期刊
DESALINATION
卷 517, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.desal.2021.115261
关键词
Thin-film nanocomposite; Polyamide; Graphene oxide; Multilayer assembly; Water purification
资金
- Guangdong Basic and Applied Basic Research Foundation [2020B1515120036]
- Hong Kong Scholars Program [XJ2019046]
- Research Grants Council of the Hong Kong Special Administrative Region, China [GRF HKU 17204220]
In this study, uniform and multilayered polyamide-graphene oxide TFN membranes were assembled by a simple and controllable strategy called multilayer deposition. These membranes showed significantly increased NaCl and antibiotic rejection, as well as enhanced antifouling property in reverse osmosis/nanofiltration processes.
Reverse osmosis and nanofiltration by thin-film nanocomposite (TFN) membranes are energy-efficient processes for water purification. However, it is difficult to fabricate high-performance TFN membranes in controllable manner. In this work, the uniform and multilayered polyamide (PA)-graphene oxide (GO) TFN membranes were assembled by a simple and controllable strategy, named as multilayer deposition, which was performed by consecutively spin-coating GO, meta-phenylene diamine (MPD)/piperazine (PIP), and trimesoyl chloride (TMC) solutions on the substrates. The introduction of GO could reduce defects, resulting in formation of smooth and defect-free reverse osmosis/nanofiltration membranes with significantly increased NaCl and antibiotic rejection. For example, the TFN reverse osmosis membrane showed NaCl rejection of 99.1% and water permeance of 1.83 L m(-2) h(-1) bar(-1), accompanied by substantially enhanced antifouling property.
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