期刊
JOURNAL OF HAZARDOUS MATERIALS
卷 424, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.jhazmat.2021.127372
关键词
Plume-chasing; Vehicle emission; Emission factors; PEMS; Heavy-duty diesel vehicles
资金
- Ministry of Science and Technology of China's International Science and Technology Cooperation Program [2018YFE0106800]
- National Natural Science Foundation of China [52075481]
- Zhejiang Provincial Natural Science Foundation [LR19E050002]
- National Engineering Laboratory for MobileSource Emission Control Technology [NELMS2019A15]
- Cornell China Center
- National Science Foundation (NSF) [1605407]
- Ministry of Science and Technology of China's International Science and Technology Cooperation Program (MOST of China)
- Ministry of Science and Technology of China's International Science and Technology Cooperation Program (European Union Horizon 2020 Collaborative Project)
The study developed a new on-board measurement system to investigate the uncertainties of on-road emission factors measured by the plume-chasing method, and found that the differences in EF estimations between plume-chasing and PEMS measurements decreased with increasing chasing speed. It also observed an overprediction of chasing-based EFs in strong crosswinds due to convective plume mixing from surrounding vehicular sources.
The plume-chasing method has shown great advantages in measuring on-road emission factors (EFs) compared with regulatory methods like dynamometer and portable emission measurement systems (PEMS). In this study, a new on-board measurement system incorporating ultrasonic anemometers and solid-state Lidar was developed to investigate the uncertainties of on-road emission factors measured by plume-chasing method due to variables such as on-road wind velocity, chasing speed, chasing distance, and turbulent kinetic energy (TKE). A series of PEMS-chasing experiments for heavy-duty diesel vehicles (HDDVs) were conducted on both highways and local roadways in Beijing, China. Our analysis demonstrated that the differences in EF estimations between concurrent plume-chasing and PEMS measurement decreased with increasing chasing speed as a result of greater vehicleinduced TKE in the wake between HDDV and the mobile platform, whereas the effect of chasing distance on EF estimations appeared insignificant within the tested distance range (12-22 m). In the case of strong crosswinds, overprediction of chasing-based EFs was observed due to convective plume mixing from surrounding vehicular sources. The findings of this study contribute greatly to interpret emission factors measured by the plume-chasing method, and also calls for a future study to develop real-time EF correction algorithms for largescale mobile chasing measurements.
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