期刊
MICROPOROUS AND MESOPOROUS MATERIALS
卷 326, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.micromeso.2021.111362
关键词
Seed-assisted; Aluminosilicate; ITQ-58 zeolite
类别
资金
- National Natural Science Foundation of China [21971259, 21850316]
The aluminosilicate form of ITQ-58 can be directly synthesized using Si/B-ITQ-58 zeolite as seed, exhibiting excellent properties for use as a heterogeneous catalyst in the Biginelli reaction. This method confirms the new function of seed-assisted synthesis in preparing aluminosilicates.
The aluminosilicate form of ITQ-58 has been directly synthesized in the synthesis gel SiO2-Al2O3-Na2O-H2O using Si/B-ITQ-58 zeolite as seed. Si/Al-ITQ-58 exhibits good crystallinity, high surface area, tetrahedral Al3+ species, and middle acid sites. The acidic form of Si/Al-ITQ-58 zeolite, is an excellent alternative heterogeneous catalyst with high yield and simple product separation, used for Biginelli reaction. Therefore, with the second case, we further confirm the new function of seed-assisted synthesis, i.e., direct aluminosilicate preparation.
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