期刊
ENVIRONMENTAL SCIENCE & TECHNOLOGY
卷 55, 期 23, 页码 15766-15775出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.est.1c04034
关键词
pan-Canadian; mercury; sediment proxy; archive; model; in situ measurements; anthropogenic pollution
资金
- Environment and Climate Change Canada's under the Clean Air Regulatory Agenda (CARA)
- Climate Change and Air Pollutants (CCAP) programs
The study found that anthropogenic atmospheric Hg deposition in western Canada is showing a synchronous decreasing trend, while increasing in the east, with spatial patterns mainly driven by longitude and proximity to point sources. Recent sediment-derived Hg fluxes were consistent with wet deposition monitoring results, validating the reliability of the research method.
Mercury (Hg) is a pollutant of concern across Canada and transboundary anthropogenic Hg sources presently account for over 95% of national anthropogenic Hg deposition. This study applies novel statistical analyses of 82 high-resolution dated lake sediment cores collected from 19 regions across Canada, including nearby point sources and in remote regions and spanning a full west-east geographical range of similar to 4900 km (south of 60 degrees N and between 132 and 64 degrees W) to quantify the recent (1990-2018) spatial and temporal trends in anthropogenic atmospheric Hg deposition. Temporal trend analysis shows significant synchronous decreasing trends in post-1990 anthropogenic Hg fluxes in western Canada in contrast to increasing trends in the east, with spatial patterns largely driven by longitude and proximity to known point source(s). Recent sediment-derived Hg fluxes agreed well with the available wet deposition monitoring. Sediment-derived atmospheric Hg deposition rates also compared well to the modeled values derived from the Hg model, when lake sites located nearby (<100 km) point sources were omitted due to difficulties in comparison between the sediment-derived and modeled values at deposition hot spots. This highlights the applicability of multi-core approaches to quantify spatio-temporal changes in Hg deposition over broad geographic ranges and assess the effectiveness of regional and global Hg emission reductions to address global Hg pollution concerns.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据