4.7 Article

Large-scale synthesis of ultra-long sodium doped MoS2 nanotubes with high electrocatalytic activity

期刊

JOURNAL OF ALLOYS AND COMPOUNDS
卷 893, 期 -, 页码 -

出版社

ELSEVIER SCIENCE SA
DOI: 10.1016/j.jallcom.2021.162362

关键词

Molybdenum disulfide(MoS2); Nanotube; Hydrothermal; Electrocatalytic activity; Scanning electron microscopy

资金

  1. National Key R&D Program of China [2017YFA0403600]
  2. Large Equipment Grants of Southeast University, China

向作者/读者索取更多资源

A low-cost method was reported in this paper to synthesize ultra-long Na-doped MoS2 nanotubes on a large scale by sulfurizing precursors produced by a hydrothermal method. These nanotubes exhibit excellent electrocatalytic activity in dye-sensitized solar cells, with a power conversion efficiency of 5.85%.
Large-scale production of high-quality molybdenum disulfide (MoS2) nanotubes is important due to their special structure and inherent properties. In this paper, we reported a low-cost approach to synthesize ultra-long Na doped MoS2 nanotubes on a large-scale by sulfurizing the precursors which produced by a hydrothermal method. Sodium chloride (NaCl) and ammonium molybdate solution are stirring in a heated water bath to prepare these precursors. Then Na doped MoS2 nanotubes are obtained by vapor-phase sulfurization using sulfur powder as S source. Transmission electron microscopy (TEM) images, X-ray dif-fraction (XRD) pattern, Raman spectra and X-ray photoelectron spectroscopy (XPS) prove the crystal structure of Na doped MoS2 with elemental composition of NaxMoS(2) (x = 0.38-0.4 4). The morphology of the samples shows pure high-quality Na doped MoS2 nanotubes with length ranging from 100 to 300 mu m. When used as the counter electrode (CE) of dye-sensitized solar cells (DSSCs), these nanotubes have excellent electrocatalytic activity. A power conversion efficiency of 5.85% is recorded in these solar cells, which is near that of the referenced Pt counter electrodes. This makes these nanotubes are ideal CEs of DSSCs. So this method is a simple and convenient approach to synthesize transition metal dichalcogenides (TMDs) nanotubes on a large scale. (C) 2021 Elsevier B.V. All rights reserved.

作者

我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。

评论

主要评分

4.7
评分不足

次要评分

新颖性
-
重要性
-
科学严谨性
-
评价这篇论文

推荐

暂无数据
暂无数据