using this film exhibit high Coulombic efficiency over 200 cycles, while LMBs paired with high-voltage cathodes maintain 80% capacity in 300 cycles.

ACS NANO (2021)

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Article Chemistry, Multidisciplinary

Identifying the Critical Anion-Cation Coordination to Regulate the Electric Double Layer for an Efficient Lithium-Metal Anode Interface

Rui Xu et al.

Summary: The electric double layer (EDL) chemistry at the electrode/electrolyte interface is found to predominantly control the competitive reduction reactions during SEI construction on Li metal anode. Introducing multi-valent cation additives has been validated as a promising strategy to enhance the performance of SEI, shedding new light on the targeted regulation of reactive alkali metal interfaces.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Gradient Solid Electrolyte Interphase and Lithium-Ion Solvation Regulated by Bisfluoroacetamide for Stable Lithium Metal Batteries

Fang Li et al.

Summary: This study focuses on the impact of bisfluoroacetamide (BFA) as an electrolyte additive on the solid electrolyte interphase (SEI) structure. By constructing a gradient SEI structure, it achieves better Li ion capture and transportation effects.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Polycationic Polymer Layer for Air-Stable and Dendrite-Free Li Metal Anodes in Carbonate Electrolytes

Jingyi Wu et al.

Summary: Controllable dendrite growth in lithium metal batteries has been a major obstacle to their commercialization. A polycationic and hydrophobic polymer protective layer has been developed to address this issue, allowing for stable and efficient Li metal anodes. This protective layer enables steady Li plating/stripping, improved Li utilization efficiency, and enhanced electrochemical performance in cells utilizing LiNi0.8Mn0.1Co0.1O2 and LiFePO4. The layer also contributes to the formation of a stable solid electrolyte interphase (SEI), as demonstrated through mechanism investigation.

ADVANCED MATERIALS (2021)

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Article Engineering, Environmental

A fast-ion conducting interface enabled by aluminum silicate fibers for stable Li metal batteries

Zhijin Ju et al.

Summary: By constructing a fast-ion conducting interface using ASO fibers, safety hazards caused by the growth of Li dendrites on the Li metal anode can be addressed, leading to a stable long-term lifespan. When paired with ASO, the cell can achieve over 500 cycles with reduced capacity degradation.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Multidisciplinary

Stabilized Solid Electrolyte Interphase Induced by Ultrathin Boron Nitride Membranes for Safe Lithium Metal Batteries

Jinzhi Sheng et al.

Summary: The use of an ultrathin hBN/PI layer on a commercial PP separator effectively suppresses dendrite growth in lithium-ion batteries and reduces active lithium consumption, while also providing good electrolyte wettability, mechanical strength, thermal conductivity, and high thermal stability. This modification results in stable battery capacity even after long cycling and at high temperatures.

NANO LETTERS (2021)

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Article Energy & Fuels

Rejuvenating dead lithium supply in lithium metal anodes by iodine redox

Chengbin Jin et al.

Summary: The researchers use an iodic species to react with inactive lithium, bringing it back to life and thus making batteries last longer.

NATURE ENERGY (2021)

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Review Chemistry, Multidisciplinary

Visualizing the Sensitive Lithium with Atomic Precision: Cryogenic Electron Microscopy for Batteries

Yujing Liu et al.

Summary: Cryo-EM technology plays a significant role in revealing the structure of electron beam-sensitive lithium in battery materials, enabling high-resolution imaging at the atomic scale. Cryo-EM allows for better monitoring of lithium lattice ordering, nanostructures of the solid electrolyte interface, and aids in the design of high-performance lithium metal batteries.

ACCOUNTS OF CHEMICAL RESEARCH (2021)

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Article Chemistry, Applied

In-situ construction of a Mg-modified interface to guide uniform lithium deposition for stable all-solid-state batteries

Tiefeng Liu et al.

Summary: Introducing a Mg-modified interface in the anode/electrolyte interface of all-solid-state Li metal batteries can lead to more uniform lithium deposition and a smoother interface. The Mg-modified electrolyte shows excellent cycling performance and cycling lifespan in Li/Li symmetric cells and full LFP/Li cells.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Article Chemistry, Physical

Silicious nanowires enabled dendrites suppression and flame retardancy for advanced lithium metal anodes

Yujing Liu et al.

Summary: By designing a three-dimensional network structure with high specific surface area, strong electrolyte affinity, and flame-retardant properties, the safety hazards caused by dendritic Li plating in lithium metal batteries can be reduced, leading to dendrite-free Li deposition and improved cycle performance and safety.

NANO ENERGY (2021)

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Article Chemistry, Multidisciplinary

Marrying Ester Group with Lithium Salt: Cellulose-Acetate-Enabled LiF-Enriched Interface for Stable Lithium Metal Anodes

Mei Chen et al.

Summary: This study investigates the use of ion-affiliative cellulose acetate and functional Li salts to suppress dendritic Li growth in high-energy-density lithium metal batteries. The SEI structure with fast Li+ diffusion kinetics efficiently prevents the formation of Li dendrites, extending battery lifespan at high current densities.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Self-Healing Nucleation Seeds Induced Long-Term Dendrite-Free Lithium Metal Anode

Pengbo Zhai et al.

Summary: Utilizing liquid gallium-indium (GaIn) nanoparticles with structural self-healing properties to guide uniform metallic lithium nucleation and deposition effectively addresses the issue of Li dendrite growth during charge/discharge processes. The self-healing design of nucleation seeds provides important insights for achieving high-performance lithium metal anodes.

NANO LETTERS (2021)

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Review Nanoscience & Nanotechnology

Cryo-Electron Microscopy for Unveiling the Sensitive Battery Materials

Zhijin Ju et al.

Summary: In-depth chemical and structural investigation of battery components is crucial for exploring new electrode materials and their performance iterations for high energy density energy storage devices. Cryo-electron microscopy offers great opportunities for high-resolution imaging of sensitive battery materials while maintaining their native state, contributing to a better understanding of electrode materials for high-performance rechargeable batteries.

SMALL SCIENCE (2021)

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Review Nanoscience & Nanotechnology

Thermally Stable and Nonflammable Electrolytes for Lithium Metal Batteries: Progress and Perspectives

Qian-Kui Zhang et al.

Summary: The article discusses the thermal runaway mechanisms of lithium metal batteries, measurement methods for thermal stability and nonflammability of liquid electrolytes, as well as recent progress in nonflammable electrolytes for lithium metal batteries. Future perspectives on designing thermally stable and nonflammable electrolytes for lithium metal batteries are also presented.

SMALL SCIENCE (2021)

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Review Nanoscience & Nanotechnology

Armed lithium metal anodes with functional skeletons

C. Jin et al.

Summary: Lithium metal batteries have attracted attention due to their high theoretical capacity and low reduction potential, but face challenges in practical applications, with functional skeletons being an attractive approach to overcome these challenges.

MATERIALS TODAY NANO (2021)

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Review Chemistry, Multidisciplinary

Biomass-based materials for green lithium secondary batteries

Chengbin Jin et al.

Summary: The advances in process engineering, nanotechnology, and materials science have made it possible for biomass to be used in novel energy storage technologies like lithium secondary batteries (LSBs). Biomass-derived materials can be sustainable battery components, contributing to green battery systems. This review provides a comprehensive overview of the fabrication and application of biomass and biomass-derived materials in LSBs, emphasizing the potential for high-performance green battery systems.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Nanoscience & Nanotechnology

Synergistic Effects of Inorganic-Organic Protective Layer for Robust Cycling Dendrite-Free Lithium Metal Batteries

Xing Gao et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Multidisciplinary

A Highly Reversible, Dendrite-Free Lithium Metal Anode Enabled by a Lithium-Fluoride-Enriched Interphase

Chunyu Cui et al.

ADVANCED MATERIALS (2020)

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Article Multidisciplinary Sciences

Biomacromolecules enabled dendrite-free lithium metal battery and its origin revealed by cryo-electron microscopy

Zhijin Ju et al.

NATURE COMMUNICATIONS (2020)

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Article Multidisciplinary Sciences

Mechanical rolling formation of interpenetrated lithium metal/lithium tin alloy foil for ultrahigh-rate battery anode

Mintao Wan et al.

NATURE COMMUNICATIONS (2020)

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Article Chemistry, Multidisciplinary

Colossal Granular Lithium Deposits Enabled by the Grain-Coarsening Effect for High-Efficiency Lithium Metal Full Batteries

Weidong Zhang et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

A Lithium Metal Anode Surviving Battery Cycling Above 200 °C

Lin Fu et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

In Situ Construction of a LiF-Enriched Interface for Stable All-Solid-State Batteries and its Origin Revealed by Cryo-TEM

Ouwei Sheng et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Physical

Arrayed silk fibroin for high-performance Li metal batteries and atomic interface structure revealed by cryo-TEM

Baolin Zhang et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Article Multidisciplinary Sciences

Immunizing lithium metal anodes against dendrite growth using protein molecules to achieve high energy batteries

Tianyi Wang et al.

NATURE COMMUNICATIONS (2020)

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Review Chemistry, Multidisciplinary

Towards practical lithium-metal anodes

Xin Zhang et al.

CHEMICAL SOCIETY REVIEWS (2020)

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Article Chemistry, Physical

Polymer-inorganic solid-electrolyte interphase for stable lithium metal batteries under lean electrolyte conditions

Yue Gao et al.

NATURE MATERIALS (2019)

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Article Chemistry, Physical

Sericin protein as a conformal protective layer to enable air-endurable Li metal anodes and high-rate Li-S batteries

Han Wu et al.

JOURNAL OF POWER SOURCES (2019)

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Article Energy & Fuels

Improving cyclability of Li metal batteries at elevated temperatures and its origin revealed by cryo-electron microscopy

Jiangyan Wang et al.

NATURE ENERGY (2019)

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Article Multidisciplinary Sciences

Quantifying inactive lithium in lithium metal batteries

Chengcheng Fang et al.

NATURE (2019)

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Article Energy & Fuels

Monolithic solid-electrolyte interphases formed in fluorinated orthoformate-based electrolytes minimize Li depletion and pulverization

Xia Cao et al.

NATURE ENERGY (2019)

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Article Chemistry, Physical

Confinement effect and air tolerance of Li plating by lithiophilic poly(vinyl alcohol) coating for dendrite-free Li metal batteries

Han Wu et al.

JOURNAL OF MATERIALS CHEMISTRY A (2019)

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Article Chemistry, Physical

High-Efficiency Lithium-Metal Anode Enabled by Liquefied Gas Electrolytes

Yangyuchen Yang et al.

JOULE (2019)

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Article Chemistry, Physical

Fabrication of Hybrid Silicate Coatings by a Simple Vapor Deposition Method for Lithium Metal Anodes

Fang Liu et al.

ADVANCED ENERGY MATERIALS (2018)

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Article Multidisciplinary Sciences

A cation-anion regulation synergistic anode host for dendrite-free lithium metal batteries

Weidong Zhang et al.

SCIENCE ADVANCES (2018)

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Article Chemistry, Multidisciplinary

An Armored Mixed Conductor Interphase on a Dendrite-Free Lithium-Metal Anode

Chong Yan et al.

ADVANCED MATERIALS (2018)

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Article Chemistry, Multidisciplinary

Lithium Nitrate Solvation Chemistry in Carbonate Electrolyte Sustains High-Voltage Lithium Metal Batteries

Chong Yan et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Article Chemistry, Multidisciplinary

Uniform Li deposition regulated via three-dimensional polyvinyl alcohol nanofiber networks for effective Li metal anodes

Gang Wang et al.

NANOSCALE (2018)

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Article Energy & Fuels

Stable metal battery anodes enabled by polyethylenimine sponge hosts by way of electrokinetic effects

Guoxing Li et al.

NATURE ENERGY (2018)

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Article Multidisciplinary Sciences

An ion redistributor for dendrite-free lithium metal anodes

Chen-Zi Zhao et al.

SCIENCE ADVANCES (2018)

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Article Chemistry, Physical

Correlating Structure and Function of Battery Interphases at Atomic Resolution Using Cryoelectron Microscopy

Yuzhang Li et al.

JOULE (2018)

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Article Chemistry, Multidisciplinary

Building Organic/Inorganic Hybrid Interphases for Fast Interfacial Transport in Rechargeable Metal Batteries

Qing Zhao et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Article Multidisciplinary Sciences

Development of Eco-friendly Soy Protein Isolate Films with High Mechanical Properties through HNTs, PVA, and PTGE Synergism Effect

Xiaorong Liu et al.

SCIENTIFIC REPORTS (2017)

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Review Chemistry, Multidisciplinary

Toward Safe Lithium Metal Anode in Rechargeable Batteries: A Review

Xin-Bing Cheng et al.

CHEMICAL REVIEWS (2017)

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Article Chemistry, Multidisciplinary

Dendrite-Free Lithium Deposition Induced by Uniformly Distributed Lithium Ions for Efficient Lithium Metal Batteries

Xin-Bing Cheng et al.

ADVANCED MATERIALS (2016)

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Article Chemistry, Multidisciplinary

Correlating Microstructural Lithium Metal Growth with Electrolyte Salt Depletion in Lithium Batteries Using 7Li MRI

Hee Jung Chang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2015)

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Article Chemistry, Physical

Carbon-Nanotube-Decorated Nano-LiFePO4 @C Cathode Material with Superior High-Rate and Low-Temperature Performances for Lithium-Ion Batteries

Xing-Long Wu et al.

ADVANCED ENERGY MATERIALS (2013)

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Editorial Material Chemistry, Multidisciplinary

Hierarchical Carbon-Coated LiFePO4 Nanoplate Microspheres with High Electrochemical Performance for Li-Ion Batteries

Yongmin Wu et al.

ADVANCED MATERIALS (2011)

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Review Biochemistry & Molecular Biology

Infrared spectroscopy of proteins

Andreas Barth

BIOCHIMICA ET BIOPHYSICA ACTA-BIOENERGETICS (2007)

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Soybean Protein Fiber Enabled Controllable Li Deposition and a LiF-Nanocrystal-Enriched Interface for Stable Li Metal Batteries

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