期刊
IEEE SENSORS JOURNAL
卷 21, 期 23, 页码 26542-26548出版社
IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC
DOI: 10.1109/JSEN.2021.3119894
关键词
Health monitoring; SF6 decomposition gases; density functional theory; gas sensors
资金
- National Key Research and Development Program [2018YFB2100100]
- National Natural Science Foundation of China [61901064]
- Graduate Research and Innovation Foundation of Chongqing, China [CYS21013, CYB21017]
- Fundamental Research Funds for Central Universities [2020CDJ-LHZZ-077]
- Natural Science Foundation of Chongqing, China [cstc2020jcyj-msxmX0397]
The study introduces H2S sensors based on metal oxide nanoparticles doped GeSe monolayer, addressing issues of poor selectivity and low sensitivity of existing sensors. The doped systems exhibit obvious interaction with H2S, excellent sensitivity, and attractive adsorption and desorption properties. Additionally, they demonstrate excellent water resistance, high thermal stability, and fascinating selectivity to H2S, verifying feasibility in practical application.
Real-time and accurate detection of H2S has been an urgent problem in industry and human health. In view of practical problems of the existing nano sensors such as poor selectivity, low sensitivity, strong or weak adsorption capacity, H2S sensors based on metal oxide nanoparticles (XO, X = Cu, Zn, Ni) doped GeSe monolayer are proposed. Compared with pure system, the improvement of the adsorption distance of doped systems proves the obvious interaction between the activated atoms and H2S. The excellent sensitivity ensures the detection effect of H2S at low concentration. The ideal adsorption energy makes doped systems have attractive adsorption and desorption properties. In addition, the excellent water resistance, high thermal stability and fascinating selectivity to H2S of doped systems verify the feasibility in practical application. This study lays a theoretical foundation for the development of new generation of wearable gas sensor for health and industrial monitoring.
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