期刊
CHINESE JOURNAL OF CHEMICAL ENGINEERING
卷 41, 期 -, 页码 260-266出版社
CHEMICAL INDUSTRY PRESS CO LTD
DOI: 10.1016/j.cjche.2021.09.022
关键词
Two-dimensional material; MXene membranes; Hollow fiber; Desalination; Nanofiltration
资金
- National Natural Science Foundation of China [22038006, 2192100621922805]
- Topnotch Academic Programs Project of Jiangsu Higher Education Institutions (TAPP)
This study presents the design and engineering of a two-dimensional Ti3C2Tx MXene membrane supported on an asymmetric polymeric hollow fiber substrate for water desalination. The membrane demonstrates fast water permeation and efficient rejection of divalent ions through the synergistic effect of surface hydrophilicity, electrostatic repulsion, and size sieving effect of interlayer channels.
Two-dimensional material membranes with fast transport channels and versatile chemical functionality are promising for molecular separation. Herein, for the first time, we reported design and engineering of two-dimensional Ti3C2Tx MXene (called transition metal carbides and nitrides) membranes supported on asymmetric polymeric hollow fiber substrate for water desalination. The membrane morphology, physicochemical properties and ions exclusion performance were systematically investigated. The results demonstrated that surface hydrophilicity and electrostatic repulsion and size sieving effect of interlayer channels synergistically endowed the MXene hollow fiber membrane with fast water permeation and efficient rejection of divalent ions during nanofiltration process. (C) 2021 The Chemical Industry and Engineering Society of China, and Chemical Industry Press Co., Ltd. All rights reserved.
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