期刊
ENERGY
卷 238, 期 -, 页码 -出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.energy.2021.121616
关键词
Biomass; Gasification; Aspen plus; Free-tar syngas; Simulation
资金
- National Natural Science Foundation of China [41702286]
- Innovation Fund of China National Petroleum Corporation [2018D-5007-0209]
- Sichuan Science and Technology Program [17GJHZ0061, 18GJHZ0206]
- State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation (Southwest Petroleum University) [PLN201724]
A multi-stage model for H-2 rich syngas production from biomass gasification was developed in this study. The results showed that under specific conditions, high H-2 content and carbon conversion efficiency can be achieved.
Due to its abundance, biomass is widely used in many engineering applications such as gasification process. Using biomass as a raw material for H-2-rich syngas production can not only reduce greenhouse gas emissions but also promote renewable energy utilization. In this study, a multi-stage model for H-2 rich syngas production from biomass gasification was developed and studied using Aspen Plus simulator. The model is divided into four sub-models including drying sub-model, devolatilization sub-model, tar cracking sub model and gasification sub model. Performance of biomass gasifier was evaluated by predicting the gas yield, lower heating value of produced syngas, carbon conversion efficiency and cold gas efficiency. The maximum H-2 content of 14.9 vol% was achived when S/B and reaction temperature were 1.0 and 1123 K, respectively. The highest CCE of 67.8 % and CGE of 37.9 % were also achieved at 1123 K. An increase in S/B from 0 to 0.5 led to a lower tar yield, which was from 133.557 g/Nm(3) to 127.193 g/Nm(3), and then leveled off as loading increased further from 0.5 to 1.0. The results also showed that during high S/B conditions, the gas-phase chemistry is dominated by water-gas shift (WGS) and Boudouard reactions. (C) 2021 Elsevier Ltd. All rights reserved.
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