期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 87, 期 1, 页码 884-891出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.1c02667
关键词
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资金
- Council of Scientific and Industrial Research (CSIR)
- Department of Science and Technology (DST), New Delhi [GAP-584]
- Science and Engineering Research Board [PDF/2020/001111]
- Dr. Reddy's Laboratory (DRL)
An efficient protocol for the synthesis of orthogonally strap diynones through one pot transition-metal-free reaction has been developed. Insights into the regioselective tandem Michael-anti-Michael processes have been gleaned through DFT calculations.
An efficient protocol involving the transformation of sequentially generated recursive anions from heterocyclic precursors to orthogonally strap diynones through one pot transition-metal-free spirocyclopentannulation has been devised, employing oxindoles and pyrazolones as prototypical platforms. Insights into these regioselective tandem Michael-anti-Michael processes have been gleaned through DFT calculations.
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