期刊
CHINESE CHEMICAL LETTERS
卷 33, 期 6, 页码 2867-2882出版社
ELSEVIER SCIENCE INC
DOI: 10.1016/j.cclet.2021.10.060
关键词
Covalent organic framework nanosheets; Top-down method; Bottom-up method; Batteries; Photocatalysts; Electrocatalysts
资金
- Class D of Qianjiang Talent Program [ZD20 011250001]
- Zhejiang University of Technology [2019125016829]
- Leading Innovative and Entrepreneur Team Introduction Program of Zhejiang [2020R01002]
- National Natural Science Foundation of China [51907173]
Two-dimensional covalent organic framework nanosheets are attracting research attention due to their unique properties with great potential in energy-related applications. They provide high transport pathways for charge carriers through two typical synthetic methods. Future research will face challenges and opportunities.
Two-dimensional (2D) covalent organic framework nanosheets (CONs) are attracting increasing research attention because of their unique properties derived from their ultrathin thickness, high surface-to-volume atomic ratio, and extremely large surface area. 2D CONs can provide high transport pathways for charge carriers (e.g., electrons, holes and ions) through either the conjugated skeletons or the open channels. Therefore, they have shown great potential in energy related applications. In this review, we firstly introduce the recent developments and characteristics of 2D CONs by focusing on the two typical synthetic methods, i.e., top-down and bottom-up methods. Then, the energy-related applications in energy storage and conversion of 2D CONs are summarized. Finally, we give our personal views on the challenges and perspectives for the future research of 2D CONs and their composites. (C) 2022 Published by Elsevier B.V. on behalf of Chinese Chemical Society and Institute of Materia Medica, Chinese Academy of Medical Sciences.
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