4.7 Article

Intensification of HCl removal from flue gas using a rotor-stator reactor

期刊

FUEL
卷 310, 期 -, 页码 -

出版社

ELSEVIER SCI LTD
DOI: 10.1016/j.fuel.2021.122335

关键词

Flue gas; Hydrogen chloride; Rotor-stator reactor; Mass transfer; Process intensification

资金

  1. National Natural Science Foundation of China [22178021]

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This study investigated the intensification of HCl removal in a rotor-stator reactor, which showed better mass-transfer performance and potential economic advantages compared to conventional columns. The comparison experiments indicated that the rotor-stator reactor had a superior capability for HCl removal in flue gas, with higher KGa and lower height of a transfer unit compared to a rotating packed bed. An artificial neural network model was established to predict the KGa, demonstrating the rotor-stator reactor as an effective process intensification technology for HCl removal from flue gas.
The emission of HCl in flue gas causes serious environmental problems and its removal methods have attracted wide attention. This work investigated the intensification of HCl removal from flue gas in a rotor-stator reactor. The effects of high gravity factor, gas flow rate, water flow rate, temperature and inlet concentration of HCl on the removal efficiency of HCl, overall volumetric gas-phase mass-transfer coefficient (KGa) and height of a transfer unit in the removal of HCl by water in the rotor-stator reactor were investigated. Comparisons with conventional column indicated that the rotor-stator reactor had better mass-transfer performance and may have economic advantages in HCl removal. Comparison experiments showed that KGa and height of a transfer unit in the rotor-stator reactor were 10.9-45.2% higher and 41.5-55.7% lower, respectively, than those in a rotating packed bed, indicating that rotor-stator reactor has a superior capability for the removal of HCl in flue gas and other processes controlled by gas-side mass transfer. An artificial neural network model was established to predict the KGa of HCl removal from flue gas by water in the rotor-stator reactor. This work demonstrates that rotor-stator reactor is an effective process intensification technology for the removal of HCl from flue gas.

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