期刊
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
卷 47, 期 7, 页码 4584-4593出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ijhydene.2021.11.093
关键词
Kitchen waste (KW); Graphene-like carbon (KW-GO); Photocatalysis produces hydrogen; VKW-GO; Recycling
资金
- National Natural Science Foundation of China [52074176]
- Shandong Society for Environmental Science [202017]
This paper investigates the use of graphene-like carbon extracted from kitchen waste to improve the photocatalytic activity and hydrogen production rate of V2O5. The addition of kitchen waste graphene-like carbon reduces the agglomeration of V2O5 and increases the specific surface area and visible light absorption range of the composite material, resulting in an enhanced hydrogen production rate. This innovative method may provide important theoretical guidance for photocatalytic hydrogen production.
In this paper, graphene-like carbon (KW-GO) extracted from kitchen waste (KW) is used to reduce the agglomeration of V2O5 and improve the separation rate of photogenerated electron-hole pairs from V2O5. We found that the V2O5-KW-GO composite material (VKW-GO) could significantly enhance the photocatalytic activity and H-2 production rate under visible light irradiation compared to pure V2O5. To analyze the composition and morphology of the materials, XRD, SEM, BET, UV-Vis, XPS, and Raman were measured. The results showed that the addition of KW-GO reduced the aggregation of V2O5 powder. At the same time, the specific surface area of the composite sample increased providing more active sites for photocatalytic hydrogen production. In addition, the visible absorption range of the composite sample also increased. As a result, the hydrogen production rate of V2O5 increased from 247.52 mol h(-1) g(-1) to 354.15 mol h(-1) g(-1). The method using V2O5 and VKW-GO as a catalyst for H-2 production is innovative, and the conclusion may provide important theoretical guidance for photocatalytic hydrogen production. (C) 2021 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
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