Insights into the performance and degradation of polybenzimidazole/muscovite composite membranes in high-temperature proton exchange membrane fuel cells

Article Chemistry, Applied

High-performance polymer electrolyte membranes incorporated with 2D silica nanosheets in high-temperature proton exchange membrane fuel cells

Zunmin Guo et al.

Summary: By incorporating silica nanosheets (SN) into PES-PVP polymer matrix, the high-temperature proton exchange membrane showed enhanced proton conductivity and power density, demonstrating the potential of using SN in HT-PEMs production.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Environmental Sciences

Zirconium-modified natural clays for phosphate removal: Effect of clay minerals

Jingwan Huo et al.

Summary: This study investigated the effect of Zr-modified clays on phosphate adsorption, showing that Zr-modified montmorillonite had the fastest kinetics and highest capacity. The different performances of Zr-modified clays may be attributed to the distinct expansion properties. All Zr-modified clays demonstrated robust phosphate adsorption under various water chemistry conditions, with inner-sphere surface complexes formation being proposed as the primary mechanism.

ENVIRONMENTAL RESEARCH (2021)

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Article Chemistry, Physical

One step electrochemical exfoliation of natural graphite flakes into graphene oxide for polybenzimidazole composite membranes giving enhanced performance in high temperature fuel cells

Jianuo Chen et al.

Summary: A 3D-printed reactor was designed for electrochemical exfoliation of natural graphite flakes to obtain high degree of oxidation graphene oxide. By adjusting the electrolyte concentration and reaction time, the degree of oxidation can be further increased. The electrochemically exfoliated graphene oxide was successfully used to prepare composite membranes for high-temperature polymer electrolyte membrane fuel cells, resulting in significant improvement in peak power density.

JOURNAL OF POWER SOURCES (2021)

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Article Chemistry, Physical

Degradation study of high temperature proton exchange membrane fuel cell under start/stop and load cycling conditions

Jingjing Li et al.

Summary: This study conducted 600-hour accelerated stress tests on high temperature proton exchange membrane fuel cells (HT-PEMFCs) and found that load cycling between 0.04 and 0.2 A cm-2 aggravates performance degradation. Activation polarization was identified as the main factor contributing to performance degradation, while ohmic polarization had a smaller impact. Severe acid loss emerged as a critical issue for the long-term durability of HT-PEMFC.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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Article Engineering, Chemical

Achieving high power density and excellent durability for high temperature proton exchange membrane fuel cells based on crosslinked branched polybenzimidazole and metal-organic frameworks

Yingnan Wu et al.

Summary: This study utilized crosslinked branched PBI as the matrix and introduced MOF UiO-66 to construct proton transport channels, effectively improving the proton conductivity and long-term stability of the composite membrane. In fuel cell tests, the MEA based on the composite membrane achieved a good peak power density at high temperatures, demonstrating excellent durability.

JOURNAL OF MEMBRANE SCIENCE (2021)

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Review Chemistry, Applied

Recent advances in phosphoric acid-based membranes for high-temperature proton exchange membrane fuel cells

Zunmin Guo et al.

Summary: Efforts to design and develop phosphoric acid-based proton exchange membrane for high-temperature fuel cells have been made globally. Various approaches, including crosslinking, introducing antioxidative groups, and incorporating inorganic materials, have been proposed to mitigate the degradation of the membranes. Crosslinking, blending with stable polymers and inorganic materials, and preparing polymers with high molecular weight are recommended to improve membrane mechanical strength. Three promising approaches to improve the durability of HT-PEMFCs include crosslinking, incorporating hygroscopic inorganic materials, and increasing membrane layers or introducing strong basic groups and electron-withdrawing groups.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Article Energy & Fuels

Novel nanocomposite membranes based on PBI and doped-perovskite nanoparticles as a strategy for improving PEMFC performance at high temperatures

Khadijeh Hooshyari et al.

INTERNATIONAL JOURNAL OF ENERGY RESEARCH (2020)

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Article Chemistry, Physical

Three-layered electrolyte membranes with acid reservoir for prolonged lifetime of high-temperature polymer electrolyte membrane fuel cells

Arvind Kannan et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2020)

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Article Materials Science, Multidisciplinary

High temperature anhydrous proton exchange membranes based on chemically-functionalized titanium/polybenzimidazole composites for fuel cells

Sangrae Lee et al.

MATERIALS LETTERS (2020)

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Article Chemistry, Physical

Sulfonated graphene oxide as an inorganic filler in promoting the properties of a polybenzimidazole membrane as a high temperature proton exchange membrane

Yusra Nadzirah Yusoff et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2020)

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Article Chemistry, Physical

Catalytic degradation of P-chlorophenol by muscovite-supported nano zero valent iron composite: Synthesis, characterization, and mechanism studies

Teng Bao et al.

APPLIED CLAY SCIENCE (2020)

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Article Engineering, Chemical

High temperature membranes based on PBI/sulfonated polyimide and doped-perovskite nanoparticles for PEM fuel cells

Khadijeh Hooshyari et al.

JOURNAL OF MEMBRANE SCIENCE (2020)

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Review Energy & Fuels

Fuel cell system for Honda CLARITY fuel cell

Shintaro Tanaka et al.

ETRANSPORTATION (2020)

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Article Engineering, Chemical

Poly(2,5-benzimidazole)/sulfonated sepiolite composite membranes with low phosphoric acid doping levels for PEMFC applications in a wide temperature range

Xiaoxiao Zhang et al.

JOURNAL OF MEMBRANE SCIENCE (2019)

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Article Polymer Science

Polybenzimidazole-Clay Nanocomposite Membrane for PEM fuel cell: Effect of organomodifier structure

Shuvra Singha et al.

POLYMER (2019)

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Article Chemistry, Physical

Van der Waals heteroepitaxial AZO/NiO/AZO/muscovite (ANA/muscovite) transparent flexible memristor

Van-Qui Le et al.

NANO ENERGY (2019)

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Article Materials Science, Multidisciplinary

van der Waals heteroepitaxy on muscovite

Min Yen et al.

MATERIALS CHEMISTRY AND PHYSICS (2019)

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Review Green & Sustainable Science & Technology

Comprehensive investigation on hydrogen and fuel cell technology in the aviation and aerospace sectors

Ahmad Baroutaji et al.

RENEWABLE & SUSTAINABLE ENERGY REVIEWS (2019)

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Article Environmental Sciences

Effective decontamination of phosphate and ammonium utilizing novel muscovite/phillipsite composite; equilibrium investigation and realistic application

Mostafa R. Abukhadra et al.

SCIENCE OF THE TOTAL ENVIRONMENT (2019)

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Article Thermodynamics

Efficiency analysis and control of a grid-connected PEM fuel cell in distributed generation

Li Sun et al.

ENERGY CONVERSION AND MANAGEMENT (2019)

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Article Nanoscience & Nanotechnology

Atomically thin micas as proton-conducting membranes

L. Mogg et al.

NATURE NANOTECHNOLOGY (2019)

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Article Engineering, Chemical

Introduction of milled kaolinite obtained by mechanosynthesis to cement mixture for the production of mortar: Study of mechanical performance of modified mortar

Rabah Hamzaoui et al.

POWDER TECHNOLOGY (2019)

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Article Chemistry, Physical

CHS-WSiA doped hexafluoropropylidene-containing polybenzimidazole composite membranes for medium temperature dry fuel cells

Y. X. Ooi et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2019)

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Article Chemistry, Physical

Design of sepiolite-supported ionogel-embedded composite membranes without proton carrier wastage for wide-temperature-range operation of proton exchange membrane fuel cells

Xiaoxiao Zhang et al.

JOURNAL OF MATERIALS CHEMISTRY A (2019)

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Article Chemistry, Physical

Comprehensive performance enhancement of polybenzimidazole based high temperature proton exchange membranes by doping with a novel intercalated proton conductor

Suwen Wang et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2018)

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Article Chemistry, Physical

Synthesis of sole cancrinite phase from raw muscovite: Characterization and optimization

Ali Q. Selim et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2018)

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Article Engineering, Chemical

High durability sulfonated poly (ether ether ketone)-ceria nanocomposite membranes for proton exchange membrane fuel cell applications

Mohammad Javad Parnian et al.

JOURNAL OF MEMBRANE SCIENCE (2018)

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Article Engineering, Chemical

1,2,4-Triazole functionalized poly(arylene ether ketone) for high temperature proton exchange membrane with enhanced oxidative stability

Fanzhe Bu et al.

JOURNAL OF MEMBRANE SCIENCE (2018)

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Article Engineering, Chemical

Polybenzimidazole (PBI-OO) based composite membranes using sulfophenylated TiO2 as both filler and crosslinker, and their use in the HT-PEM fuel cell

N. Nambi Krishnana et al.

JOURNAL OF MEMBRANE SCIENCE (2018)

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Article Chemistry, Physical

Crosslinked polybenzimidazoles containing branching structure as membrane materials with excellent cell performance and durability for fuel cell applications

Meishao Hu et al.

JOURNAL OF POWER SOURCES (2018)

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Article Electrochemistry

Long-Term Durability of PBI-Based HT-PEM Fuel Cells: Effect of Operating Parameters

Tonny Sondergaard et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2018)

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Article Chemistry, Physical

Electric response and conductivity mechanism reciprocity in H3PO4-doped Polybenzimidazole-4N-ZrO2 nanocomposite membranes

Graeme Nawn et al.

SOLID STATE IONICS (2018)

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Article Chemistry, Physical

Effects of carbon corrosion on mass transfer losses in proton exchange membrane fuel cells

Xu Zhang et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2017)

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Article Chemistry, Physical

Construction of proton channels and reinforcement of physicochemical properties of oPBI/FeSPP/GF high temperature PEM via building hydrogen bonding network

Peng Sun et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2017)

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Article Chemistry, Physical

Polybenzimidazole based nanocomposite membranes with enhanced proton conductivity for high temperature PEM fuel cells

Yagmur Ozdemir et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2017)

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Article Chemistry, Physical

Development of polybenzimidazole/graphene oxide composite membranes for high temperature PEM fuel cells

Nurhan Uregen et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2017)

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Article Electrochemistry

In Situ Formed Phosphoric Acid/Phosphosilicate Nanoclusters in the Exceptional Enhancement of Durability of Polybenzimidazole Membrane Fuel Cells at Elevated High Temperatures

Jin Zhang et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2017)

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Article Chemistry, Physical

Polybenzimidazole-based mixed membranes with exceptionally high water vapor permeability and selectivity

F. H. Akhtar et al.

JOURNAL OF MATERIALS CHEMISTRY A (2017)

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Article Electrochemistry

Electric Response and Conductivity Mechanism in H3PO4-Doped Polybenzimidazole-4N-HfO2 Nanocomposite Membranes for High Temperature Fuel Cells

Graeme Nawn et al.

ELECTROCHIMICA ACTA (2017)

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Article Chemistry, Physical

Effects of mechanical and thermal activation on pozzolanic activity of kaolin containing mica

Biljana Ilic et al.

APPLIED CLAY SCIENCE (2016)

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Article Electrochemistry

Impact of Accelerated Stress Tests on High Temperature PEMFC Degradation

D. Schonvogel et al.

FUEL CELLS (2016)

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Article Chemistry, Physical

Enhancement of performance of pyridine modified polybenzimidazole fuel cell membranes using zirconium oxide nanoclusters and optimized phosphoric acid doping level

Mohamed Mahmoud Nasef et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2016)

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Review Chemistry, Physical

A comprehensive review of PBI-based high temperature PEM fuel cells

Samuel Simon Araya et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2016)

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Article Chemistry, Physical

Polybenzimidazole/SiO2 hybrid membranes for high temperature proton exchange membrane fuel cells

Yilser Devrim et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2016)

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Article Polymer Science

Influence of interfacial interactions on the properties of polybenzimidazole/clay nanocomposite electrolyte membrane

Shuvra Singha et al.

POLYMER (2016)

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Article Chemistry, Multidisciplinary

Nanocomposite Membranes based on Polybenzimidazole and ZrO2 for High-Temperature Proton Exchange Membrane Fuel Cells

Graeme Nawn et al.

CHEMSUSCHEM (2015)

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Article Electrochemistry

Dynamic Operation of HT-PEFC: In-Operando Imaging of Phosphoric Acid Profiles and (Re)distribution

S. H. Eberhardt et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2015)

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Article Engineering, Chemical

Structural and thermal behavior of proclay kaolinite using high energy ball milling process

Rabah Hamzaoui et al.

POWDER TECHNOLOGY (2015)

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Review Green & Sustainable Science & Technology

Approaches to polymer electrolyte membrane fuel cells (PEMFCs) and their cost

Nayibe Guerrero Moreno et al.

RENEWABLE & SUSTAINABLE ENERGY REVIEWS (2015)

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Article Polymer Science

Interplay between Composition, Structure, and Properties of New H3PO4-Doped PBI4N-HfO2 Nanocomposite Membranes for High-Temperature Proton Exchange Membrane Fuel Cells

Graeme Nawn et al.

MACROMOLECULES (2015)

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Article Electrochemistry

Toyota MIRAI Fuel Cell Vehicle and Progress Toward a Future Hydrogen Society

Toshihiko Yoshida et al.

ELECTROCHEMICAL SOCIETY INTERFACE (2015)

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Article Chemistry, Physical

Ion Conducting Membranes for Fuel Cells and other Electrochemical Devices

Klaus-Dieter Kreuer

CHEMISTRY OF MATERIALS (2014)

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Article Engineering, Electrical & Electronic

Analysis and Compensation of PEM Fuel Cell Instabilities in Low-Frequency EIS Measurements

Giovanni Dotelli et al.

IEEE TRANSACTIONS ON INSTRUMENTATION AND MEASUREMENT (2014)

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Article Engineering, Chemical

Influence of the size and shape of silica nanoparticles on the properties and degradation of a PBI-based high temperature polymer electrolyte membrane

T. Ossiander et al.

JOURNAL OF MEMBRANE SCIENCE (2014)

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Article Materials Science, Multidisciplinary

Protonated montmorillonite as a highly effective proton-conductivity enhancer in p-PBI membranes for PEM fuel cells

Filip Ublekov et al.

MATERIALS LETTERS (2014)

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Article Chemistry, Physical

Degradation in phosphoric acid doped polymer fuel cells: A 6000 h parametric investigation

Samuele Galbiati et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2013)

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Review Chemistry, Physical

High temperature (HT) polymer electrolyte membrane fuel cells (PEMFC) - A review

Amrit Chandan et al.

JOURNAL OF POWER SOURCES (2013)

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Article Chemistry, Physical

Crosslinked Hexafluoropropylidene Polybenzimidazole Membranes with Chloromethyl Polysulfone for Fuel Cell Applications

Jingshuai Yang et al.

ADVANCED ENERGY MATERIALS (2013)

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Article Engineering, Chemical

High-temperature proton exchange membranes based on polybenzimidazole and clay composites for fuel cells

David Plackett et al.

JOURNAL OF MEMBRANE SCIENCE (2011)

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Article Chemistry, Physical

Role of Clays Structures on the Polybenzimidazole Nanocomposites: Potential Membranes for the Use in Polymer Electrolyte Membrane Fuel Cell

Sandip Ghosh et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2011)

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Review Chemistry, Multidisciplinary

Proton-conducting membranes based on benzimidazole polymers for high-temperature PEM fuel cells. A chemical quest

Juan Antonio Asensio et al.

CHEMICAL SOCIETY REVIEWS (2010)

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Article Electrochemistry

Design of an allsolid-state'' supercapacitor based on phosphoric acid doped polybenzimidazole (PBI) electrolyte

Dhanraj Rathod et al.

JOURNAL OF APPLIED ELECTROCHEMISTRY (2009)

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Article Engineering, Chemical

Enhancement of the gas separation properties of polybenzimidazole (PBI) membrane by incorporation of silica nano particles

Morteza Sadeghi et al.

JOURNAL OF MEMBRANE SCIENCE (2009)

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Review Polymer Science

High temperature proton exchange membranes based on polybenzimidazoles for fuel cells

Qingfeng Li et al.

PROGRESS IN POLYMER SCIENCE (2009)

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Article Electrochemistry

Durability studies of PBI-based high temperature PEMFCs

S. Yu et al.

FUEL CELLS (2008)

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Review Chemistry, Physical

Understanding and approaches for the durability issues of Pt-based catalysts for PEM fuel cell

Yuyan Shao et al.

JOURNAL OF POWER SOURCES (2007)

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Article Chemistry, Physical

Hydrogen crossover in high-temperature PEM fuel cells

Xuan Cheng et al.

JOURNAL OF POWER SOURCES (2007)

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Article Chemistry, Applied

The preparation and characterization of cetyltrimethylammonium intercalated muscovite

Xiaofeng Yu

MICROPOROUS AND MESOPOROUS MATERIALS (2007)

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Article Electrochemistry

Polymer electrolyte fuel cells based on phosphoric acid-impregnated poly(2,5-benzimidazole) membranes

JA Asensio et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2004)

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Review Polymer Science

Polymer/layered silicate nanocomposites: a review from preparation to processing

SS Ray et al.

PROGRESS IN POLYMER SCIENCE (2003)

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Insights into the performance and degradation of polybenzimidazole/muscovite composite membranes in high-temperature proton exchange membrane fuel cells

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