☆ 4.7 Review

Recent developments on transition metal-based electrocatalysts for application in anion exchange membrane water electrolysis

INTERNATIONAL JOURNAL OF ENERGY RESEARCH (2022)

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Article Electrochemistry

Overview: State-of-the Art Commercial Membranes for Anion Exchange Membrane Water Electrolysis

Dirk Henkensmeier et al.

Summary: Water electrolysis is considered a promising method for storing and distributing large amounts of renewable energy, but current technologies face challenges such as high costs and scarce catalysts. Anion exchange membrane (AEM) water electrolysis is seen as a potential solution, with advantages including low cost, high operational capacity, and fast response times.

JOURNAL OF ELECTROCHEMICAL ENERGY CONVERSION AND STORAGE (2021)

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Article Chemistry, Physical

Facile synthesis of nanoflower-like phosphorus-doped Ni3S2/CoFe2O4 arrays on nickel foam as a superior electrocatalyst for efficient oxygen evolution reaction

Jiao-Jiao Duan et al.

Summary: The research developed flower-like phosphorus doped Ni3S2/CoFe2O4 arrays on three-dimensional nickel foam via a two-step hydrothermal treatment and subsequent phosphorization, demonstrating greatly improved OER performance in 1.0 M KOH solution.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Review Engineering, Chemical

Comparison of catalyst-coated membranes and catalyst-coated substrate for PEMFC membrane electrode assembly: A review

Bee Huah Lim et al.

Summary: Catalyst-coated membranes (CCMs) have advantages in reducing platinum catalyst loading and improving catalyst-utilization efficiency compared to other methods. Considerations on material-manufacturing effects and overall performance analysis are important in MEA fabrication methods. Further research is needed to enhance fuel cell performance through the use of CCM methods in MEA fabrication.

CHINESE JOURNAL OF CHEMICAL ENGINEERING (2021)

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Article Energy & Fuels

Direct electrodeposition ofNi-Co-Son carbon paper as an efficient cathode for anion exchange membrane water electrolysers

Wenwu Guo et al.

Summary: The development of an efficient Ni-Co-S cathode for the hydrogen evolution reaction (HER) enables high activity in an anion exchange membrane water electrolizer (AEMWE). By optimizing the Ni-Co-S/CP electrode, the HER performance is enhanced, leading to a higher current density in AEMWE single cells compared to traditional Pt/C/CP cathodes. Enhancements in electron and reactant/product transfer play a key role in improving overall performance.

INTERNATIONAL JOURNAL OF ENERGY RESEARCH (2021)

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Review Chemistry, Applied

Electrodeposition: Synthesis of advanced transition metal-based catalyst for hydrogen production via electrolysis of water

Ruopeng Li et al.

Summary: This review highlights the importance and potential of electrodeposition in catalyst preparation and its application in hydrogen production. By summarizing the existing research progress and discussing the advantages of electrodeposition technology, new perspectives and directions are provided for future catalyst design and synthesis.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Article Engineering, Environmental

Free-standing nanoporous NiMnFeMo alloy: An efficient non-precious metal electrocatalyst for water splitting

Hao Liu et al.

Summary: The study introduces a flexible and free-standing nano porous NiMnFeMo alloy with ultrahigh catalytic activity for both anode and cathode in electrochemical water splitting. The alloy exhibits excellent performance even at high current density and shows superior stability when used in a water electrolyzer. DFT calculations suggest that the catalyst's activity is attributed to the synergetic effect of solid solution elements.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Active site and intermediate modulation of 3D CoSe2 nanosheet array on Ni foam by Mo doping for high-efficiency overall water splitting in alkaline media

Junlin Huang et al.

Summary: Researchers have developed a Mo-doped three-dimensional porous CoSe2 nanosheet array on commercial Ni foam, which exhibits remarkable bifunctional electrocatalytic performance in alkaline media, reducing the overpotential for hydrogen and oxygen evolution reactions while increasing the current density.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Electrochemistry

NiCu mixed metal oxide catalyst for alkaline hydrogen evolution in anion exchange membrane water electrolysis

Alaa Y. Faid et al.

Summary: The optimization of nickel-copper catalysts for cathode performance in anion exchange membrane (AEM) water electrolysis has been reported, with NiCu mixed metal oxide nanosheets showing rapid kinetics for the hydrogen evolution reaction (HER). In alkaline electrolytes, the activity and stability of NiCu MMO increase with KOH concentration, and the use of Nafion ionomer in the ink results in higher HER current density. The NiCu MMO cathode, paired with Ir black as the anode, achieves AEM electrolyzer performance comparable to PEM water electrolysis.

ELECTROCHIMICA ACTA (2021)

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Article Chemistry, Physical

Next-generation anion exchange membrane water electrolyzers operating for commercially relevant lifetimes

Behrooz Motealleh et al.

Summary: The use of Sustainion (R) anion exchange membranes in alkaline anion exchange membrane water electrolysis has shown good performance relative to industrial parameters, with stability and longer lifetime. Accelerated voltage shock tests were used to simulate daily cycling performance over 30 years, showing that performance can be improved by adding zirconia to the polymer matrix and mechanically reinforcing the membrane.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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Article Chemistry, Physical

Cobalt-Iron nanoparticles encapsulated in mesoporous carbon nanosheets: A one-pot synthesis of highly stable electrocatalysts for overall water splitting

Waleed Yaseen et al.

Summary: This study presents a simple one-pot method to synthesize cobalt-iron nanoparticles encapsulated in mesoporous carbon nanosheets for high-performance electrocatalysis. The electrocatalyst exhibits notable performance, showcasing potential for the development of cost-effective non-noble metal-based bifunctional electrocatalysts.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2021)

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Article Chemistry, Physical

Effects of the operation mode on the degradation behavior of anion exchange membrane water electrolyzers

Atif Khan Niaz et al.

Summary: In this study, the effects of different operation modes on the stability of anion exchange membrane water electrolyzers (AEMWEs) were investigated. It was found that the short periodic operation mode led to performance degradation due to ohmic resistance, while the long periodic operation mode resulted in better stability with constant resistance values. The study suggests that even small operating factors like rest time frequency can have a significant impact on cell stability.

JOURNAL OF POWER SOURCES (2021)

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Article Electrochemistry

Ionomer Optimization for Water Uptake and Swelling in Anion Exchange Membrane Electrolyzer: Hydrogen Evolution Electrode

Garrett Huang et al.

Summary: Green hydrogen produced through anion exchange membrane water electrolysis is a promising, low-cost chemical storage solution that requires a balance between ionic conductivity, water uptake, and ionomer swelling in the ACI to improve the performance of AEM-based devices. Higher IEC ACIs with light crosslinking are preferred in the HER electrode to fine-tune water uptake and ionomer swelling for optimal cell performance and reduced operating voltages.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2021)

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Article Materials Science, Multidisciplinary

Highly active non-noble electrocatalyst from Co2P/Ni2P nanohybrids for pH-universal hydrogen evolution reaction

D. Y. Li et al.

Summary: A highly porous hydrogen-evolving electrocatalyst comprising Co2P/Ni2P nanohybrids on a conductive CoNi foam demonstrates outstanding pH-universal catalytic activities for hydrogen evolution. It shows exceptional performance in a wide pH range and can bear high current densities in neutral, alkaline, and acidic solutions, outperforming most non-noble electrocatalysts and even matching or surpassing noble Pt catalysts. This discovery may pave a new avenue for the development of robust inexpensive electrocatalysts for hydrogen production in unfavorable neutral or alkaline media.

MATERIALS TODAY PHYSICS (2021)

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Article Chemistry, Physical

Controlled synthesis and high performance of Zn-Ni-Co-M (M = O, S, P and Se) nanoneedle arrays as an advanced electrode for overall water splitting

Yangyang Ding et al.

Summary: The study successfully synthesized Zn-Ni-Co-M (M = O, S, P, and Se) nanoneedle arrays on nickel foam for the first time using typical synthesis methods. The Zn-Ni-Co-S material exhibited a small overpotential for water oxidation, while the Zn-Ni-Co-P material showed a relatively small overpotential for water reduction. The assembled electrolytic cell with Zn-Ni-Co-S/NF as the positive electrode and Zn-Ni-Co-P/NF as the negative material displayed superior electrocatalytic activity and durability.

APPLIED SURFACE SCIENCE (2021)

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Article Engineering, Environmental

Selective-etching of MOF toward hierarchical porous Mo-doped CoP/N-doped carbon nanosheet arrays for efficient hydrogen evolution at all pH values

Yuanjian Li et al.

Summary: The Mo-CoP/NC/TF electrocatalysts, with optimized electronic and geometric structures, show superior activity and stability for pH-universal hydrogen evolution reaction, demonstrating potential as a viable alternative to precious metal electrocatalysts.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Electrochemistry

Development of Co/Co9S8 metallic nanowire anchored on N-doped CNTs through the pyrolysis of melamine for overall water splitting

Anchu Ashok et al.

Summary: In this study, Co9S8 metal-sulfide nanowire trapped in multi walled carbon nanotube (MWCNT) was successfully synthesized and found to be an effective catalyst for water splitting. The addition of sulfur during synthesis enhanced the surface area and oxygen vacancy defects of the nanotubes, leading to improved catalytic performance. Doping with Pyridinic-N atoms, Graphitic-N atoms and thioamide S-atoms also contributed to the enhanced electrocatalytic performance of Co/Co9S8/CNT.

ELECTROCHIMICA ACTA (2021)

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Article Electrochemistry

Enhanced electrocatalytic performance of FeNiCoP amorphous alloys as oxygen-evolving catalysts for electrolytic water splitting application

Shuangshuang Jiang et al.

Summary: Novel quaternary FeNiCoP amorphous alloys have been synthesized as self-supporting electrocatalysts for investigating OER performances. The material exhibited excellent activity in acidic solutions, with a comparable performance to IrO2 in alkaline solutions.

ELECTROCHIMICA ACTA (2021)

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Article Chemistry, Physical

Electrochemically active surface area controls HER activity for FexNi100-x films in alkaline electrolyte

Sergio I. Perez Bakovic et al.

Summary: The study found that films with higher Fe content exhibited higher electrocatalytic activity in alkaline media, while intrinsic HER activity also increased with higher Ni content. Different analysis methods revealed the effects of surface area and activity on overall measured HER activity, emphasizing the importance of ECSA.

JOURNAL OF CATALYSIS (2021)

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Article Chemistry, Physical

Multicomponent Co9S8@MoS2 nanohybrids as a novel trifunctional electrocatalyst for efficient methanol electrooxidation and overall water splitting

Linghao He et al.

Summary: In this study, Co9S8@MoS2 nanohybrids were designed and synthesized as trifunctional electrocatalysts for hydrogen evolution, oxygen evolution, and methanol oxidation reactions. The nanostructure and chemical components of the nanohybrids can be modulated by changing the mole ratios of precursors. The nanohybrid exhibited superior catalytic efficiency and low overpotential for overall water splitting at a current density of 10 mA cm(-2).

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2021)

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Article Chemistry, Physical

Active sites and optimization of mixed copper-cobalt oxide anodes for anion exchange membrane water electrolysis

E. Lopez-Fernandez et al.

Summary: The optimization of catalysts in anion exchange membrane water electrolyzers is crucial for improving the activity of the oxygen evolution reaction. Research has shown that modifying the microstructure and chemical properties of mixed copper-cobalt oxide anodes can increase the reaction activity.

JOURNAL OF POWER SOURCES (2021)

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Article Chemistry, Physical

Evaluating the effect of membrane-ionomer combinations and supporting electrolytes on the performance of cobalt nanoparticle anodes in anion exchange membrane electrolyzers

Shraboni Ghoshal et al.

Summary: This study investigates the influence of component choices and MEA fabrication in low temperature polymer electrolyte membrane electrolyzers. Changes in ionomer type, membrane, and supporting electrolyte were found to affect catalyst redox, resulting in variations in exchange current densities and Tafel slopes. Additionally, differences in membrane conductivity were identified as a key factor in performance variability among different MEAs, with higher conductivity minimizing ohmic losses.

JOURNAL OF POWER SOURCES (2021)

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Article Materials Science, Multidisciplinary

Multi-metallic electrodeposited catalysts applicable for oxygen evolution reaction in AEM water electrolysis

G. Borisov et al.

Summary: Metallic catalysts prepared by electrodeposition on carbon gas diffusion electrodes were investigated for oxygen evolution reaction in water electrolysis cells. Among the samples studied, NiFeCoP alloy demonstrated superior performance as an anode.

MATERIALS LETTERS (2021)

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Article Chemistry, Applied

Rational design of hollow oxygen deficiency-enriched NiFe2O4@N/rGO as bifunctional electrocatalysts for overall water splitting

Lei Cao et al.

Summary: Utilizing bimetallic metal organic frameworks as precursors, catalysts with bifunctional catalytic activity of oxygen evolution reaction (OER) and hydrogen evolution reaction (HER) can be prepared. The synthesized NiFe2O4 demonstrates promising catalytic performance in 1 M KOH, suggesting potential application in overall water splitting reactions.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Article Materials Science, Multidisciplinary

Recent development on self-supported transition metal-based catalysts for water electrolysis at large current density

Xin-Yu Zhang et al.

Summary: This review discusses the recent development of self-supported transition metal-based catalysts that can operate stably at high current density, focusing on their catalytic performance in three important reactions of electrolytic cells. It also generalizes some design requirements, relevant test conditions, and potential conversion of large current density catalysts. Finally, some perspectives for further development of large current density-based electrocatalysts are proposed.

APPLIED MATERIALS TODAY (2021)

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Article Chemistry, Physical

Assessment of active areas for the oxygen evolution reaction on an amorphous iridium oxide surface

Regina M. Kluge et al.

Summary: Efficient production of hydrogen from water using electrocatalysis is hindered by slow kinetics of the oxygen evolution reaction (OER). Iridium (Ir) oxide catalysts in polymer electrolyte membrane electrolysers show promising activity and stability, but the structure-activity relations are not well understood. Noise in electrochemical scanning tunnelling microscopy (n-ECSTM) measurements on amorphous iridium oxide surfaces suggest little structure-sensitivity in OER, unlike in other catalytic reactions.

JOURNAL OF CATALYSIS (2021)

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Article Engineering, Environmental

Corrosion-engineered bimetallic oxide electrode as anode for high-efficiency anion exchange membrane water electrolyzer

Jooyoung Lee et al.

Summary: The study demonstrates that corroding conventional nickel foam in the presence of exotic Fe3+ cations can transform it into a high catalytic electrode for the oxygen evolution reaction. The resulting electrode, made of densely packed Ni0.75Fe2.25O4 nanoparticles less than 5 nm in size, outperforms state-of-the-art IrO2 catalyst by requiring a lower overpotential for OER activity. This approach offers a simple, cost-effective, and scalable route to high-performance OER electrodes for efficient AEM water electrolysis.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Applied

Highly active sites of NiVB nanoparticles dispersed onto graphene nanosheets towards efficient and pH-universal overall water splitting

Muhammad Arif et al.

Summary: The study developed high-performance non-noble metal electrocatalysts for pH-universal water splitting with low overpotential. The catalyst demonstrated excellent electrocatalytic performance in various pH conditions, showing promising potential for efficient water splitting.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Review Chemistry, Physical

Recent advances in non-precious metal electrocatalysts for pH-universal hydrogen evolution reaction

Shen Zhang et al.

Summary: This review summarizes recent progress in understanding the mechanism of non-precious metal electrocatalysts for pH-universal HER, and demonstrates general approaches to overcome the limitations of electrocatalysts in a broad pH range. It also proposes perspectives and challenges for the development of pH-universal HER electrocatalysts.

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Bi-metallic cobalt-nickel phosphide nanowires for electrocatalysis of the oxygen and hydrogen evolution reactions

Isilda Amorim et al.

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Comparative study of anion exchange membranes for low-cost water electrolysis

I. Pushkareva et al.

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A highly active and durable electrocatalyst for large current density hydrogen evolution reaction

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One-step electrosynthesis of NiFe-NF electrodes for highly efficient overall water splitting

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Novel electrocatalyst of nanoporous FeP cubes prepared by fast electrodeposition coupling with acid-etching for efficient hydrogen evolution

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Co3S4 nanosheets on Ni foam via electrodeposition with sulfurization as highly active electrocatalysts for anion exchange membrane electrolyzer

Yoo Sei Park et al.

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Assessment of the FAA3-50 polymer electrolyte in combination with a NiMn2O4 anode catalyst for anion exchange membrane water electrolysis

A. Carbone et al.

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Ya Tan et al.

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The effects of morphology, microstructure and mixed-valent states of MnO2 on the oxygen evolution reaction activity in alkaline anion exchange membrane water electrolysis

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NiMn layered double hydroxide nanosheets/NiCo2O4 nanowires with surface rich high valence state metal oxide as an efficient electrocatalyst for oxygen evolution reaction

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